Anneal hardening has been one of the approaches to improve mechanical properties of solid solution alloys with the face-centered cubic(FCC) structure,whereby a considerable strengthening can be attained by annealing o...Anneal hardening has been one of the approaches to improve mechanical properties of solid solution alloys with the face-centered cubic(FCC) structure,whereby a considerable strengthening can be attained by annealing of cold-worked alloys below the recrystallization temperature(T_(rx)).Microscopically,this hardening effect has been ascribed to several mechanisms,i.e.solute segregation to defects(dislocation and stacking fault) and short-range chemical ordering,etc.However,none of these mechanisms can well explain the anneal hardening recently observed in phase-pure and coarse-grained FCC-structured high-entropy alloys(HEAs).Here we report the observations,using high-resolution electron channeling contrast imaging and transmission electron microscopy,of profuse and stable dislocation substructures in a cold-rolled CoCrFeMnNi HEA subject to an annealing below T_(rx).The dislocation substructures are observed to be thermally stable up to T_(rx),which could arise from the chemical complexity of the high-entropy system where certain elemental diffusion retardation occurs.The microstructure feature is markedly different from that of conventional dilute solid solution alloys,in which dislocation substructures gradually vanish by recovery during annealing,leading to a strength drop.Furthermore,dilute addition of 2 at.% Al leads to a reduction in both microhardness and yield strength of the cold-rolled and subsequently annealed(≤500℃) HEA.This Al induced softening effect,could be associated with the anisotropic formation of dislocation substructure,resulting from enhanced dislocation planar slip due to glide plane softening effect.These findings suggest that the strength of HEAs can be tailored through the anneal hardening effect from dislocation substructure strengthening.展开更多
Polypropylene （PP） was treated by an oxygen capacitively coupled radio frequency plasma （CCP） under a radio frequency （RF） power of 200 W for exposure time of 1, 5, and 10 rain. The ageing process of the plasma-...Polypropylene （PP） was treated by an oxygen capacitively coupled radio frequency plasma （CCP） under a radio frequency （RF） power of 200 W for exposure time of 1, 5, and 10 rain. The ageing process of the plasma- treated PP was studied at an ageing temperature of 90 ~C during an ageing time up to 25 h. The formation of the nanotextures with different geometry and aspect ratio and the grafting of large number of oxygen- containing groups were achieved on as-treated PP surfaces under the oxygen CCP treatment for the increased exposure time. The hydrophilicity on the as-treated PP surfaces with the stable nanotextures was rapidly depressed during the ageing process at 90 ℃ due to the restructuring of chemical composition. The surface restructuring rate was dependent on the aspect ratio and the oxygen-containing groups on the nanotextured PP with increasing exposure time. The hydrophobic over-recovery to high hydrophobicity and superhydrophobicity were observed on the post-aged surfaces with the stable nanofibrils from as-treated hydrophilic surfaces. The superhydrophobicity with the low water adhesion was achieved on the post-aged surfaces preserving the nanofibrils with high aspect ratio and large distance due to the decrease of the oxygen-containing groups after the surface restructuring.展开更多
Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limi...Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.展开更多
Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No s...Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).展开更多
基金financially supported by the National Natural Science Foundation of China (No. 52001120)the Fundamental Research Funds for the Central Universities (No. 531118010450)+10 种基金the Hundred Talent Program of Hunan Provincethe State Key Laboratory of Powder Metallurgy,Central South University,Changshathe State Key Laboratory of Advanced Metals and Materials(No. 2021-Z09)University of Science&Technology Beijing,Chinasupported by the National Natural Science Foundation of China (No. 51801060)supported by the Swedish Research Councilsupported by the National Science Foundation under Contract (No. DMR-1408722)sponsored by the Whiting School of EngineeringJohns Hopkins Universityfunded by the National Key Research and Development Program of China (No. 2016YFB0300801)the National NaturalScience Foundation of China (Nos. 51831004, 11427806, 51671082,51471067)。
文摘Anneal hardening has been one of the approaches to improve mechanical properties of solid solution alloys with the face-centered cubic(FCC) structure,whereby a considerable strengthening can be attained by annealing of cold-worked alloys below the recrystallization temperature(T_(rx)).Microscopically,this hardening effect has been ascribed to several mechanisms,i.e.solute segregation to defects(dislocation and stacking fault) and short-range chemical ordering,etc.However,none of these mechanisms can well explain the anneal hardening recently observed in phase-pure and coarse-grained FCC-structured high-entropy alloys(HEAs).Here we report the observations,using high-resolution electron channeling contrast imaging and transmission electron microscopy,of profuse and stable dislocation substructures in a cold-rolled CoCrFeMnNi HEA subject to an annealing below T_(rx).The dislocation substructures are observed to be thermally stable up to T_(rx),which could arise from the chemical complexity of the high-entropy system where certain elemental diffusion retardation occurs.The microstructure feature is markedly different from that of conventional dilute solid solution alloys,in which dislocation substructures gradually vanish by recovery during annealing,leading to a strength drop.Furthermore,dilute addition of 2 at.% Al leads to a reduction in both microhardness and yield strength of the cold-rolled and subsequently annealed(≤500℃) HEA.This Al induced softening effect,could be associated with the anisotropic formation of dislocation substructure,resulting from enhanced dislocation planar slip due to glide plane softening effect.These findings suggest that the strength of HEAs can be tailored through the anneal hardening effect from dislocation substructure strengthening.
基金supported by the projects supported by the National Natural Science Foundation of China(Nos.51005032 and 51321004)
文摘Polypropylene （PP） was treated by an oxygen capacitively coupled radio frequency plasma （CCP） under a radio frequency （RF） power of 200 W for exposure time of 1, 5, and 10 rain. The ageing process of the plasma- treated PP was studied at an ageing temperature of 90 ~C during an ageing time up to 25 h. The formation of the nanotextures with different geometry and aspect ratio and the grafting of large number of oxygen- containing groups were achieved on as-treated PP surfaces under the oxygen CCP treatment for the increased exposure time. The hydrophilicity on the as-treated PP surfaces with the stable nanotextures was rapidly depressed during the ageing process at 90 ℃ due to the restructuring of chemical composition. The surface restructuring rate was dependent on the aspect ratio and the oxygen-containing groups on the nanotextured PP with increasing exposure time. The hydrophobic over-recovery to high hydrophobicity and superhydrophobicity were observed on the post-aged surfaces with the stable nanofibrils from as-treated hydrophilic surfaces. The superhydrophobicity with the low water adhesion was achieved on the post-aged surfaces preserving the nanofibrils with high aspect ratio and large distance due to the decrease of the oxygen-containing groups after the surface restructuring.
基金supported in part by National Key R&D Program of China(2020YFA0406400,2023YFA1606000,2020YFA0406300)National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+18 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)CAS(YSBR-101)100 Talents Program of CASCAS Project for Young Scientists in Basic Research(YSBR-117)The Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID),Chile(ANID PIA/APOYO AFB230003)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.
基金Supported in part by National Key R&D Program of China(2023YFA1606000,2023YFA1606704)National Natural Science Foundation of China(NSFC)(12035009,11875170,11635010,11935015,11935016,11935018,12025502,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+16 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Program,CAS(YSBR-101)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID)Chile(ANID PIA/APOYO AFB230003)ERC(758462)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaPolish National Science Centre(2024/53/B/ST2/00975)STFC(United Kingdom)Swedish Research Council(2019.04595)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).
