Based on the number of asthmatic children in the Children's Hospital of Yulin City,the monitoring data of daily pollen concentration,and routine meteorological and environmental monitoring data of Yulin City from ...Based on the number of asthmatic children in the Children's Hospital of Yulin City,the monitoring data of daily pollen concentration,and routine meteorological and environmental monitoring data of Yulin City from 2020 to 2022,the meteorological and environmental conditions of a thunderstorm asthma event in Yulin City in northern Shaanxi on September 9,2022 were analyzed.The results show that the strong convective weather was accompanied by a strong thunderstorm,lightning,gusts,short-time heavy precipitation and small hail,and the convective activity lasted for nearly 7 h.The short-term abrupt change of allergenic substances such as artemisia pollen caused by lightning,gusts and precipitation,the sudden drop in temperature,the inversion near the surface and the stimulation of cold air were the key meteorological conditions for the subsequent outbreak of asthma.In early September in 2022,the daily average pollen concentration in Yulin City was up to 1067.9 particles/1000 mm^(2),which was 113.3%and 41.2%higher than that of the same period in 2021 and 2020,respectively.The day before the thunderstorm,the pollen concentration soared to 2680 particles/1000 mm^(2),reaching the maximum of the year.The synergistic effect of the thunderstorm event and the sharp increase in pollen concentration on the previous day provided the background of heavy pollen pollution for this outbreak of thunderstorm asthma.O_(3)concentration was consistently high on the day of thunderstorm and the day before,and the peaks of O_(3)and PM 10 concentration appeared subsequently in the afternoon of the day,which became the background of air pollution for the asthma outbreak.展开更多
Understanding the variations and potential source of air pollution is essential for implementing targeted mitigation actions.However,the distribution and long-term trends of Aerosol Optical Depth(AOD)and its component...Understanding the variations and potential source of air pollution is essential for implementing targeted mitigation actions.However,the distribution and long-term trends of Aerosol Optical Depth(AOD)and its components over the Fenwei Plain(FWP)have not been thoroughly investigated.Furthermore,the potential source contribution of AOD loading is still unclear.Thus,maximum synthesis and Mann-Kendall trend(MK)test with Sen's Slope methods are employed to reveal the spatiotemporal variation characteristics of AOD over the FWP.The Potential Source Contribution Function(PSCF)model was applied to analyze the potential source contribution of AOD over the FWP.Results demonstrated that the AOD in spatial pattern exhibited consistency with the topography.AOD over the FWP fluctuated annually from 2000 to 2020,with an increase in the previous decade followed by a gradual decline after 2011.There was a significant monthly variation in AOD with higher values in August(0.47±0.21)and lower in November(0.29±0.12).A positive AOD trend was confirmed from 2000 to 2010 yet a negative trend is identified from 2011 to 2020.The sulfate aerosol(AODSU)exhibited an increasing trend over an extended period.Clear-sky radiation shows a negative trend at the surface and the top of the atmosphere(TOA)from 2000 to 2010,which is consistent with the trend in AOD.The AOD in FWP was primarily influenced by local emissions,with contributions from northern and northwestern sources.This research offers an enhanced overarching comprehension of the distribution and regional climate effects of aerosols over the FWP.展开更多
Vertical distributions of aerosol optical properties based on aircraft measurements over the Loess Plateau were measured for the first time during a summertime aircraft campaign, 2013 in Shanxi, China. Data from four ...Vertical distributions of aerosol optical properties based on aircraft measurements over the Loess Plateau were measured for the first time during a summertime aircraft campaign, 2013 in Shanxi, China. Data from four flights were analyzed. The vertical distributions of aerosol optical properties including aerosol scattering coefficients（σsc）, absorption coefficients（σab）,Angstr？m exponent（α）, single scattering albedo（ω）, backscattering ratio（βsc）, aerosol mass scattering proficiency（Q sc） and aerosol surface scattering proficiency（Q sc′） were obtained. The mean statistical values of σsc were 77.45 Mm-1（at 450 nm）, 50.72 Mm-1（at 550 nm）, and32.02 Mm-1（at 700 nm）. The mean value of σab was 7.62 Mm-1（at 550 nm）. The mean values ofα, βsc and ω were 1.93, 0.15, and 0.91, respectively. Aerosol concentration decreased with altitude. Most effective diameters（ED） of aerosols were less than 0.8 μm. The vertical profiles of σsc,, α, βsc, Q sc and Q sc′ showed that the aerosol scattering properties at lower levels contributed the most to the total aerosol radiative forcing. Both α and βsc had relatively large values, suggesting that most aerosols in the observational region were small particles. The mean values of σsc, α, βsc, Q sc, Q sc′, σab and ω at different height ranges showed that most of the parameters decreased with altitude. The forty-eight hour backward trajectories of air masses during the observation days indicated that the majority of aerosols in the lower level contributed the most to the total aerosol loading, and most of these particles originated from local or regional pollution emissions.展开更多
Precipitation scavenging of aerosol particles is an important removal process in the atmosphere that can change aerosol physical and optical properties. This paper analyzes the changes in aerosol physical and optical ...Precipitation scavenging of aerosol particles is an important removal process in the atmosphere that can change aerosol physical and optical properties. This paper analyzes the changes in aerosol physical and optical properties before and after four rain events using in situ observations of mass concentration, number concentration, particle size distribution, scattering and absorption coefficients of aerosols in June and July 2013 at the Xianghe comprehensive atmospheric observation station in China. The results show the effect of rain scavenging is related to the rain intensity and duration, the wind speed and direction. During the rain events, the temporal variation of aerosol number concentration was consistent with the variation in mass concentration, but their size-resolved scavenging ratios were different. After the rain events, the increase in aerosol mass concentration began with an increase in particles with diameter ＆lt;0.8 μm [measured using an aerodynamic particle sizer（APS）], and fine particles with diameter ＆lt;0.1 μm [measured using a scanning mobility particle sizer（SMPS）]. Rainfall was most efficient at removing particles with diameter ～0.6 μm and greater than 3.5 μm. The changes in peak values of the particle number distribution（measured using the SMPS） before and after the rain events reflect the strong scavenging effect on particles within the 100–120 nm size range. The variation patterns of aerosol scattering and absorption coefficients before and after the rain events were similar, but their scavenging ratios differed, which may have been related to the aerosol particle size distribution and chemical composition.展开更多
基金Supported by the People's Government of Yulin City(2023-SF-09)Yulin Meteorological Bureau(2024Y-02)Open Research Fund Project of Key Laboratory of Ecological Environment and Meteorology in the Qinling Mountains and Loess Plateau(2022Y-21).
文摘Based on the number of asthmatic children in the Children's Hospital of Yulin City,the monitoring data of daily pollen concentration,and routine meteorological and environmental monitoring data of Yulin City from 2020 to 2022,the meteorological and environmental conditions of a thunderstorm asthma event in Yulin City in northern Shaanxi on September 9,2022 were analyzed.The results show that the strong convective weather was accompanied by a strong thunderstorm,lightning,gusts,short-time heavy precipitation and small hail,and the convective activity lasted for nearly 7 h.The short-term abrupt change of allergenic substances such as artemisia pollen caused by lightning,gusts and precipitation,the sudden drop in temperature,the inversion near the surface and the stimulation of cold air were the key meteorological conditions for the subsequent outbreak of asthma.In early September in 2022,the daily average pollen concentration in Yulin City was up to 1067.9 particles/1000 mm^(2),which was 113.3%and 41.2%higher than that of the same period in 2021 and 2020,respectively.The day before the thunderstorm,the pollen concentration soared to 2680 particles/1000 mm^(2),reaching the maximum of the year.The synergistic effect of the thunderstorm event and the sharp increase in pollen concentration on the previous day provided the background of heavy pollen pollution for this outbreak of thunderstorm asthma.O_(3)concentration was consistently high on the day of thunderstorm and the day before,and the peaks of O_(3)and PM 10 concentration appeared subsequently in the afternoon of the day,which became the background of air pollution for the asthma outbreak.
基金supported by the National Natural Science Foundation of China(No.41905016)the Key Research and Development Program of Shaanxi Province(No.2024SF-YBXM-583)+1 种基金the Key Research and Development Project of Shaanxi Province(No.2021ZDLSF-05-07)the National Key Research and Development Plan of China(No.2017YFC0212206).
文摘Understanding the variations and potential source of air pollution is essential for implementing targeted mitigation actions.However,the distribution and long-term trends of Aerosol Optical Depth(AOD)and its components over the Fenwei Plain(FWP)have not been thoroughly investigated.Furthermore,the potential source contribution of AOD loading is still unclear.Thus,maximum synthesis and Mann-Kendall trend(MK)test with Sen's Slope methods are employed to reveal the spatiotemporal variation characteristics of AOD over the FWP.The Potential Source Contribution Function(PSCF)model was applied to analyze the potential source contribution of AOD over the FWP.Results demonstrated that the AOD in spatial pattern exhibited consistency with the topography.AOD over the FWP fluctuated annually from 2000 to 2020,with an increase in the previous decade followed by a gradual decline after 2011.There was a significant monthly variation in AOD with higher values in August(0.47±0.21)and lower in November(0.29±0.12).A positive AOD trend was confirmed from 2000 to 2010 yet a negative trend is identified from 2011 to 2020.The sulfate aerosol(AODSU)exhibited an increasing trend over an extended period.Clear-sky radiation shows a negative trend at the surface and the top of the atmosphere(TOA)from 2000 to 2010,which is consistent with the trend in AOD.The AOD in FWP was primarily influenced by local emissions,with contributions from northern and northwestern sources.This research offers an enhanced overarching comprehension of the distribution and regional climate effects of aerosols over the FWP.
基金supported partially by the Ministry of Science and Technology of China under its national key project on global change studies (No.2013CB955804)the Special Fund for doctorate programs in Chinese Universities (No.20113228110002)+1 种基金the Public Meteorology Special Foundation of MOST (No.GYHY201306065)the Shanxi Meteorological Bureau Key Research Projects (No.SXKZDTC20140605)
文摘Vertical distributions of aerosol optical properties based on aircraft measurements over the Loess Plateau were measured for the first time during a summertime aircraft campaign, 2013 in Shanxi, China. Data from four flights were analyzed. The vertical distributions of aerosol optical properties including aerosol scattering coefficients（σsc）, absorption coefficients（σab）,Angstr？m exponent（α）, single scattering albedo（ω）, backscattering ratio（βsc）, aerosol mass scattering proficiency（Q sc） and aerosol surface scattering proficiency（Q sc′） were obtained. The mean statistical values of σsc were 77.45 Mm-1（at 450 nm）, 50.72 Mm-1（at 550 nm）, and32.02 Mm-1（at 700 nm）. The mean value of σab was 7.62 Mm-1（at 550 nm）. The mean values ofα, βsc and ω were 1.93, 0.15, and 0.91, respectively. Aerosol concentration decreased with altitude. Most effective diameters（ED） of aerosols were less than 0.8 μm. The vertical profiles of σsc,, α, βsc, Q sc and Q sc′ showed that the aerosol scattering properties at lower levels contributed the most to the total aerosol radiative forcing. Both α and βsc had relatively large values, suggesting that most aerosols in the observational region were small particles. The mean values of σsc, α, βsc, Q sc, Q sc′, σab and ω at different height ranges showed that most of the parameters decreased with altitude. The forty-eight hour backward trajectories of air masses during the observation days indicated that the majority of aerosols in the lower level contributed the most to the total aerosol loading, and most of these particles originated from local or regional pollution emissions.
基金supported by the National Natural Science Foundation of China(Grant No.41375155)the National Basic Program of China(973)(Grant No.2013CB955800)the China Special Fund for Meteorological Research in the Public Interest(Grant No.GYHY201306005)
文摘Precipitation scavenging of aerosol particles is an important removal process in the atmosphere that can change aerosol physical and optical properties. This paper analyzes the changes in aerosol physical and optical properties before and after four rain events using in situ observations of mass concentration, number concentration, particle size distribution, scattering and absorption coefficients of aerosols in June and July 2013 at the Xianghe comprehensive atmospheric observation station in China. The results show the effect of rain scavenging is related to the rain intensity and duration, the wind speed and direction. During the rain events, the temporal variation of aerosol number concentration was consistent with the variation in mass concentration, but their size-resolved scavenging ratios were different. After the rain events, the increase in aerosol mass concentration began with an increase in particles with diameter ＆lt;0.8 μm [measured using an aerodynamic particle sizer（APS）], and fine particles with diameter ＆lt;0.1 μm [measured using a scanning mobility particle sizer（SMPS）]. Rainfall was most efficient at removing particles with diameter ～0.6 μm and greater than 3.5 μm. The changes in peak values of the particle number distribution（measured using the SMPS） before and after the rain events reflect the strong scavenging effect on particles within the 100–120 nm size range. The variation patterns of aerosol scattering and absorption coefficients before and after the rain events were similar, but their scavenging ratios differed, which may have been related to the aerosol particle size distribution and chemical composition.
