Optically coupled microcavities have emerged as photonic structures with promising properties for investigation of fundamental science as well as for applications.We report on the fabrication and spatially resolved sp...Optically coupled microcavities have emerged as photonic structures with promising properties for investigation of fundamental science as well as for applications.We report on the fabrication and spatially resolved spectroscopy of on-chip photonic molecule(PM)lasers consisting of two coupled,dye-doped polymeric microdisks on a silicon substrate.We investigate the fundamental lasing properties with focus on the spatial distribution of modes,the coupling dependent suppression of lasing modes,and in particular the application-oriented operation of these devices in aqueous environments.By depositing an additional polymer layer onto the lithographically structured cavities made of dye-doped poly(methyl methacrylate),coupling-gap widths below 150 nm with aspect ratios of the micro-/nanostructure exceeding 9:1 are achieved.This enables strong optical coupling at visible wavelengths despite relatively small resonator radii of 25 μm.The lasing properties of dye-doped PMs are investigated using spatially resolved micro-photoluminescence(μ-PL)spectroscopy.This technique allows for the direct imaging of whispering-gallery modes(WGMs)in the photonics molecules.For subwavelength coupling gaps,we observe lasing from delocalized eigenstates of the PMs(termed in the following as super-modes).Using size-mismatched cavities,the lasing mode suppression for different coupling-gap widths is investigated.We further demonstrate single-mode lasing operation in aqueous environments with PMs,which are realized on a low-cost,polymer-on-silicon platform.展开更多
Whole-body optical imaging of post-embryonic stage model organisms is a challenging and long sought-after goal.It requires a combination of high-resolution performance and high-penetration depth.Optoacoustic(photoacou...Whole-body optical imaging of post-embryonic stage model organisms is a challenging and long sought-after goal.It requires a combination of high-resolution performance and high-penetration depth.Optoacoustic(photoacoustic)mesoscopy holds great promise,as it penetrates deeper than optical and optoacoustic microscopy while providing high-spatial resolution.However,optoacoustic mesoscopic techniques only offer partial visibility of oriented structures,such as blood vessels,due to a limited angular detection aperture or the use of ultrasound frequencies that yield insufficient resolution.We introduce 3601 multi orientation(multi-projection)raster scan optoacoustic mesoscopy(MORSOM)based on detecting an ultra-wide frequency bandwidth(up to 160 MHz)and weighted deconvolution to synthetically enlarge the angular aperture.We report unprecedented isotropic inplane resolution at the 9–17μm range and improved signal to noise ratio in phantoms and opaque 21-day-old Zebrafish.We find that MORSOM performance defines a new operational specification for optoacoustic mesoscopy of adult organisms,with possible applications in the developmental biology of adulthood and aging.展开更多
基金This work has been supported by the DFG Research Center for Functional Nanostructures(CFN)Karlsruheby a grant from the Ministry of Science,Research,and the Arts of Baden-Wurttemberg(Grant No.Az:7713.14-300)+3 种基金by the German Federal Ministry for Education and Research BMBF(Grant No.FKZ 13N8168A)This work was partly carried out with the support of the Karlsruhe Nano Micro Facility(KNMF),a Helmholtz Research Infrastructure at KITTG gratefully acknowledges financial support of the Deutsche Telekom Stiftung and the Karlsruhe House of Young Scientists(KHYS)The authors thank the Karlsruhe School of Optics and Photonics(KSOP)for continuous support.
文摘Optically coupled microcavities have emerged as photonic structures with promising properties for investigation of fundamental science as well as for applications.We report on the fabrication and spatially resolved spectroscopy of on-chip photonic molecule(PM)lasers consisting of two coupled,dye-doped polymeric microdisks on a silicon substrate.We investigate the fundamental lasing properties with focus on the spatial distribution of modes,the coupling dependent suppression of lasing modes,and in particular the application-oriented operation of these devices in aqueous environments.By depositing an additional polymer layer onto the lithographically structured cavities made of dye-doped poly(methyl methacrylate),coupling-gap widths below 150 nm with aspect ratios of the micro-/nanostructure exceeding 9:1 are achieved.This enables strong optical coupling at visible wavelengths despite relatively small resonator radii of 25 μm.The lasing properties of dye-doped PMs are investigated using spatially resolved micro-photoluminescence(μ-PL)spectroscopy.This technique allows for the direct imaging of whispering-gallery modes(WGMs)in the photonics molecules.For subwavelength coupling gaps,we observe lasing from delocalized eigenstates of the PMs(termed in the following as super-modes).Using size-mismatched cavities,the lasing mode suppression for different coupling-gap widths is investigated.We further demonstrate single-mode lasing operation in aqueous environments with PMs,which are realized on a low-cost,polymer-on-silicon platform.
基金sponsored by the Federal Ministry of Education and Research,Photonic Science Germany,Tech2See-13N12624.
文摘Whole-body optical imaging of post-embryonic stage model organisms is a challenging and long sought-after goal.It requires a combination of high-resolution performance and high-penetration depth.Optoacoustic(photoacoustic)mesoscopy holds great promise,as it penetrates deeper than optical and optoacoustic microscopy while providing high-spatial resolution.However,optoacoustic mesoscopic techniques only offer partial visibility of oriented structures,such as blood vessels,due to a limited angular detection aperture or the use of ultrasound frequencies that yield insufficient resolution.We introduce 3601 multi orientation(multi-projection)raster scan optoacoustic mesoscopy(MORSOM)based on detecting an ultra-wide frequency bandwidth(up to 160 MHz)and weighted deconvolution to synthetically enlarge the angular aperture.We report unprecedented isotropic inplane resolution at the 9–17μm range and improved signal to noise ratio in phantoms and opaque 21-day-old Zebrafish.We find that MORSOM performance defines a new operational specification for optoacoustic mesoscopy of adult organisms,with possible applications in the developmental biology of adulthood and aging.
