Strong coupling between plasmons and multiple different exciton states(MESs)enables the creation of multiple hybrid polariton states under ambient conditions.These hybrid states possess unique optical properties diffe...Strong coupling between plasmons and multiple different exciton states(MESs)enables the creation of multiple hybrid polariton states under ambient conditions.These hybrid states possess unique optical properties different from those of their separate identities,making them ideal candidates for exploiting room-temperature multimode hybridization and multiqubit operation.In this study,we revealed the static spectral response properties of plasmon-MES strong coupling via a fully quantum mechanics approach.These theoretical predictions were experimentally demonstrated in plasmonic nanocavities containing two and three different exciton species.Additionally,the dynamical absorption processes of such strong coupling systems were investigated,and results indicated that the damping of the hybrid polariton states induced by the strong coupling could be markedly modulated by the acoustic oscillations from the plasmonic nanocavities.Our findings contribute a theoretical approach for accurately describing the plasmon-MES interactions and a platform for developing the high-speed active plasmonic devices based on multiqubit strong coupling.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.11874438,22105063,61905066,61805070,1200410122103024)+1 种基金Natural Science Foundation of Guangdong(Grant Nos.2021A1515010050,and 2018A030313722)Guangdong Polytechnic Normal University Talent Introduction Project Foundation of China(Grant No.XY2019022)。
文摘Strong coupling between plasmons and multiple different exciton states(MESs)enables the creation of multiple hybrid polariton states under ambient conditions.These hybrid states possess unique optical properties different from those of their separate identities,making them ideal candidates for exploiting room-temperature multimode hybridization and multiqubit operation.In this study,we revealed the static spectral response properties of plasmon-MES strong coupling via a fully quantum mechanics approach.These theoretical predictions were experimentally demonstrated in plasmonic nanocavities containing two and three different exciton species.Additionally,the dynamical absorption processes of such strong coupling systems were investigated,and results indicated that the damping of the hybrid polariton states induced by the strong coupling could be markedly modulated by the acoustic oscillations from the plasmonic nanocavities.Our findings contribute a theoretical approach for accurately describing the plasmon-MES interactions and a platform for developing the high-speed active plasmonic devices based on multiqubit strong coupling.
