We present in situ measurements of spectrally resolved X-ray scattering and X-ray diffraction from monocrystalline diamond samples heatedwith an intense pulse of heavy ions.In this way,we determine the samples’heatin...We present in situ measurements of spectrally resolved X-ray scattering and X-ray diffraction from monocrystalline diamond samples heatedwith an intense pulse of heavy ions.In this way,we determine the samples’heating dynamics and their microscopic and macroscopic structuralintegrity over a timespan of several microseconds.Connecting the ratio of elastic to inelastic scattering with state-of-the-art density functionaltheory molecular dynamics simulations allows the inference of average temperatures around 1300 K,in agreement with predictions fromstopping power calculations.The simultaneous diffraction measurements show no hints of any volumetric graphitization of the material,butdo indicate the onset of fracture in the diamond sample.Our experiments pave the way for future studies at the Facility for Antiproton andIon Research,where a substantially increased intensity of the heavy ion beam will be available.展开更多
The electrical conductivity of water under extreme temperatures and densities plays a central role in modeling planetary magnetic fields.Experimental data are vital to test theories of high-energy-densitywater and ass...The electrical conductivity of water under extreme temperatures and densities plays a central role in modeling planetary magnetic fields.Experimental data are vital to test theories of high-energy-densitywater and assess the possible development and presence of extraterrestrial life.These states are also important in biology and chemistry studies when specimens in water are confined and excited using ultrafast optical or free-electron lasers(FELs).Here we utilize femtosecond optical lasers to measure the transient reflection and transmission of ultrathin water sheet samples uniformly heated by a 13.6 nm FEL approaching a highly conducting state at electron temperatures exceeding 20000 K.The experiment probes the trajectory ofwater through the high-energy-density phase space and provides insights into changes in the index of refraction,charge carrier densities,andACelectrical conductivity at optical frequencies.At excitation energy densities exceeding 10MJ/kg,the index of refraction falls to n0.7,and the thermally excited free-carrier density reaches ne531027 m−3,which is over an order of magnitude higher than that of the electron carriers produced by direct photoionization.Significant specular reflection is observed owing to critical electron density shielding of electromagnetic waves.Themeasured optical conductivity reaches 23104 S/m,a value that is one to two orders of magnitude lower than those of simplemetals in a liquid state.At electron temperatures below 15000 K,the experimental results agreewell with the theoretical calculations using density-functional theory/molecular-dynamics simulations.With increasing temperature,the electron density increases and the system approaches a Fermi distribution.In this regime,the conductivities agree better with predictions from the Ziman theory of liquid metals.展开更多
基金support by the Federal Ministry of Education and Research(BMBF)under Grant No.05P21RFFA2supported by the Helmholtz Association under Grant No.ERC-RA-0041.
文摘We present in situ measurements of spectrally resolved X-ray scattering and X-ray diffraction from monocrystalline diamond samples heatedwith an intense pulse of heavy ions.In this way,we determine the samples’heating dynamics and their microscopic and macroscopic structuralintegrity over a timespan of several microseconds.Connecting the ratio of elastic to inelastic scattering with state-of-the-art density functionaltheory molecular dynamics simulations allows the inference of average temperatures around 1300 K,in agreement with predictions fromstopping power calculations.The simultaneous diffraction measurements show no hints of any volumetric graphitization of the material,butdo indicate the onset of fracture in the diamond sample.Our experiments pave the way for future studies at the Facility for Antiproton andIon Research,where a substantially increased intensity of the heavy ion beam will be available.
基金supported by the U.S.Department of Energy,Office of Science,Fusion Energy Science under Grant No.FWP 100182support from the Natural Sciences and Engineering Research Council of Canada(NSERC)+4 种基金supported by the U.S.Department of Energy,Office of Science,Office of Basic Energy Sciences under Contract No.DE-AC02-76SF00515support from the U.S.Department of Energy,Laboratory Directed Research and Development(LDRD)Program at SLAC National Accelerator Laboratory,under Contract No.DE-AC02-76SF00515support within the Research Unit Grant No.FOR 2440supported in part by the U.S.Department of Energy,Office of Science,Office of Workforce Development for Teachers and Scientists(WDTS)under the Science Undergraduate Laboratory Internships(SULI)Programsupport from the LOEWE Excellence Initiative of the State of Hessen.
文摘The electrical conductivity of water under extreme temperatures and densities plays a central role in modeling planetary magnetic fields.Experimental data are vital to test theories of high-energy-densitywater and assess the possible development and presence of extraterrestrial life.These states are also important in biology and chemistry studies when specimens in water are confined and excited using ultrafast optical or free-electron lasers(FELs).Here we utilize femtosecond optical lasers to measure the transient reflection and transmission of ultrathin water sheet samples uniformly heated by a 13.6 nm FEL approaching a highly conducting state at electron temperatures exceeding 20000 K.The experiment probes the trajectory ofwater through the high-energy-density phase space and provides insights into changes in the index of refraction,charge carrier densities,andACelectrical conductivity at optical frequencies.At excitation energy densities exceeding 10MJ/kg,the index of refraction falls to n0.7,and the thermally excited free-carrier density reaches ne531027 m−3,which is over an order of magnitude higher than that of the electron carriers produced by direct photoionization.Significant specular reflection is observed owing to critical electron density shielding of electromagnetic waves.Themeasured optical conductivity reaches 23104 S/m,a value that is one to two orders of magnitude lower than those of simplemetals in a liquid state.At electron temperatures below 15000 K,the experimental results agreewell with the theoretical calculations using density-functional theory/molecular-dynamics simulations.With increasing temperature,the electron density increases and the system approaches a Fermi distribution.In this regime,the conductivities agree better with predictions from the Ziman theory of liquid metals.
