The isomeric transition of thorium-229(^(229)Th),as the only known laser-accessible nuclear transition,offers the possibility for the development of a new generation of optical clocks.Solid-state nuclear optical clock...The isomeric transition of thorium-229(^(229)Th),as the only known laser-accessible nuclear transition,offers the possibility for the development of a new generation of optical clocks.Solid-state nuclear optical clock based on^(229)Th-doped crystals or thin films has attracted much attention due to its potential advantages in high stability,miniaturization,and robustness.This paper reviews the research progress of solid-state nuclear optical clock materials,analyzes the preparation,defects,and properties of the candidate solid material systems for^(229)Th,explores the influence of the local crystal environment on the nuclear transition,focuses on introducing the latest research results of crystal materials such as Th-doped CaF_(2)and LiSrAlF_(6),and looks forward to the future development direction of this field.It could provide a reference for the material selection and optimization of solid-state nuclear optical clocks.展开更多
基金supported by Zhangjiang Laboratory(Grant No.ZJSP21A001D)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0920000)the National Natural Science Foundation of China(Grant Nos.12341402 and 12341403)。
文摘The isomeric transition of thorium-229(^(229)Th),as the only known laser-accessible nuclear transition,offers the possibility for the development of a new generation of optical clocks.Solid-state nuclear optical clock based on^(229)Th-doped crystals or thin films has attracted much attention due to its potential advantages in high stability,miniaturization,and robustness.This paper reviews the research progress of solid-state nuclear optical clock materials,analyzes the preparation,defects,and properties of the candidate solid material systems for^(229)Th,explores the influence of the local crystal environment on the nuclear transition,focuses on introducing the latest research results of crystal materials such as Th-doped CaF_(2)and LiSrAlF_(6),and looks forward to the future development direction of this field.It could provide a reference for the material selection and optimization of solid-state nuclear optical clocks.