The degradation performance of pervious concrete containing TiO_(2)/LDHs-loaded recycled aggregates for NO gas was analyzed using a gas phase catalytic degradation test device,simulating different environmental condit...The degradation performance of pervious concrete containing TiO_(2)/LDHs-loaded recycled aggregates for NO gas was analyzed using a gas phase catalytic degradation test device,simulating different environmental conditions such as load,ambient temperature,and illumination intensity,which provides theoretical support for practical engineering.The experimental results indicate that when the ambient temperature is controlled at 25℃and the illumination intensity is 30 W/m^(2),the sample prepared by soaking recycled aggregates in a 0.8%TiO_(2)/LDHs suspension exhibits the highest photocatalytic degradation rate for NO gas,reaching 72.54%.Further investigation on the influence of environmental temperature reveals that,at 25℃,the maximum photocatalytic degradation rate for NO gas is 72.9%.Moreover,at an illumination intensity of 40 W/m^(2),the maximum photocatalytic degradation rate for NO gas is 87.08%.Additionally,after three repeated photocatalytic tests,the sample demonstrates good stability,with a photocatalytic degradation rate of 58%.The nitrogen content in the eluent obtained from soaking the sample was determined to be 0.0022 mol/L,with a recovery rate of 80%.The adsorption experiment demonstrates that the sample exhibits a favorable adsorption effect on nitrate ions,reaching a maximum of 56.8%.展开更多
氧化石墨烯(graphene oxide,GO)对水泥基复合材料的调控与增强效应成为了研究的热点问题.文中系统研究了GO对水泥胶砂的流动性和物理力学性能的影响,并借助X-射线衍射(X-ray diffraction,XRD)、扫描电子显微镜(scanning electron micros...氧化石墨烯(graphene oxide,GO)对水泥基复合材料的调控与增强效应成为了研究的热点问题.文中系统研究了GO对水泥胶砂的流动性和物理力学性能的影响,并借助X-射线衍射(X-ray diffraction,XRD)、扫描电子显微镜(scanning electron microscope,SEM)等手段进行微观表证.结果表明,水泥胶砂的流动性随GO掺量的增加而降低,GO对水泥水化行为具有显著的促进作用,对水泥水化产物有调控作用,能够使水泥水化产物有序规整发展,减少微观缺陷,实验证明GO掺量为0.1%时可大幅提高水泥基复合材料的抗折强度与抗压强度.展开更多
基金Funded by the National Natural Science Foundation of China(No.52478281)the Natural Science Foundation of Zhejiang Province(No.LZ22E080003)the Science and Technology Project of Zhejiang Provincial Department of Transport(No.202225)。
文摘The degradation performance of pervious concrete containing TiO_(2)/LDHs-loaded recycled aggregates for NO gas was analyzed using a gas phase catalytic degradation test device,simulating different environmental conditions such as load,ambient temperature,and illumination intensity,which provides theoretical support for practical engineering.The experimental results indicate that when the ambient temperature is controlled at 25℃and the illumination intensity is 30 W/m^(2),the sample prepared by soaking recycled aggregates in a 0.8%TiO_(2)/LDHs suspension exhibits the highest photocatalytic degradation rate for NO gas,reaching 72.54%.Further investigation on the influence of environmental temperature reveals that,at 25℃,the maximum photocatalytic degradation rate for NO gas is 72.9%.Moreover,at an illumination intensity of 40 W/m^(2),the maximum photocatalytic degradation rate for NO gas is 87.08%.Additionally,after three repeated photocatalytic tests,the sample demonstrates good stability,with a photocatalytic degradation rate of 58%.The nitrogen content in the eluent obtained from soaking the sample was determined to be 0.0022 mol/L,with a recovery rate of 80%.The adsorption experiment demonstrates that the sample exhibits a favorable adsorption effect on nitrate ions,reaching a maximum of 56.8%.
文摘氧化石墨烯(graphene oxide,GO)对水泥基复合材料的调控与增强效应成为了研究的热点问题.文中系统研究了GO对水泥胶砂的流动性和物理力学性能的影响,并借助X-射线衍射(X-ray diffraction,XRD)、扫描电子显微镜(scanning electron microscope,SEM)等手段进行微观表证.结果表明,水泥胶砂的流动性随GO掺量的增加而降低,GO对水泥水化行为具有显著的促进作用,对水泥水化产物有调控作用,能够使水泥水化产物有序规整发展,减少微观缺陷,实验证明GO掺量为0.1%时可大幅提高水泥基复合材料的抗折强度与抗压强度.
