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CO_(2)nanobubble-enhanced cement-fly ash backfill:Optimizing aggregate gradation and microstructure
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作者 Xiaoxiao Cao Haoyan Lyu +4 位作者 yanlong chen Jiangyu Wu Hideki Shimada Takashi Sasaoka Akihiro Hamanaka 《International Journal of Minerals,Metallurgy and Materials》 2026年第1期129-140,共12页
Mine filling materials urgently need to improve mechanical properties and achieve low-carbon transformation.This study explores the mechanism of the synergistic effect of optimizing aggregate fractal grading and intro... Mine filling materials urgently need to improve mechanical properties and achieve low-carbon transformation.This study explores the mechanism of the synergistic effect of optimizing aggregate fractal grading and introducing CO_(2)nanobubble technology to improve the performance of cement-fly ash-based backfill materials(CFB).The properties including fluidity,setting time,uniaxial compressive strength,elastic modulus,porosity,microstructure and CO_(2)storage performance were systematically studied through methods such as fluidity evaluation,time test,uniaxial compression test,mercury intrusion porosimetry(MIP),scanning electron microscopy-energy dispersive spectroscopy analysis(SEM-EDS),and thermogravimetric-differential thermogravimetric analysis(TG-DTG).The experimental results show that the density and strength of the material are significantly improved under the synergistic effect of fractal dimension and CO_(2)nanobubbles.When the fractal dimension reaches 2.65,the mass ratio of coarse and fine aggregates reaches the optimal balance,and the structural density is greatly improved at the same time.At this time,the uniaxial compressive strength and elastic modulus reach their peak values,with increases of up to 13.46%and 27.47%,respectively.CO_(2)nanobubbles enhance the material properties by promoting hydration reaction and carbonization.At the microscopic level,CO_(2)nanobubble water promotes the formation of C-S-H(hydrated calcium silicate),C-A-S-H(hydrated calcium aluminium silicate)gel and CaCO_(3),which is the main way to enhance the performance.Thermogravimetric studies have shown that when the fractal dimension is 2.65,the dehydration of hydration products and the decarbonization process of CaCO_(3)are most obvious,and CO_(2)nanobubble water promotes the carbonization reaction,making it surpass the natural state.The CO_(2)sequestration quality of cement-fly ash-based materials treated with CO_(2)nanobubble water at different fractal dimensions increased by 12.4wt%to 99.8wt%.The results not only provide scientific insights for the design and implementation of low-carbon filling materials,but also provide a solid theoretical basis for strengthening green mining practices and promoting sustainable resource utilization. 展开更多
关键词 cement-fly ash-based backfill CO_(2)nanobubble fractal dimension macro and micro performance carbon sequestration
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Accelerated optical remote sensing mapping of oil spills in the China Seas using the Segment Anything Model
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作者 Hang Lv Yingcheng Lu +5 位作者 Lifeng Wang Shuxian Song Wei Zhao yanlong chen Yuntao Wang Qingjun Song 《Acta Oceanologica Sinica》 2025年第10期184-197,共14页
Efficient segmentation of oiled pixels in optical remotely sensed images is the precondition of optical identification and classification of different spilled oils,which remains one of the keys to optical remote sensi... Efficient segmentation of oiled pixels in optical remotely sensed images is the precondition of optical identification and classification of different spilled oils,which remains one of the keys to optical remote sensing of oil spills.Optical remotely sensed images of oil spills are inherently multidimensional and embedded with a complex knowledge framework.This complexity often hinders the effectiveness of mechanistic algorithms across varied scenarios.Although optical remote-sensing theory for oil spills has advanced,the scarcity of curated datasets and the difficulty of collecting them limit their usefulness for training deep learning models.This study introduces a data expansion strategy that utilizes the Segment Anything Model(SAM),effectively bridging the gap between traditional mechanism algorithms and emergent self-adaptive deep learning models.Optical dimension reduction is achieved through standardized preprocessing processes that address the decipherable properties of the input image.After preprocessing,SAM can swiftly and accurately segment spilled oil in images.The unified AI-based workflow significantly accelerates labeled-dataset creation and has proven effective for both rapid emergency intelligence during spill incidents and the rapid mapping and classification of oil footprints across China’s coastal waters.Our results show that coupling a remote sensing mechanism with a foundation model enables near-real-time,large-scale monitoring of complex surface slicks and offers guidance for the next generation of detection and quantification algorithms. 展开更多
关键词 marine oil spills optical remote sensing segment anything model extract oil footprint spatiotemporal distribution
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Investigation of crack propagation and acoustic emission characteristics in jointed rock under freeze-thaw cycles based on DEM
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作者 Yong Zhao Qianbai Zhao +3 位作者 Tianhong Yang yanlong chen Penghai Zhang Honglei Liu 《International Journal of Mining Science and Technology》 2025年第7期1171-1195,共25页
In cold-region environments,where complex stresses and mining disturbances occur,rock masses are frequently segmented into discontinuous bodies by fractured structural planes,leading to anisotropic physical and mechan... In cold-region environments,where complex stresses and mining disturbances occur,rock masses are frequently segmented into discontinuous bodies by fractured structural planes,leading to anisotropic physical and mechanical properties.To explore the evolution of microcracks,degradation characteristics,and failure modes of fractured rocks in cold regions under the influence of freeze-thaw cycles,integrating laboratory experiments with the damage mechanics of freeze-thaw cycles.A numerical model for freeze-thaw cycle damage in rocks with various fracture dip angles was developed.The study revealed that the freeze-thaw expansion force generated during the pore water-ice phase transition is the primary driving factor behind freeze-thaw cycle damage.The initiation and propagation of microcracks and micropores,the detachment of matrix particles,and the loosening of clay mineral structures result in the transformation of the rock from a dense to a porous state,causing significant degradation in macroscopic mechanical properties.As freeze-thaw cycles increase,both the uniaxial compressive strength and the deformation modulus of the rock decrease significantly,with the failure mode gradually shifting from brittle instability to brittle-plastic or plastic failure.The findings of this study offer a practical approach to uncovering the mechanical response mechanisms between freeze-thaw damage in fractured rocks and structural planes. 展开更多
关键词 Freeze-thaw cycles Acoustic emission Micro-damage Failure mechanism Fracture dipangle
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Research on the Construction Strategies of College Yoga Courses Based on SWOT Analysis
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作者 Qian Luo yanlong chen Peng Ning 《Journal of Contemporary Educational Research》 2025年第10期340-345,共6页
This article comprehensively examines the current situation of yoga course construction in universities through the SWOT analysis method,and explores the significance and value of yoga courses in universities.The stud... This article comprehensively examines the current situation of yoga course construction in universities through the SWOT analysis method,and explores the significance and value of yoga courses in universities.The study indicates that at present,yoga courses in universities have advantages in aspects such as policy support,teacher training,student interest,and campus facilities;however,there are disadvantages in aspects such as existing teachers,course design,course promotion,and resource allocation among different universities.The opportunities for the current development of the courses lie in national policy support,increased social demand,international cooperation and exchange,and technological innovation.At the same time,the courses also face threats such as intense course competition,teacher loss,insufficient funds,and students’cognitive biases. 展开更多
关键词 SWOT analysis UNIVERSITIES Yoga courses
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Stability analysis of rib pillars in highwall mining under dynamic and static loads in open‑pit coal mine 被引量:6
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作者 Haoshuai Wu yanlong chen +3 位作者 Haoyan Lv Qihang Xie Yuanguang chen Jun Gu 《International Journal of Coal Science & Technology》 EI CAS CSCD 2022年第3期120-135,共16页
The retained coal in the end slope of an open-pit mine can be mined by the highwall mining techniques.However,the instability mechanism of the reserved rib pillar under dynamic loads of mining haul trucks and static l... The retained coal in the end slope of an open-pit mine can be mined by the highwall mining techniques.However,the instability mechanism of the reserved rib pillar under dynamic loads of mining haul trucks and static loads of the overlying strata is not clear,which restricts the safe and efcient application of highwall mining.In this study,the load-bearing model of the rib pillar in highwall mining was established,the cusp catastrophe theory and the safety coefcient of the rib pillar were considered,and the criterion equations of the rib pillar stability were proposed.Based on the limit equilibrium theory,the limit stress of the rib pillar was analyzed,and the calculation equations of plastic zone width of the rib pillar in highwall mining were obtained.Based on the Winkler foundation beam theory,the elastic foundation beam model composed of the rib pillar and roof under the highwall mining was established,and the calculation equations for the compression of the rib pillar under dynamic and static loads were developed.The results showed that with the increase of the rib pillar width,the total compression of the rib pillar under dynamic and static loads decreases nonlinearly,and the compression of the rib pillar caused by static loads of the overlying strata and trucks has a decisive role.Numerical simulation and theoretical calculation were also performed in this study.In the numerical simulation,the coal seam with a buried depth of 122 m and a thickness of 3 m is mined by highwall mining techniques.According to the established rib pillar instability model of the highwall mining system,it is found that when the mining opening width is 3 m,the reasonable width of the rib pillar is at least 1.3 m,and the safety factor of the rib pillar is 1.3.The numerical simulation results are in good agreement with the results of theoretical calculation,which verifes the feasibility of the theoretical analysis of the rib pillar stability.This research provides a reference for the stability analysis of rib pillars under highwall mining. 展开更多
关键词 Open-pit coal mine Dynamic and static loads Highwall mining Rib pillar Catastrophe instability
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Numerical modeling on strain energy evolution in rock system interaction with energy-absorbing prop and rock bolt 被引量:5
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作者 Yang Hao Chunhui Liu +4 位作者 Yu Wu Hai Pu yanlong chen Lingling Shen Guichen Li 《International Journal of Mining Science and Technology》 SCIE EI CAS CSCD 2023年第10期1273-1288,共16页
The interaction mechanism between coal and rock masses with supporting materials is significant in roadway control, especially in deep underground mining situations where dynamic hazards frequently happened due to hig... The interaction mechanism between coal and rock masses with supporting materials is significant in roadway control, especially in deep underground mining situations where dynamic hazards frequently happened due to high geo-stress and strong disturbed effects. This paper is to investigate the strain energy evolution in the interaction between coal and rock masses with self-designed energy-absorbing props and rock bolts by numerical modeling with the finite difference method. The interaction between rock and rock bolt/prop is accomplished by the cables element and the interface between the inner and outer props. Roadway excavation and coal extraction conditions in deep mining are numerically employed to investigate deformation, plastic zone ranges, strain energy input, accumulation, dissipation,and release. The effect on strain energy input, accumulation, dissipation, and release with rock deformation, and the plastic zone is addressed. A ratio of strain energy accumulation, dissipation, and release with energy input a, β, γ is to assess the dynamic hazards. The effects on roadway excavation and coal extraction steps of a, β, γ are discussed. The results show that:(1) In deep high geo-stress roadways, the energyabsorbing support system plays a dual role in resisting deformation and reducing the scope of plastic zones in surrounding rock, as well as absorbing energy release in the surrounding rock, especially in the coal extraction state to mitigate disturbed effects.(2) The strain energy input, accumulation is dependent on roadway deformation, the strain energy dissipation is relied on plastic zone area and disturbed effects, and strain energy release density is the difference among the three. The function of energyabsorbing rock bolts and props play a key role to mitigate strain energy release density and amount, especially in coal extraction condition, with a peak density value from 4×10^(4) to 1×10^(4)J/m^(3), and amount value from 3.57×10^(8) to 1.90×10^(6)J.(3) When mining is advanced in small steps, the strain energy accumulation is dominated. While in a large step, the released energy is dominant, thus a more dynamic hazards proneness. The energy-absorbing rock bolt and prop can reduce three times strain energy release amount, thus reducing the dynamic hazards. The results suggest that energy-absorbing props and rock bolts can effectively reduce the strain energy in the coal and rock masses, and prevent rock bursts and other hazards.The numerical model developed in this study can also be used to optimize the design of energyabsorbing props and rock bolts for specific mining conditions. 展开更多
关键词 Strain energy Coal and rock mass Energy-absorbing prop and rock bolt Strain energy evolution
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A fast,edge-preserving,distance-regularized model with bilateral filtering for oil spill segmentation of SAR images 被引量:4
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作者 Wandi WANG Hui SHENG +4 位作者 yanlong chen Shanwei LIU Jijun MAO Zhe ZENG Jianhua WAN 《Journal of Oceanology and Limnology》 SCIE CAS CSCD 2021年第4期1198-1210,共13页
Marine oil spills are among the most significant sources of marine pollution.Synthetic aperture radar(SAR)has been used to improve oil spill observations because of its advantages in oil spill detection and identifica... Marine oil spills are among the most significant sources of marine pollution.Synthetic aperture radar(SAR)has been used to improve oil spill observations because of its advantages in oil spill detection and identification.However,speckle noise,weak boundaries,and intensity inhomogeneity often exist in the oil spill regions of SAR imagery,which will seriously aff ect the accurate identification of oil spills.To enhance marine oil spill segmentation of SAR images,a fast,edge-preserving framework based on the distance-regularized level set evolution(DRLSE)model was proposed.Specifically,a bilateral filter penalty term is designed and incorporated into the DRLSE energy function(BF-DRLSE)to preserve the edges of oil spills,and an adaptive initial box boundary was selected for the DRLSE model to reduce the operation time complexity.Two sets of RadarSat-2 SAR data were used to test the proposed method.The experimental results indicate that the bilateral filtering scheme incorporated into the energy function during level set evolution improved the stability of level set evolution.Compared with other methods,the proposed improved BF-DRLSE algorithm displayed a higher overall segmentation accuracy(97.83%).In addition,using an appropriate initial box boundary for the DRLSE method accelerated the global search process,improved the accuracy of oil spill segmentation,and reduced computational time.Therefore,the results suggest that the proposed framework is eff ective and applicable for marine oil spill segmentation. 展开更多
关键词 level sets bilateral filter marine oil spill segmentation synthetic aperture radar(SAR)imagery
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Stability analysis of a slope containing water-sensitive mudstone considering different rainfall conditions at an open-pit mine 被引量:3
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作者 Guoyu Yang yanlong chen +3 位作者 Xuanyu Liu Ri Yang Yafei Zhang Jialong Zhang 《International Journal of Coal Science & Technology》 EI CAS CSCD 2023年第4期233-253,共21页
Mudstone, as a typical soft rock with wide distribution, has been endangering the slopes containing mudstone by its watersensitivity of swelling and weakening strength when encountering water. To comprehensively under... Mudstone, as a typical soft rock with wide distribution, has been endangering the slopes containing mudstone by its watersensitivity of swelling and weakening strength when encountering water. To comprehensively understand the water-sensitivity of mudstone and reveal its infuence on slope stability, we took the working slope containing water-sensitive mudstone of Shengli No.1 open-pit coal mine in Xilinhot, Inner Mongolia, China, as an example. Mudstone samples taken from the working slope were remodeled and saturated, and then triaxial tested to obtain the efective cohesion and efective internal friction angle. The flter paper method was used to obtain the soil–water characteristic curve of unsaturated mudstone. The pore structure of mudstone samples with diferent water contents were analyzed using the mercury intrusion porosimetry tests combined with the fractal dimension. The total pore content of the mudstone sample with lower water content is greater than that of the mudstone sample with higher water content. The mesopores are more in the mudstone sample with lower water content, while the small pores are more in the mudstone sample with higher water content. The variation of water content will change the complexity of mudstone pore structure. The higher the water content, the simpler the mudstone pore structure and the smoother the pore surface. Numerical calculations were conducted on the stability of the working slope under diferent rainfall conditions. The efective saturation on the mudstone layer surface changed and the plastic strain all occurred on the mudstone steps under diferent rainfall conditions. The key to preventing landslide of the slope containing water-sensitive mudstone in Shengli No.1 open-pit coal mine is to control the deformation and sliding of the mudstone layer. 展开更多
关键词 Water-sensitivity SWCC Pore structure Rainfall infltration Slope stability
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Validation of MODIS ocean-colour products in the coastal waters of the Yellow Sea and East China Sea 被引量:2
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作者 Lingling Jiang Xiangyu Guo +4 位作者 Lin Wang Shubha Sathyendranath Hayley Evers-King yanlong chen Bingnan Li 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2020年第1期91-101,共11页
An extensive study collected in situ data along the Yellow Sea(YS) and East China Sea(ECS) to assess the radiometric properties and the concentration of the water constituents derived from Moderate Resolution Imaging ... An extensive study collected in situ data along the Yellow Sea(YS) and East China Sea(ECS) to assess the radiometric properties and the concentration of the water constituents derived from Moderate Resolution Imaging Spectroradiometer(MODIS). Thirteen high quality match-ups were obtained for evaluating the MODIS estimates of Rrs(λ), chlorophyll a(Chl a) and concentrations of suspended particulate sediment matter(SPM). For MODIS Rrs(λ), the mean absolute percentage difference(APD) was in the range of 20%–36%, and the highest uncertainty appeared at 412 nm, whereas the band ratio of Rrs(λ) at 488 nm compared with that at 547 nm was highly consistent, with an APD of 7%. A combination of near-infrared bands and shortwave infrared wavelengths atmosphere correction algorithm(NIR-SWIR algorithm) was applied to the MODIS data, and the estimation accuracy of Rrs were improved at most of the visible spectral bands except 645 nm, 667 nm and 678 nm. Two ocean-colour empirical algorithms for Chl a estimation were applied to the processed data, the results indicated that the accuracy of the derived Chl a values was obviously improved, the four-band algorithms outperformed the other algorithm for measured and simulated datasets, and the minimum APD was 35%. The SPM was also quantified. Two regional and two coastal SPM algorithms were modified according to the in situ data. By comparison, the modified Tassan model had a higher accuracy for the application along the YS and ECS with an APD of 21%. However, given the limited match-up dataset and the potential influence of the aerosol properties on atmosphere correction, further research is required to develop additional algorithms especially for the low Chl a coastal water. 展开更多
关键词 MODIS turbid waters chlorophyll a SPM retrieval algorithms Yellow and East China Sea
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First Records of Late Triassic Conodont Fauna andδ13Ccarb from the Dengdengqiao Section,Dangchang County,Gansu Province,Northwestern China 被引量:1
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作者 Hanxiao Li Miaoyan Wang +9 位作者 Muhui Zhang Paul B.Wignall Manuel Rigo yanlong chen Xianlang Wu Zhumin Ouyang Baojin Wu Zhaoyang Yi Zaitian Zhang Xulong Lai 《Journal of Earth Science》 SCIE CAS CSCD 2021年第3期646-656,共11页
Based on a study of 49 conodont and 57 geochemical samples from the Upper Triassic,carbonate-dominated Dengdengqiao Formation,Qinling Basin,China,the Carnian conodonts and carbon isotope records are first reported.Two... Based on a study of 49 conodont and 57 geochemical samples from the Upper Triassic,carbonate-dominated Dengdengqiao Formation,Qinling Basin,China,the Carnian conodonts and carbon isotope records are first reported.Two genera and four species have been identified amongst 87 conodont elements:Mosherella praebudaensis,Mo.longnanensis sp.nov.,Mo.sp.,and"Misikella"longidentata.The presence of Mo.praebudaensis indicates that the lower part(bed 2)of the formation is attributable to the Julian(lower Carnian)substage.A radiolarian fauna identified in a previous study belongs to the upper Carnian,but the sampling horizon is unclear.Theδ13Ccarb curve shows a~1.8‰negative excursion beginning from upper part of bed 3,but its stratigraphic location is uncertain.The Dengdengqiao Formation is clearly at least partly of Carnian age but could include younger strata.The abundant calcareous algae at the section is probably due to some transport rather than preserved in site.The unusual ecosystem with rare marine organisms may reflect long-term stressful and unfavorable conditions at Dengdengqiao. 展开更多
关键词 CONODONTS Late Triassic Julian QINLING
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A multi-module with a two-way feedback method for Ulva drift-diffusion
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作者 Hui Sheng Jianmeng Li +7 位作者 Qimao Wang Bin Zou Lijian Shi Mingming Xu Shanwei Liu Jianhua Wan Zhe Zeng yanlong chen 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2023年第12期118-134,共17页
The outbreak of Ulva in the Yellow Sea has seriously affected marine ecology and economic activities.Therefore,effective prediction of the distribution of Ulva is of great significance for disaster prevention and redu... The outbreak of Ulva in the Yellow Sea has seriously affected marine ecology and economic activities.Therefore,effective prediction of the distribution of Ulva is of great significance for disaster prevention and reduction.However,the prediction method of Ulva is mainly based on numerical simulation.There are two problems with these methods.First is that the initial distribution of Ulva is simulated using independent pixel-level particles.Besides,the influence of Ulva growth and diffusion on the drift is not considered.Therefore,this paper proposes a multi-module with a two-way feedback method(MTF)to solve the above problems.The main contributions of our approach are summarized as follows.First,the initialization module,the generation and elimination module,and the drive module are composed in our way.Second,we proposed an initialization method using rectangle objects to simulate the Ulva distribution extracted from remote sensing images.Thirdly,the drift and diffusion mechanism of the Ulva is considered to realize the two-way feedback between the generation and elimination module and the drive module.The results of our experiments show that the MTF performs better than the traditional method in predicting the drift and diffusion of Ulva.The code is already publicly available at https://github.com/UPCGIT/A-multi-module-with-a-two-way-feedback-method-for-Ulva-drift-diffusion. 展开更多
关键词 ULVA remote sensing DRIFT DIFFUSION FEEDBACK
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Quality Problems and Preventive Measures for Municipal Road and Bridge Construction
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作者 yanlong chen 《Journal of Architectural Research and Development》 2019年第2期9-13,共5页
In the process of construction of municipal roads and bridges,it is especially important for the construction of waterproof roadbed.If the leakage of waterproof foundation surface will inevitably lead to the impact of... In the process of construction of municipal roads and bridges,it is especially important for the construction of waterproof roadbed.If the leakage of waterproof foundation surface will inevitably lead to the impact of the quality of roads and bridges,not only the economic and social benefits of the enterprise be lost but also threaten the safety of pedestrians'lives and property.Therefore,this paper analyzes the influencing factors in the waterproof roadbed surface of municipal road bridge construction,and proposes corresponding solutions. 展开更多
关键词 MUNICIPAL ROAD and BRIDGE CONSTRUCTION WATERPROOF ROADBED CONSTRUCTION technology
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Unprecedent green macroalgae bloom:mechanism and implication to disaster prediction and prevention 被引量:1
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作者 Mengmeng Cao Xuyan Li +15 位作者 Tingwei Cui Xinliang Pan Yan Li yanlong chen Ning Wang Yanfang Xiao Xingai Song Yuzhu Xu Runa A Bing Mu Song Qing Rongjie Liu Wenjing Zhao Yuhai Bao Jie Zhang Lan Wei 《International Journal of Digital Earth》 SCIE EI 2023年第1期3772-3793,共22页
Green macroalgae bloom(GMB),with the dominant species of Ulva prolifera,has regularly occurred since 2007 along the China coast.Although disaster prevention and control achieved favorable results in 2020,the satellite... Green macroalgae bloom(GMB),with the dominant species of Ulva prolifera,has regularly occurred since 2007 along the China coast.Although disaster prevention and control achieved favorable results in 2020,the satellite-observed GMB annual maximum coverage(AMC)rebounded sharply in 2021 to an unprecedented level.The reasons for this rebound and the significant interannual variability over past 15 years are still open questions.Here,by using long-term time-series(2007-2022)optical and Synthetic Aperture Radar satellite observations(1000+scenes),meteorological data and water quality statistics,the mechanism analysis was performed by exploring effects from natural factors and human activities.Two key determinants for AMC are successfully identified from numerous potential factors which are the macroalgae distribution in a key area(the Subei Shoal)during a critical period(from April to May 20)and the nutrient availability.Furthermore,by using these two parameters,a novel model for AMC prediction(R^(2)=0.87,p<0.01)is proposed and independently validated,which can reasonably explain the significant interannual variability(2014-2021)and agree well with the latest observation in 2022(percentage difference 12%).Finally,suggestions are proposed for future disaster prevention and alleviation.This work may aid future bloom prediction and management measure optimization. 展开更多
关键词 green macroalgae annual maximum coverage(AMC) the Yellow Sea Porphyra mariculture extreme weather water quality
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Microbial-driven ectopic uranium extraction with net electrical energy production
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作者 Xin Tang Yin Ye +9 位作者 Chunlin Wang Bingqian Wang Zemin Qin Cui Li yanlong chen Yuheng Wang Zhiling Li Miao Lv Aijie Wang Fan chen 《Frontiers of Environmental Science & Engineering》 SCIE EI CSCD 2024年第1期49-58,共10页
The extraction of uranium (U) from U-bearing wastewater is of paramount importance for mitigating negative environmental impacts and recovering U resources. Microbial reduction of soluble hexavalent uranium (U(VI)) to... The extraction of uranium (U) from U-bearing wastewater is of paramount importance for mitigating negative environmental impacts and recovering U resources. Microbial reduction of soluble hexavalent uranium (U(VI)) to insoluble tetravalent uranium (U(IV)) holds immense potential for this purpose, but its practical application has been impeded by the challenges associated with managing U-bacterial mixtures and the biotoxicity of U. To address these challenges, we present a novel spontaneous microbial electrochemical (SMEC) method that spatially decoupled the microbial oxidation reaction and the U(VI) reduction reaction. Our results demonstrated stable and efficient U extraction with net electrical energy production, which was achieved with both synthetic and real wastewater. U(VI) removal occurred via diffusion-controlled U(VI)-to-U(IV) reduction-precipitation at the cathode, and the UIVO_(2) deposited on the surface of the cathode contributed to the stability and durability of the abiotic U(VI) reduction. Metagenomic sequencing revealed the formation of efficient electroactive communities on the anodic biofilm and enrichment of the key functional genes and metabolic pathways involved in electron transfer, energy metabolism, the TCA cycle, and acetate metabolism, which indicated the ectopic reduction of U(VI) at the cathode. Our study represents a significant advancement in the cost-effective recovery of U from U(VI)-bearing wastewater and may open a new avenue for sustainable uranium extraction. 展开更多
关键词 U(VI)bioreduction Electricity production Reaction decoupling Uranium-bearing wastewater Biofilm microbiome
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