Quantum control allows a wide range of quantum operations employed in molecular physics,nuclear magnetic resonance and quantum information processing.Thanks to the existing microelectronics industry,semiconducting qub...Quantum control allows a wide range of quantum operations employed in molecular physics,nuclear magnetic resonance and quantum information processing.Thanks to the existing microelectronics industry,semiconducting qubits,where quantum information is encoded in spin or charge degree freedom of electrons or nuclei in semiconductor quantum dots,constitute a highly competitive candidate for scalable solid-state quantum technologies.In quantum information processing,advanced control techniques are needed to realize quantum manipulations with both high precision and noise resilience.In this review,we first introduce the basics of various widely-used control methods,including resonant excitation,adabatic passage,shortcuts to adiabaticity,composite pulses,and quantum optimal control.Then we review the practical aspects in applying these methods to realize accurate and robust quantum gates for single semiconductor qubits,such as Loss–DiVincenzo spin qubit,spinglet-triplet qubit,exchange-only qubit and charge qubit.展开更多
Wide-bandgap two-dimensional (2D) β-TeO_(2) has been reported as a high-mobility p-type transparent semiconductor [Nat. Electron. 4 277 (2021)], attracting significant attention. This "breakthrough" not onl...Wide-bandgap two-dimensional (2D) β-TeO_(2) has been reported as a high-mobility p-type transparent semiconductor [Nat. Electron. 4 277 (2021)], attracting significant attention. This "breakthrough" not only challenges the conventional characterization of TeO_(2) as an insulator but also conflicts with the anticipated difficulty in hole doping of TeO_(2) by established chemical trends. Notably, the reported Fermi level of 0.9 eV above the valence band maximum actually suggests that the material is an insulator, contradicting the high hole density obtained by Hall effect measurement. Furthermore, the detected residual Se and the possible reduced elemental Te in the 2D β-TeO_(2) samples introduces complexity, considering that elemental Se, Te, and Te_(1−x)Se_(x) themselves are high-mobility p-type semiconductors. Therefore, doubts regarding the true cause of the p-type conductivity observed in the 2D β-TeO_(2) samples arise. In this Letter, we employ density functional theory calculations to illustrate that TeO_(2), whether in its bulk forms of α-, β-, or γ-TeO_(2), or in the 2D β-TeO_(2) nanosheets, inherently exhibits insulating properties and poses challenges in carrier doping due to its shallow conduction band minimum and deep valence band maximum. Our findings shed light on the insulating properties and doping difficulty of TeO_(2), contrasting with the claimed p-type conductivity in the 2D β-TeO_(2) samples, prompting inquiries into the true origin of the p-type conductivity.展开更多
基金support by the National Natural Science Foundation of China(Nos.12174379,E31Q02BG)the Chinese Academy of Sciences(Nos.E0SEBB11,E27RBB11)+1 种基金the Innovation Program for Quantum Science and Technology(No.2021ZD0302300)Chinese Academy of Sciences Project for Young Scientists in Basic Research(No.YSBR-090)。
文摘Quantum control allows a wide range of quantum operations employed in molecular physics,nuclear magnetic resonance and quantum information processing.Thanks to the existing microelectronics industry,semiconducting qubits,where quantum information is encoded in spin or charge degree freedom of electrons or nuclei in semiconductor quantum dots,constitute a highly competitive candidate for scalable solid-state quantum technologies.In quantum information processing,advanced control techniques are needed to realize quantum manipulations with both high precision and noise resilience.In this review,we first introduce the basics of various widely-used control methods,including resonant excitation,adabatic passage,shortcuts to adiabaticity,composite pulses,and quantum optimal control.Then we review the practical aspects in applying these methods to realize accurate and robust quantum gates for single semiconductor qubits,such as Loss–DiVincenzo spin qubit,spinglet-triplet qubit,exchange-only qubit and charge qubit.
基金supported by the National Natural Science Foundation of China(Grant Nos.52372150,12088101,and 11991060)the National Key R&D Program of China(Grant No.2022YFB4200305)。
文摘Wide-bandgap two-dimensional (2D) β-TeO_(2) has been reported as a high-mobility p-type transparent semiconductor [Nat. Electron. 4 277 (2021)], attracting significant attention. This "breakthrough" not only challenges the conventional characterization of TeO_(2) as an insulator but also conflicts with the anticipated difficulty in hole doping of TeO_(2) by established chemical trends. Notably, the reported Fermi level of 0.9 eV above the valence band maximum actually suggests that the material is an insulator, contradicting the high hole density obtained by Hall effect measurement. Furthermore, the detected residual Se and the possible reduced elemental Te in the 2D β-TeO_(2) samples introduces complexity, considering that elemental Se, Te, and Te_(1−x)Se_(x) themselves are high-mobility p-type semiconductors. Therefore, doubts regarding the true cause of the p-type conductivity observed in the 2D β-TeO_(2) samples arise. In this Letter, we employ density functional theory calculations to illustrate that TeO_(2), whether in its bulk forms of α-, β-, or γ-TeO_(2), or in the 2D β-TeO_(2) nanosheets, inherently exhibits insulating properties and poses challenges in carrier doping due to its shallow conduction band minimum and deep valence band maximum. Our findings shed light on the insulating properties and doping difficulty of TeO_(2), contrasting with the claimed p-type conductivity in the 2D β-TeO_(2) samples, prompting inquiries into the true origin of the p-type conductivity.
