The increasing focus on electrocatalysis for sustainable hydrogen(H_(2))production has prompted significant interest in MXenes,a class of two-dimensional(2D)materials comprising metal carbides,carbonitrides,and nitrid...The increasing focus on electrocatalysis for sustainable hydrogen(H_(2))production has prompted significant interest in MXenes,a class of two-dimensional(2D)materials comprising metal carbides,carbonitrides,and nitrides.These materials exhibit intriguing chemical and physical properties,including excellent electrical conductivity and a large surface area,making them attractive candidates for the hydrogen evolution reaction(HER).This scientific review explores recent advancements in MXene-based electrocatalysts for HER kinetics.It discusses various compositions,functionalities,and explicit design principles while providing a comprehensive overview of synthesis methods,exceptional properties,and electro-catalytic approaches for H_(2) production via electrochemical reactions.Furthermore,challenges and future prospects in designing MXenes-based electrocatalysts with enhanced kinetics are highlighted,emphasizing the potential of incorporating different metals to expand the scope of electrochemical reactions.This review suggests possible efforts for developing advanced MXenes-based electrocatalysts,particularly for efficient H_(2) generation through electrochemical water-splitting reactions..展开更多
Fly ash,as a byproduct of municipal solid waste incineration,contains several kinds of pollutants,especially dissolvable salts that cause a severe challenge for fly ash disposal.Washing combined with cement kiln co-pr...Fly ash,as a byproduct of municipal solid waste incineration,contains several kinds of pollutants,especially dissolvable salts that cause a severe challenge for fly ash disposal.Washing combined with cement kiln co-processing for fly ash disposal has been applied in China.After washing,the wastewater was evaporated to produce fly ash salt(FAS).In this study,FAS was mixed the KCl and LiCl to be used as molten chloride salt for energy storage material.Twenty-three types of molten salts with various ratios of FAS-KCl-LiCl were evaluated.Thermophysical properties(melting point and latent heat)and thermal stability of these salts were characterized.The increase in FAS fraction decreased the latent heat of molten salts.Among the tested samples,the best compatibility ratio of FAS:KCl:LiCl was 10:50:40(%,in weight),with latent heat of 108.7 J/g and melting point of 333℃.This molten salt also showed good thermal stability after 1–13 h of thermal experiments,and the mass loss was less than 2%after 5 heating cycles at 600℃.By corrosion test,FAS-KCl-LiCl(10:50:40,%in weight)could be more safely used in vessels made of nickel-based alloy,but it might cause corrosion risk for stainless steel.展开更多
Correction to:Waste Disposal&Sustainable Energy(2022)4:193-203 https:/doi.0rg/10.1007/s42768-022-00110-6 The section‘Conflict of Interest'has been amended:‘Mi Yan is the Young Editorial Board member of Waste...Correction to:Waste Disposal&Sustainable Energy(2022)4:193-203 https:/doi.0rg/10.1007/s42768-022-00110-6 The section‘Conflict of Interest'has been amended:‘Mi Yan is the Young Editorial Board member of Waste Disposal&Sustainable Energy.'The revised‘Conflict of Interest'is as follows:Mi Yan is the Young Editorial Board member of Waste Disposal&Sustainable Energy.The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.展开更多
基金the financial support from the Sunway University International Research Network Grant Scheme(STR-IRNGSSET-GAMRG-01-2022)the Universiti Kebangsaan Malaysia Grant(GUP-2022-080)。
文摘The increasing focus on electrocatalysis for sustainable hydrogen(H_(2))production has prompted significant interest in MXenes,a class of two-dimensional(2D)materials comprising metal carbides,carbonitrides,and nitrides.These materials exhibit intriguing chemical and physical properties,including excellent electrical conductivity and a large surface area,making them attractive candidates for the hydrogen evolution reaction(HER).This scientific review explores recent advancements in MXene-based electrocatalysts for HER kinetics.It discusses various compositions,functionalities,and explicit design principles while providing a comprehensive overview of synthesis methods,exceptional properties,and electro-catalytic approaches for H_(2) production via electrochemical reactions.Furthermore,challenges and future prospects in designing MXenes-based electrocatalysts with enhanced kinetics are highlighted,emphasizing the potential of incorporating different metals to expand the scope of electrochemical reactions.This review suggests possible efforts for developing advanced MXenes-based electrocatalysts,particularly for efficient H_(2) generation through electrochemical water-splitting reactions..
基金support from the International Cooperation Project of Zhejiang Province(No.2019C04026)National Natural Science Foundation,China(No.51976196).
文摘Fly ash,as a byproduct of municipal solid waste incineration,contains several kinds of pollutants,especially dissolvable salts that cause a severe challenge for fly ash disposal.Washing combined with cement kiln co-processing for fly ash disposal has been applied in China.After washing,the wastewater was evaporated to produce fly ash salt(FAS).In this study,FAS was mixed the KCl and LiCl to be used as molten chloride salt for energy storage material.Twenty-three types of molten salts with various ratios of FAS-KCl-LiCl were evaluated.Thermophysical properties(melting point and latent heat)and thermal stability of these salts were characterized.The increase in FAS fraction decreased the latent heat of molten salts.Among the tested samples,the best compatibility ratio of FAS:KCl:LiCl was 10:50:40(%,in weight),with latent heat of 108.7 J/g and melting point of 333℃.This molten salt also showed good thermal stability after 1–13 h of thermal experiments,and the mass loss was less than 2%after 5 heating cycles at 600℃.By corrosion test,FAS-KCl-LiCl(10:50:40,%in weight)could be more safely used in vessels made of nickel-based alloy,but it might cause corrosion risk for stainless steel.
文摘Correction to:Waste Disposal&Sustainable Energy(2022)4:193-203 https:/doi.0rg/10.1007/s42768-022-00110-6 The section‘Conflict of Interest'has been amended:‘Mi Yan is the Young Editorial Board member of Waste Disposal&Sustainable Energy.'The revised‘Conflict of Interest'is as follows:Mi Yan is the Young Editorial Board member of Waste Disposal&Sustainable Energy.The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
