The effects of acyclic liquid nitrogen(LN)treatment in a temperature range of-196℃to 50℃on the thermal and magnetic stability of Fe78Si9B13 and Fe73.5Si13.5B9Nb3Cu1 glassy ribbons have been studied.The intrinsic het...The effects of acyclic liquid nitrogen(LN)treatment in a temperature range of-196℃to 50℃on the thermal and magnetic stability of Fe78Si9B13 and Fe73.5Si13.5B9Nb3Cu1 glassy ribbons have been studied.The intrinsic heterogeneities of the metallic glasses can be activated through cryogenic thermal cycling,making irreversible structural changes after the treatment and inducing rejuvenation to the materials.The microstructural changes of both Fe-based metallic glass(MG)and nanocrystalline alloy induced by LN treatment were investigated.The experimental results show that the LN treatment could effectively rejuvenate the Fe-Si-B MGs and change their thermomechanical and magnetic properties.Based on the partially-crystallinity and well-known magnetic constants,the increase of the energy at the order of 10m J/g and magnetic domain wall movement and rotation at the order of 5-6μm and 0.5°-0.8°are found for FINEMET-type amorphous alloy after LN treatment.It is also found that LN treatment can contribute a little stored energy to the magnetic domain wall movement and magnetic domain rotation.展开更多
The fracture of metallic glasses(MGs)of different compositions and sizes down to micrometers under torsion loading were systematically investigated.Contrary to the flat shear fracture along the circumferential plane a...The fracture of metallic glasses(MGs)of different compositions and sizes down to micrometers under torsion loading were systematically investigated.Contrary to the flat shear fracture along the circumferential plane as commonly supposed under torsion,we find that the torsion fracture of metallic glasses can deviate from flat shear plane,and the fracture angle is closely dependent on the composition and the size of MG samples.With a conversion method,we show that the torsion fracture of both millimeterand micrometer-sized MGs can be described by the ellipse fracture criterion as originally proposed for the tension fracture.The deviation from the circumferential shear plane under torsion is further shown to intrinsically relate to the fracture toughness of MGs.The tougher MG tends to have a smaller fracture angle with respect to the maximum shear plane,and vice versa,indicating a correlation between the fracture toughness and pressure/normal stress sensitivity in MGs.Our results provide new insights on the fracture mechanism and are helpful to design and control the deformation and fracture behavior of MGs under torsion loading.展开更多
The structural evolution fromβ_(1)(Mg_(3)Ce)toβ(Mg_(12)Ce)precipitates,which takes place at the over-aged stage of binary Mg-Ce alloys,are investigated by high-angle annular dark-field scanning transmission electron...The structural evolution fromβ_(1)(Mg_(3)Ce)toβ(Mg_(12)Ce)precipitates,which takes place at the over-aged stage of binary Mg-Ce alloys,are investigated by high-angle annular dark-field scanning transmission electron microscopy.The structural transformation mainly occurs in the{111}_(β1)crystallographic planes,where the newly formedβlattices exhibit two categories of domain structures,namely rotational and translational domains.The rotational domain is composed of threeβdomains(β_(RA),β_(RB)andβ_(RC)),which are related by a 120°rotation with respect to each other around the 111_(β1)axis of theirβ_(1)parent phase.The{111}_(β1)crystallographic planes can provide four sets of sublattices with the same orientation for an initial nucleation ofβlattice.It leads to the formation of four translationalβdomains(β_(TA),β_(TB),β_(TC)andβ_(TD)),among which any two differ by a vector of 1/6112_(β1).We deduce theoretically that there exist twenty-fourβdomains during this transition.However,considering the interfacial misfit,only one-third of domains can grow up and eventually formsβribbon.Furthermore,a majority ofβribbons overlap partiallyβ_(1)plate,which is beneficial to relax interfacial strain amongβ,β_(1)andα-Mg matrix(α/β/β_(1)).The configuration of multipleβdomains can effectively regulate interfacial misfit ofα/βandβ/β_(1),which are responsible for enhancing the hardness and strength of Mg-Ce alloy.Additionally,this study aims to provide some clues to improve the over-aged performance of magnesium alloys by constructingβdomains and optimizing theα/β/β_(1)interface.展开更多
Small-angle X-ray scattering(SAXS)using synchrotron radiation as X-ray source has been employed to charactcizc the microscopic structrure of organo-modified mesoporous molecular sieves(organo-MSU-X)prepared by a one-p...Small-angle X-ray scattering(SAXS)using synchrotron radiation as X-ray source has been employed to charactcizc the microscopic structrure of organo-modified mesoporous molecular sieves(organo-MSU-X)prepared by a one-pot template-directed synthesis.It is shown that the SAXS profile is hardly constant with Porod’s law showing a negative slope,i.e.,negative deviation.This suggests that there is diffuse interfacial layer located between the pores and the matrix.This suggests that the organic groups remain covalently linked to the matrix,as indicated by ^29SiCP MAS NMR and FT-IR.The average thickness of the interfacial layer was found to be about 1nm for each of the three samples with different kinds and the same amounts(20? of organic groups.This kind of material has also been proved to possess both surface and mass fractal structure of the amophous porous silica materials.2001 Elsevier Science B.V.All rights reserved.展开更多
Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limi...Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.展开更多
Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No s...Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).展开更多
Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed h...Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed hadronic decaysΛ_(c)^(+)→Σ^(0)K^(+)π^(0)andΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−)and with a single-tag method.No significant signals were observed for both decays.The upper limits on the branching fractions at the 90%confidence level were determined to be 5.0×10^(-4)for and forΛ_(c)^(+)→Σ^(0)K^(+)π^(0)and 6.5×10^(-4)forΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−).展开更多
基金the National Natural Science Foundation of China(No.51871234)the National Key Research and Development Plan(No.2016YFB0300500)+2 种基金the Open Fund of Key Laboratory of Materials Preparation and Protection for Harsh Environment(Nanjing University of Aeronautics and Astronautics),Ministry of Industry and Information Technology(No.XCA19013-04)the Beijing Municipal Science&Technology Commission(No.Z191100007219006)the Key Research Program of Frontier Sciences,CAS(No.QYZDY-SSW-JSC017)。
文摘The effects of acyclic liquid nitrogen(LN)treatment in a temperature range of-196℃to 50℃on the thermal and magnetic stability of Fe78Si9B13 and Fe73.5Si13.5B9Nb3Cu1 glassy ribbons have been studied.The intrinsic heterogeneities of the metallic glasses can be activated through cryogenic thermal cycling,making irreversible structural changes after the treatment and inducing rejuvenation to the materials.The microstructural changes of both Fe-based metallic glass(MG)and nanocrystalline alloy induced by LN treatment were investigated.The experimental results show that the LN treatment could effectively rejuvenate the Fe-Si-B MGs and change their thermomechanical and magnetic properties.Based on the partially-crystallinity and well-known magnetic constants,the increase of the energy at the order of 10m J/g and magnetic domain wall movement and rotation at the order of 5-6μm and 0.5°-0.8°are found for FINEMET-type amorphous alloy after LN treatment.It is also found that LN treatment can contribute a little stored energy to the magnetic domain wall movement and magnetic domain rotation.
基金supported by the National Key Research and Development Plan(Grant No.2017YFB0903902,2018YFA0703603,2016YFB0300501)the National Natural Science Foundation of China(NSFC)(Grant No.51822107,11790291,51671121,51761135125,61888102)+1 种基金the National Natural Science Foundation of Guangdong Province(Grant No.2019B030302010)the Strategic Priority Research Program of Chinese Academy of Sciences with Grant No.XDB30000000。
文摘The fracture of metallic glasses(MGs)of different compositions and sizes down to micrometers under torsion loading were systematically investigated.Contrary to the flat shear fracture along the circumferential plane as commonly supposed under torsion,we find that the torsion fracture of metallic glasses can deviate from flat shear plane,and the fracture angle is closely dependent on the composition and the size of MG samples.With a conversion method,we show that the torsion fracture of both millimeterand micrometer-sized MGs can be described by the ellipse fracture criterion as originally proposed for the tension fracture.The deviation from the circumferential shear plane under torsion is further shown to intrinsically relate to the fracture toughness of MGs.The tougher MG tends to have a smaller fracture angle with respect to the maximum shear plane,and vice versa,indicating a correlation between the fracture toughness and pressure/normal stress sensitivity in MGs.Our results provide new insights on the fracture mechanism and are helpful to design and control the deformation and fracture behavior of MGs under torsion loading.
文摘The structural evolution fromβ_(1)(Mg_(3)Ce)toβ(Mg_(12)Ce)precipitates,which takes place at the over-aged stage of binary Mg-Ce alloys,are investigated by high-angle annular dark-field scanning transmission electron microscopy.The structural transformation mainly occurs in the{111}_(β1)crystallographic planes,where the newly formedβlattices exhibit two categories of domain structures,namely rotational and translational domains.The rotational domain is composed of threeβdomains(β_(RA),β_(RB)andβ_(RC)),which are related by a 120°rotation with respect to each other around the 111_(β1)axis of theirβ_(1)parent phase.The{111}_(β1)crystallographic planes can provide four sets of sublattices with the same orientation for an initial nucleation ofβlattice.It leads to the formation of four translationalβdomains(β_(TA),β_(TB),β_(TC)andβ_(TD)),among which any two differ by a vector of 1/6112_(β1).We deduce theoretically that there exist twenty-fourβdomains during this transition.However,considering the interfacial misfit,only one-third of domains can grow up and eventually formsβribbon.Furthermore,a majority ofβribbons overlap partiallyβ_(1)plate,which is beneficial to relax interfacial strain amongβ,β_(1)andα-Mg matrix(α/β/β_(1)).The configuration of multipleβdomains can effectively regulate interfacial misfit ofα/βandβ/β_(1),which are responsible for enhancing the hardness and strength of Mg-Ce alloy.Additionally,this study aims to provide some clues to improve the over-aged performance of magnesium alloys by constructingβdomains and optimizing theα/β/β_(1)interface.
文摘Small-angle X-ray scattering(SAXS)using synchrotron radiation as X-ray source has been employed to charactcizc the microscopic structrure of organo-modified mesoporous molecular sieves(organo-MSU-X)prepared by a one-pot template-directed synthesis.It is shown that the SAXS profile is hardly constant with Porod’s law showing a negative slope,i.e.,negative deviation.This suggests that there is diffuse interfacial layer located between the pores and the matrix.This suggests that the organic groups remain covalently linked to the matrix,as indicated by ^29SiCP MAS NMR and FT-IR.The average thickness of the interfacial layer was found to be about 1nm for each of the three samples with different kinds and the same amounts(20? of organic groups.This kind of material has also been proved to possess both surface and mass fractal structure of the amophous porous silica materials.2001 Elsevier Science B.V.All rights reserved.
基金supported in part by National Key R&D Program of China(2020YFA0406400,2023YFA1606000,2020YFA0406300)National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+18 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)CAS(YSBR-101)100 Talents Program of CASCAS Project for Young Scientists in Basic Research(YSBR-117)The Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID),Chile(ANID PIA/APOYO AFB230003)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.
基金Supported in part by National Key R&D Program of China(2023YFA1606000,2023YFA1606704)National Natural Science Foundation of China(NSFC)(12035009,11875170,11635010,11935015,11935016,11935018,12025502,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+16 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Program,CAS(YSBR-101)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID)Chile(ANID PIA/APOYO AFB230003)ERC(758462)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaPolish National Science Centre(2024/53/B/ST2/00975)STFC(United Kingdom)Swedish Research Council(2019.04595)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).
基金supported in part by National Key R&D Program of China(2020YFA0406300,2020YFA0406400,2023YFA1606000)National Natural Science Foundation of China(NSFC)(12205141,11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+16 种基金Natural Science Foundation of Hunan Province(2024JJ2044)the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyGerman Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B16F640076,B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed hadronic decaysΛ_(c)^(+)→Σ^(0)K^(+)π^(0)andΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−)and with a single-tag method.No significant signals were observed for both decays.The upper limits on the branching fractions at the 90%confidence level were determined to be 5.0×10^(-4)for and forΛ_(c)^(+)→Σ^(0)K^(+)π^(0)and 6.5×10^(-4)forΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−).
