Construction of metal-organic-frame works-based composite photocatalysts has attracted much attention for the reasonable band gap and high surface areas to improve the photocatalytic activity.In this study,the ternary...Construction of metal-organic-frame works-based composite photocatalysts has attracted much attention for the reasonable band gap and high surface areas to improve the photocatalytic activity.In this study,the ternary heterojunction Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)nanocomposites were facilely prepared for the first time by a two-step method.The visible-light-promoted hydrogen production rate of 0.3%Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)reaches up to 5.26 mmol g^(-1)h^(-1),which is evidently much higher than pure UiO-66-NH_(2),ZnIn_(2)S_(4)and binary UiO-66-NH_(2)/ZnIn_(2)S_(4)composites.Such a huge improvement in the photocatalytic performance is mainly attributed to the matched band gap of ZnIn_(2)S_(4)and UiO-66-NH_(2),and the introduction of Pd NPs into photocatalysts that broaden spectral response range and promote the photon induced charge carrier separation.This work may provide a feasible approach for the design and construction of metal-organic-frameworks-based photocatalytic materials.展开更多
Photoactive WO3is attractive as a photocatalyst for green energy evolution through water splitting.In the present work,an electrochemical anodic oxidation method was used to fabricate a photo‐responsive nanotube arra...Photoactive WO3is attractive as a photocatalyst for green energy evolution through water splitting.In the present work,an electrochemical anodic oxidation method was used to fabricate a photo‐responsive nanotube array‐like WO3/W(NA‐WO3/W)photoanode from W foil as a precursor.Compared with a reference commercial WO3/W electrode,the NA‐WO3/W photoanode exhibited enhanced and stable photoelectrocatalytic(PEC)activity for visible‐light‐driven water splitting with a typical H2/O2stoichiometric ratio of2:1and quantum efficiency of approximately5.23%under visible‐light irradiation from a light‐emitting diode(λ=420nm,15mW/cm2).The greatly enhanced PEC performance of the NA‐WO3/Wphotoanode was attributed to its fast electron–hole separation rate,which resulted from the one‐dimensional nanotube array‐like structure,high crystallinity of monoclinic WO3,and strong interaction between WO3and W foil.This work paves the way to a facile route to prepare highly active photoelectrodes for solar light transfer to chemical energy.展开更多
In this work,the rare-earth doped ternary lead zirconate titanate ceramics with chemical formula of[0.3 Pb(Zn_(1/3)Nb_(2/3))O_(3)-0.7Pb(Zr_(0.52)Ti_(0.48))O_(3)]+x wt%CeO_(2)(x=0-0.5,abbreviated as 0.3PZN-0.7PZT-xCe)w...In this work,the rare-earth doped ternary lead zirconate titanate ceramics with chemical formula of[0.3 Pb(Zn_(1/3)Nb_(2/3))O_(3)-0.7Pb(Zr_(0.52)Ti_(0.48))O_(3)]+x wt%CeO_(2)(x=0-0.5,abbreviated as 0.3PZN-0.7PZT-xCe)were synthesized by a conventional solid-state reaction route,specific attentions was focused on the effects of CeO_(2)dopants on the structures and electrical properties of the 0.3PZN-0.7PZT ceramics,revealing the role conve rsion of CeO_(2)dopants with its doping amount(x).When less CeO_(2)(x≤0.2)is introduced into 0.3PZN-0.7PZT,the prepared ceramics are identified as the coexistence of rhombohedral and tetragonal phases,also involved with an increased grain size and a reduced atomic ratio of Pb/(Zr+Ti+Zn+Nb).The increased remanent polarization(Pr)and deceased coercive filed(Ec),as well as improved dielectric permittivity(er)and piezoelectric coefficient(d_(33))de monstrate the donor substitution of Ce^(3+)for Pb^(2+)at the A-site of perovskite lattice.Conversely,the introduction of excessive CeO_(2)(x>0.2)causes a reversal evolution in the electrical properties of ceramics,suggesting that some of the introduced cerium element tends to become Ce4+,which equivalently substitutes for Zr^(4+)at the B-site.Additionally,the diffused phase transition(DPT)behaviors of the 0.3PZN-0.7PZT-xCe ceramics were investigated by the modified Curie-Weiss Law.The sample with x=0.2 shows reduced DPT character and optimized electrical properties,including TC=297℃,εr=1400,d_(33)=480 pC/N,tanδ=1.6%,kp=65%,d_(33)·g_(33)=16.32×10^(-12)m^(2)/N,Pr=38.3μC/cm^(2)and Ec=1.02 kV/mm.These enhanced electrical properties not only are contributed by the donor substitution effect of Ce^(3+),but also benefit from the optimized morphotropic phase boundary that is close to the tetragonal-rich side.展开更多
High-Speed Trains (HSTs) have emerged as a mainstream mode of transportation in China, owing to their exceptional safety and efficiency. Ensuring the reliable operation of HSTs is of paramount economic and societal im...High-Speed Trains (HSTs) have emerged as a mainstream mode of transportation in China, owing to their exceptional safety and efficiency. Ensuring the reliable operation of HSTs is of paramount economic and societal importance. As critical rotating mechanical components of the transmission system, bearings make their fault diagnosis a topic of extensive attention. This paper provides a systematic review of image encoding-based bearing fault diagnosis methods tailored to the condition monitoring of HSTs. First, it categorizes the image encoding techniques applied in the field of bearing fault diagnosis. Then, a review of state-of-the-art studies has been presented, encompassing both monomodal image conversion and multimodal image fusion approaches. Finally, it highlights current challenges and proposes future research directions to advance intelligent fault diagnosis in HSTs, aiming to provide a valuable reference for researchers and engineers in the field of intelligent operation and maintenance.展开更多
In order to control the large deformation of tunnel surrounding rock,a new energy-absorbing bolt is developed.This bolt can be transformed into a rigid support when the deformation of the surrounding rock reaches the ...In order to control the large deformation of tunnel surrounding rock,a new energy-absorbing bolt is developed.This bolt can be transformed into a rigid support when the deformation of the surrounding rock reaches the length of the sleeve tube,thus preventing the surrounding rock from continuing to deform.Moreover,this bolt has a simple structure and is easy to manufacture and assemble.Then the static tensile test is conducted on the bolt specimen to test its working performance.The test results show that when the cone angle of the cone block is small,the load–displacement curve of the bolt contains three stages;when the cone angle is large,the load–displacement curve contains only two stages.Meanwhile,both the average constant resistance and the maximum absorbed energy increase linearly with the increase of cone angle.On this basis,ignoring the influence of shear stress,and it is supposed that the thickness of the sleeve tube is constant,then the theoretical calculation formula of constant resistance for the new bolt is derived,and the rationality of the formula is verified using the static tensile test results.It is found that the error of the calculated result is less than 15%when the cone angle does not exceed 15.At last,the numerical simulation method is used to analyze the performance of the new bolt.The simulation results indicate that the generation of shear stress and the change of tube thickness during the movement of the cone block are two important factors that cause theoretical errors.展开更多
Tiller number and grain size are important agronomic traits that determine grain yield in rice.Here,we demonstrate that DEFECTIVE TILLER GROWTH 1(DTG1),a member of the casein kinase 1 protein family,exerts a co-regula...Tiller number and grain size are important agronomic traits that determine grain yield in rice.Here,we demonstrate that DEFECTIVE TILLER GROWTH 1(DTG1),a member of the casein kinase 1 protein family,exerts a co-regulatory effect on tiller number and grain size.We identified a single amino acid substitution in DTG1(I357K)that caused a decrease in tiller number and an increase in grain size in NIL-dtg1.Genetic analyses revealed that DTG1 plays a pivotal role in regulation of tillering and grain size.The DTG1^(I357K) allelic variant exhibited robust functionality in suppressing tillering.We show that DTG1 is preferentially expressed in tiller buds and young panicles,and negatively regulates grain size by restricting cell proliferation in spikelet hulls.We further confirm that DTG1 functioned in grain size regulation by directly interacting with Grain Width 2(GW2),a critical grain size regulator in rice.The CRISPR/Cas9-mediated elimination of DTG1 significantly enhanced tiller number and grain size,thereby increasing rice grain yield under field conditions,thus highlighting potential value of DTG1 in rice breeding.展开更多
Background:Long non-coding ribonucleic acids(lncRNAs)regulate messenger RNA(mRNA)expression and influence cancer development and progression.Cuproptosis,a newly discovered form of cell death,plays an important role in...Background:Long non-coding ribonucleic acids(lncRNAs)regulate messenger RNA(mRNA)expression and influence cancer development and progression.Cuproptosis,a newly discovered form of cell death,plays an important role in cancer.Nonetheless,additional research investigating the association between cuproptosisrelated lncRNAs and prostate cancer(PCa)prognosis is required.Methods:Sequencing data and copy number variant data were obtained from 492 patients with PCa from The Cancer Genome Atlas(TCGA)Program.Prognostic models of PCa based on cuproptosis-related lncRNAs were constructed using a multi-level attention graph neural network(MLA-GNN)deep learning algorithm.Immune escape scoring was performed using Tumor Immune Dysfunction and Exclusion.Cellular experiments were conducted to explore the correlation between key lncRNAs and cuproptosis.Results:Data from 492 patients with PCa were randomized into two groups at a 1:1 ratio.Prognostic modeling was successfully established using MLA-GNN.Survival analysis suggested that patients could be divided into high-and low-risk groups according to model scores and that there was a significant difference in disease-free survival(DFS)(P<0.01).The area under the receiver operating characteristic(ROC)curve(AUC)indicated a strong predictive performance for the model,with AUCs of 0.913,0.847,and 0.863 for the training group and 0.815,0.907,and 0.866 for the test group at 12,36,and 60 months,respectively.The immune escape score and immune microenvironment analysis suggested that the high-risk group corresponded to a stronger immune escape and a poorer immune microenvironment(P<0.05).Cellular experiments revealed that the expression of all six key lncRNAs was upregulated in the presence of copper ion carriers(P<0.05).Conclusions:This study identified cuproptosis-related lncRNAs that were strongly associated with PCa prognosis.Key lncRNAs could affect copper metabolism and may serve as new therapeutic targets.展开更多
Biomimetic scaffolds made by synthetic materials are usually used to replace the natural tissues aimed at speeding up the skin regeneration.In this study,a flexible and cytocompatible poly(glycerol sebacate)@poly-l-la...Biomimetic scaffolds made by synthetic materials are usually used to replace the natural tissues aimed at speeding up the skin regeneration.In this study,a flexible and cytocompatible poly(glycerol sebacate)@poly-l-lactic acid(PGS@PLLA)fibrous scaffold with a core-shell structure was fabricated by coaxial electrospinning,where the shell PLLA was used to be a skeleton with pores on the fibrous surface.The fibrous morphology with pores on the surface of the prepared fibers was observed by SEM.The core-shell microstructure of PGS@PLLA fibers was confirmed by TEM and Laser Scanning Confocal Microscopy(LSCM).In addition,the prepared fibers exhibited a strong ability to repair tissues of the skin wound,where the stability of cell security and proliferation,and the lower inflammatory response were all superior to those of pure PLLA scaffold.It’s worth noting that the percentage of skin tissue was regenerated by 95%within 14 days,which suggests the potential application for electrospun-based synthetic fibrous scaffolds on wound healing.展开更多
In this work,we study gradient-based regularization methods for neural networks.We mainly focus on two regularization methods:the total variation and the Tikhonov regularization.Adding the regularization term to the t...In this work,we study gradient-based regularization methods for neural networks.We mainly focus on two regularization methods:the total variation and the Tikhonov regularization.Adding the regularization term to the training loss is equivalent to using neural networks to solve some variational problems,mostly in high dimensions in practical applications.We introduce a general framework to analyze the error between neural network solutions and true solutions to variational problems.The error consists of three parts:the approximation errors of neural networks,the quadrature errors of numerical integration,and the optimization error.We also apply the proposed framework to two-layer networks to derive a priori error estimate when the true solution belongs to the so-called Barron space.Moreover,we conduct some numerical experiments to show that neural networks can solve corresponding variational problems sufficiently well.The networks with gradient-based regularization are much more robust in image applications.展开更多
In this work,we present a new method for convex shape representation,which is regardless of the dimension of the concerned objects,using level-set approaches.To the best of our knowledge,the proposed prior is the firs...In this work,we present a new method for convex shape representation,which is regardless of the dimension of the concerned objects,using level-set approaches.To the best of our knowledge,the proposed prior is the first one which can work for high dimensional objects.Convexity prior is very useful for object completion in computer vision.It is a very challenging task to represent high dimensional convex objects.In this paper,we first prove that the convexity of the considered object is equivalent to the convexity of the associated signed distance function.Then,the second order condition of convex functions is used to characterize the shape convexity equivalently.We apply this new method to two applications:object segmentation with convexity prior and convex hull problem(especially with outliers).For both applications,the involved problems can be written as a general optimization problem with three constraints.An algorithm based on the alternating direction method of multipliers is presented for the optimization problem.Numerical experiments are conducted to verify the effectiveness of the proposed representation method and algorithm.展开更多
Correction to:Radiation Detection Technology and Methods(2024)8:1-1105.https://doi.org/10.1007/s41605-024-00463-y.In this article all authors name was missing in the springer link.It has been corrected.The original ar...Correction to:Radiation Detection Technology and Methods(2024)8:1-1105.https://doi.org/10.1007/s41605-024-00463-y.In this article all authors name was missing in the springer link.It has been corrected.The original article has been corrected.展开更多
We discuss the landscape of flavor physics at the Circular Electron-Positron Collider(CEPC),based on the nominal luminosity outlined in its Technical Design Report.The CEPC is designed to operate in multiple modes to ...We discuss the landscape of flavor physics at the Circular Electron-Positron Collider(CEPC),based on the nominal luminosity outlined in its Technical Design Report.The CEPC is designed to operate in multiple modes to address a variety of tasks.At the Z pole,the expected production of 4 Tera Z bosons will provide unique and highly precise measurements of Z boson couplings,while the substantial number of boosted heavy-flavored quarks and leptons produced in clean Z decays will facilitate investigations into their flavor physics with unprecedented precision.We investigate the prospects of measuring various physics benchmarks and discuss their implications for particle theories and phenomenological models.Our studies indicate that,with its highlighted advantages and anticipated excellent detector performance,the CEPC can explore beauty andτphysics in ways that are superior to or complementary with the Belle II and Large-Hadron-Collider-beauty experiments,potentially enabling the detection of new physics at energy scales of 10 TeV and above.This potential also extends to the observation of yet-to-be-discovered rare and exotic processes,as well as testing fundamental principles such as lepton flavor universality,lepton and baryon number conservation,etc.,making the CEPC a vibrant platform for flavor physics research.The WW threshold scan,Higgs-factory operation and top-pair productions of the CEPC further enhance its merits in this regard,especially for measuring the Cabibbo-Kobayashi-Maskawa matrix elements,and Flavor-Changing-NeutralCurrent physics of Higgs boson and top quarks.We outline the requirements for detector performance and considerations for future development to achieve the anticipated scientific goals.The role of machine learning for innovative detector design and advanced reconstruction algorithms is also stressed.The CEPC flavor physics program not only develops new capabilities for exploring flavor physics beyond existing projects but also enriches the physics opportunities of this machine.It should be remarked that,given the richness of the CEPC flavor physics,this manuscript is not meant to be a comprehensive survey,but rather an investigation of representative cases.Uncovering the full potential of flavor physics at the CEPC will require further dedicated explorations in the future.展开更多
High-performance Pb(Zr_(1−x)Ti_(x))O_(3)(PZT)piezoceramics are urgently desired by the market in view of their expanded operating temperature range,reduced property temperature dependence,and enhanced sensitivity and ...High-performance Pb(Zr_(1−x)Ti_(x))O_(3)(PZT)piezoceramics are urgently desired by the market in view of their expanded operating temperature range,reduced property temperature dependence,and enhanced sensitivity and acoustic power.In this work,we reported a kind of low-cost and high-performance 0.06BiYbO_(3)–0.94Pb(Zr_(0.48)Ti_(0.52))O_(3) ternary piezoceramics;the modifying effects of La_(2)O_(3) on this perovskite system were investigated in terms of the structures,electrical properties,and thermal depolarization behaviors of ceramics.The field-dependent dielectric and conduction properties indicated that there are close correlations among oxygen vacancies(VO),conducting electrons,and intrinsic conduction process.The degradation in ferroelectric properties observed in those samples doped with more than 0.15 wt%of La_(2)O_(3) indicated that the occupying mechanisms of La^(3+)changed from the donor substitution for Pb^(2+)to the isovalent substitution for Bi^(3+).The thermally depoling micromechanisms of ceramics were revealed from the thermodynamic processes of defect dipoles and intrinsic dipoles within ferroelectric domains.The sample doped with 0.15 wt%of La_(2)O_(3) shows excellent electrical properties with TC=387℃,d33=332 pC/N,TKε=5.81×10^(−3)℃−1,Pr=20.66μC/cm^(2),Td=356℃.The significantly enhanced electrical properties and thermal depolarization temperature benefited from the donor substitution of La3+,decreasing the oxygen vacancy concentration in the lattice and possibly optimizing the ferroelectric domain structure of ceramics.展开更多
The Circular Electron Positron Collider(CEPC)is a large scientific project initiated and hosted by China,fostered through extensive collaboration with international partners.The complex comprises four accelerators:a 3...The Circular Electron Positron Collider(CEPC)is a large scientific project initiated and hosted by China,fostered through extensive collaboration with international partners.The complex comprises four accelerators:a 30 GeV Linac,a 1.1 GeV Damping Ring,a Booster capable of achieving energies up to 180 GeV,and a Collider operating at varying energy modes(Z,W,H,and tt).The Linac and Damping Ring are situated on the surface,while the subterranean Booster and Collider are housed in a 100 km circumference underground tunnel,strategically accommodating future expansion with provisions for a potential Super Proton Proton Collider(SPPC).The CEPC primarily serves as a Higgs factory.In its baseline design with synchrotron radiation(SR)power of 30 MW per beam,it can achieve a luminosity of 5×10^(34)cm^(-2)s^(-1)per interaction point(IP),resulting in an integrated luminosity of 13 ab^(-1)for two IPs over a decade,producing 2.6 million Higgs bosons.Increasing the SR power to 50 MW per beam expands the CEPC's capability to generate 4.3 million Higgs bosons,facilitating precise measurements of Higgs coupling at sub-percent levels,exceeding the precision expected from the HL-LHC by an order of magnitude.This Technical Design Report(TDR)follows the Preliminary Conceptual Design Report(Pre-CDR,2015)and the Conceptual Design Report(CDR,2018),comprehensively detailing the machine's layout,performance metrics,physical design and analysis,technical systems design,R&D and prototyping efforts,and associated civil engineering aspects.Additionally,it includes a cost estimate and a preliminary construction timeline,establishing a framework for forthcoming engineering design phase and site selection procedures.Construction is anticipated to begin around 2027-2028,pending government approval,with an estimated duration of 8 years.The commencement of experiments and data collection could potentially be initiated in the mid-2030s.展开更多
As a typical Aurivillius-type compound, CaBi_(4)Ti_(4)O_(15) (CBT) is considered a strong competitor among hightemperature piezoelectric materials, but it is difficult to achieve both high piezoelectric activity and a...As a typical Aurivillius-type compound, CaBi_(4)Ti_(4)O_(15) (CBT) is considered a strong competitor among hightemperature piezoelectric materials, but it is difficult to achieve both high piezoelectric activity and a high Curie temperaturefor CBT. In this work, the method of double-ion co-substituting at different crystalline sites was used to modify the electricalproperties of CBT. The Gd/Mn co-doped CBT ceramics with the chemical formula of Ca_(1−x)Gd_(x)Bi_(4)Ti_(4)O_(15)+0.2 wt% MnO_(2)(CBT–100xGM, x = 0–0.11) were prepared via the conventional sintering process. The phase and valence band structures,chemical compositions and microstructures, dielectric and ferroelectric properties, electrical conduction behaviors, andelectroelastic and piezoelectric properties of the ceramics were characterized. The doping concentration effects of Gd^(3+)were analyzed according to the composition-dependent structures and properties of CBT–100xGM. The donor substitutionof Gd^(3+) for Ca^(2+) at the A-site reduced the tolerance factor of the perovskite-like structure and decreased the concentration ofintrinsic oxygen vacancies. While Mn^(3+) tended to substitute for Ti4+ at the B-site, the extrinsic oxygen vacancies are limitednear the defect center of Ti(Mn) because of the formation of ( ‒MnTi')• as defect dipoles. The thermal depoling behavior ofthe CBT–100xGM ceramics between 300 and 700 ℃ was explained by the thermodynamic characteristics of the defectdipoles. The optimized composition with x = 0.08 (CBT–8GM) had a high TC ≈ 809 ℃ and a high piezoelectric coefficient(d33) ≈ 23 pC/N, as well as a piezoelectric voltage constant (g33) value of up to 21.5×10^(−3)(V·m)/N. Moreover, it can maintaina residual d33 ≈ 80% after being annealed at 700 ℃. This good anti-thermal depoling ability endows this material with greatapplication potential in high-temperature piezoelectric devices with operating temperatures exceeding 500 ℃. Thesynergistic enhancement in the piezoelectric activity and Curie temperature of CBT can be attributed mainly to the donorsubstituting effect of Gd^(3+) at the A-site, as well as the decreased elastic compliance contributed by MnO_(2) as the B-sitedopant.展开更多
Recently,high-performance lead zirconate titanate(Pb(Zr_(1-x)Ti_(x))O_(3),PZT)ferroelectric ceramics have attracted intensive attention due to their wider operating temperature range,better temperature stability,as we...Recently,high-performance lead zirconate titanate(Pb(Zr_(1-x)Ti_(x))O_(3),PZT)ferroelectric ceramics have attracted intensive attention due to their wider operating temperature range,better temperature stability,as well as larger piezoelectric properties and higher energy conversion efficiency.In this study,the perovskite-type ferroelectric ceramics with a chemical formula of Pb_(0.99-x)Gd_(0.01)Sr_(x)Zr_(0.53)Ti_(0.47)O_(3)(x=0 and 0.02,abbr.PGZT and PGSZT,respectively)were prepared by the traditional solid-state reaction route.The influences of Sr-doping on the phase structure,dielectric properties,ferroelectric properties and piezoelectric properties of the PGZT ceramics were comprehensively investigated.The field-dependent P–E hysteresis loops of PGSZT were measured in the frequency range of 0.05–10 Hz and temperature range of 20–100℃.The results show that Sr-doping not only enhances the dielectric permittivity and piezoelectric coefficient of PGZT,but also decreases its dielectric loss tangent,with the d_(33) value of 473 pC/N,ε_(r) value of 1586 and tanδvalue of 0.016 found in PGSZT.Also,PGSZT shows a high Curie temperature(T_(C))of 350℃.The underlying mechanisms of the property enhancement were identified as that the introduced Sr^(2+) replaces the volatile Pb^(2+) located at the A-site of the perovskite structure,thereby reducing the concentration of lead vacancies and promoting the grain growth of the ceramics,consequently enhancing the dielectric and piezoelectric properties of PGZT.On the other hand,the frequency change in the low-frequency range(<1 Hz)played a significant impact on the remanent polarization(P_(r))and internal biased electric field(E_(i))of PGSZT,but the frequency dependence of coercive field(E_(c))tends to diminish in the high-frequency range(≥1 Hz).展开更多
I.EXECUTIVE SUMMARY next-generation,high-intensity electron-positron collider"Higgs factory",such as the Circular Electron-Positron Collider(CEPC),is among the highest priorities for the global high-energy c...I.EXECUTIVE SUMMARY next-generation,high-intensity electron-positron collider"Higgs factory",such as the Circular Electron-Positron Collider(CEPC),is among the highest priorities for the global high-energy collider physics community.The CEPC can provide unprecedented opportunities for making fundamental discoveries and providing decisive insights in the quest for a"New Standard Model(SM)"of nature's fundamental interactions.The CEPC could:·Identify the origin of matter,especially the mechanism related to the first-order phase transition in the early Universe,which could produce a detectable gravitational wave signal.展开更多
基金the Natural Science Foundation of Shanghai(No.19ZR1403500)the National Natural Science Foundation of China(No.21373054)the Natural Science Foundation of Shanghai Science and Technology Committee(No.19DZ2270100)。
文摘Construction of metal-organic-frame works-based composite photocatalysts has attracted much attention for the reasonable band gap and high surface areas to improve the photocatalytic activity.In this study,the ternary heterojunction Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)nanocomposites were facilely prepared for the first time by a two-step method.The visible-light-promoted hydrogen production rate of 0.3%Pd@UiO-66-NH_(2)@ZnIn_(2)S_(4)reaches up to 5.26 mmol g^(-1)h^(-1),which is evidently much higher than pure UiO-66-NH_(2),ZnIn_(2)S_(4)and binary UiO-66-NH_(2)/ZnIn_(2)S_(4)composites.Such a huge improvement in the photocatalytic performance is mainly attributed to the matched band gap of ZnIn_(2)S_(4)and UiO-66-NH_(2),and the introduction of Pd NPs into photocatalysts that broaden spectral response range and promote the photon induced charge carrier separation.This work may provide a feasible approach for the design and construction of metal-organic-frameworks-based photocatalytic materials.
基金supported by the National Natural Science Foundation of China(21207090,21477079,21261140333)PCSIRT(IRT1269)a scheme administrated by Shanghai Normal University(DXL122,and S30406)~~
文摘Photoactive WO3is attractive as a photocatalyst for green energy evolution through water splitting.In the present work,an electrochemical anodic oxidation method was used to fabricate a photo‐responsive nanotube array‐like WO3/W(NA‐WO3/W)photoanode from W foil as a precursor.Compared with a reference commercial WO3/W electrode,the NA‐WO3/W photoanode exhibited enhanced and stable photoelectrocatalytic(PEC)activity for visible‐light‐driven water splitting with a typical H2/O2stoichiometric ratio of2:1and quantum efficiency of approximately5.23%under visible‐light irradiation from a light‐emitting diode(λ=420nm,15mW/cm2).The greatly enhanced PEC performance of the NA‐WO3/Wphotoanode was attributed to its fast electron–hole separation rate,which resulted from the one‐dimensional nanotube array‐like structure,high crystallinity of monoclinic WO3,and strong interaction between WO3and W foil.This work paves the way to a facile route to prepare highly active photoelectrodes for solar light transfer to chemical energy.
基金Project supported by the Natural Science Foundation of Sichuan Province(2024NSFSC0219)。
文摘In this work,the rare-earth doped ternary lead zirconate titanate ceramics with chemical formula of[0.3 Pb(Zn_(1/3)Nb_(2/3))O_(3)-0.7Pb(Zr_(0.52)Ti_(0.48))O_(3)]+x wt%CeO_(2)(x=0-0.5,abbreviated as 0.3PZN-0.7PZT-xCe)were synthesized by a conventional solid-state reaction route,specific attentions was focused on the effects of CeO_(2)dopants on the structures and electrical properties of the 0.3PZN-0.7PZT ceramics,revealing the role conve rsion of CeO_(2)dopants with its doping amount(x).When less CeO_(2)(x≤0.2)is introduced into 0.3PZN-0.7PZT,the prepared ceramics are identified as the coexistence of rhombohedral and tetragonal phases,also involved with an increased grain size and a reduced atomic ratio of Pb/(Zr+Ti+Zn+Nb).The increased remanent polarization(Pr)and deceased coercive filed(Ec),as well as improved dielectric permittivity(er)and piezoelectric coefficient(d_(33))de monstrate the donor substitution of Ce^(3+)for Pb^(2+)at the A-site of perovskite lattice.Conversely,the introduction of excessive CeO_(2)(x>0.2)causes a reversal evolution in the electrical properties of ceramics,suggesting that some of the introduced cerium element tends to become Ce4+,which equivalently substitutes for Zr^(4+)at the B-site.Additionally,the diffused phase transition(DPT)behaviors of the 0.3PZN-0.7PZT-xCe ceramics were investigated by the modified Curie-Weiss Law.The sample with x=0.2 shows reduced DPT character and optimized electrical properties,including TC=297℃,εr=1400,d_(33)=480 pC/N,tanδ=1.6%,kp=65%,d_(33)·g_(33)=16.32×10^(-12)m^(2)/N,Pr=38.3μC/cm^(2)and Ec=1.02 kV/mm.These enhanced electrical properties not only are contributed by the donor substitution effect of Ce^(3+),but also benefit from the optimized morphotropic phase boundary that is close to the tetragonal-rich side.
基金supported by the Fundamental Research Funds for the Central Universities(No.2024JBZX027)the National Natural Science Foundation of China(No.52375078).
文摘High-Speed Trains (HSTs) have emerged as a mainstream mode of transportation in China, owing to their exceptional safety and efficiency. Ensuring the reliable operation of HSTs is of paramount economic and societal importance. As critical rotating mechanical components of the transmission system, bearings make their fault diagnosis a topic of extensive attention. This paper provides a systematic review of image encoding-based bearing fault diagnosis methods tailored to the condition monitoring of HSTs. First, it categorizes the image encoding techniques applied in the field of bearing fault diagnosis. Then, a review of state-of-the-art studies has been presented, encompassing both monomodal image conversion and multimodal image fusion approaches. Finally, it highlights current challenges and proposes future research directions to advance intelligent fault diagnosis in HSTs, aiming to provide a valuable reference for researchers and engineers in the field of intelligent operation and maintenance.
基金The paper is supported by the National Natural Science Foundation of China(Nos.52178393 and 52178354)the Housing and Urban-Rural Construction Science and Technology Planning Project of Shaanxi Province(No.2019-K39)the Innovation Capability Support Plan of Shaanxi-Innovation Team(No.2020TD-005).
文摘In order to control the large deformation of tunnel surrounding rock,a new energy-absorbing bolt is developed.This bolt can be transformed into a rigid support when the deformation of the surrounding rock reaches the length of the sleeve tube,thus preventing the surrounding rock from continuing to deform.Moreover,this bolt has a simple structure and is easy to manufacture and assemble.Then the static tensile test is conducted on the bolt specimen to test its working performance.The test results show that when the cone angle of the cone block is small,the load–displacement curve of the bolt contains three stages;when the cone angle is large,the load–displacement curve contains only two stages.Meanwhile,both the average constant resistance and the maximum absorbed energy increase linearly with the increase of cone angle.On this basis,ignoring the influence of shear stress,and it is supposed that the thickness of the sleeve tube is constant,then the theoretical calculation formula of constant resistance for the new bolt is derived,and the rationality of the formula is verified using the static tensile test results.It is found that the error of the calculated result is less than 15%when the cone angle does not exceed 15.At last,the numerical simulation method is used to analyze the performance of the new bolt.The simulation results indicate that the generation of shear stress and the change of tube thickness during the movement of the cone block are two important factors that cause theoretical errors.
基金supported by the Sichuan Science and Technology Support Project (2022ZDZX0012,2021YFYZ0016,2023YFN0007,2021YFYZ0027)the National Natural Science Foundation of China (32171966,U23A20180).
文摘Tiller number and grain size are important agronomic traits that determine grain yield in rice.Here,we demonstrate that DEFECTIVE TILLER GROWTH 1(DTG1),a member of the casein kinase 1 protein family,exerts a co-regulatory effect on tiller number and grain size.We identified a single amino acid substitution in DTG1(I357K)that caused a decrease in tiller number and an increase in grain size in NIL-dtg1.Genetic analyses revealed that DTG1 plays a pivotal role in regulation of tillering and grain size.The DTG1^(I357K) allelic variant exhibited robust functionality in suppressing tillering.We show that DTG1 is preferentially expressed in tiller buds and young panicles,and negatively regulates grain size by restricting cell proliferation in spikelet hulls.We further confirm that DTG1 functioned in grain size regulation by directly interacting with Grain Width 2(GW2),a critical grain size regulator in rice.The CRISPR/Cas9-mediated elimination of DTG1 significantly enhanced tiller number and grain size,thereby increasing rice grain yield under field conditions,thus highlighting potential value of DTG1 in rice breeding.
基金supported by grants from the National Natural Science Foundation of China(Nos.82372912,81802527,81972471,82073408,81974395,and 82173036)National Key Research and Development Program of China(Nos.2022YFC3602900 and 2022YFC3602904)+13 种基金BeijingBethune CharitableFoundation(Nos.mnzl202001 and mnzl202026)Guangzhou Science and Technology Project(Nos.202206010078 and 202201020574)Sun Yat-sen University Clinical Research 5010 Program(Nos.2018007 and 2019005)Sun Yat-sen Clinical Research Cultivating Program(No.SYS-C-201801)Guangdong Medical Science and Technology Program(No.A2020558)Tencent Charity Foundation(No.7670020025)Scientific Research Launch Project of Sun Yat-sen Memorial Hospital(No.YXQH202209)GuangdongBasicand AppliedBasicResearchFoundation(No.2019A1515011437)International Science and Technology Cooperation Project Plan of Guangdong Province(No.2021A0505030085)Guangzhou Science and Technology Key R&D Project(No.202206010117)Beijing CSCO Clinical Oncology Research Foundation(No.Y-tongshu2021/ms-0162)Guangdong Provincial Clinical Research Center for Urological Diseases(No.2020B1111170006)Guangdong Science and Technology Department(No.2020B1212060018)open research funds from the Sixth Affiliated Hospital of Guangzhou Medical University,Qingyuan People's Hospital.
文摘Background:Long non-coding ribonucleic acids(lncRNAs)regulate messenger RNA(mRNA)expression and influence cancer development and progression.Cuproptosis,a newly discovered form of cell death,plays an important role in cancer.Nonetheless,additional research investigating the association between cuproptosisrelated lncRNAs and prostate cancer(PCa)prognosis is required.Methods:Sequencing data and copy number variant data were obtained from 492 patients with PCa from The Cancer Genome Atlas(TCGA)Program.Prognostic models of PCa based on cuproptosis-related lncRNAs were constructed using a multi-level attention graph neural network(MLA-GNN)deep learning algorithm.Immune escape scoring was performed using Tumor Immune Dysfunction and Exclusion.Cellular experiments were conducted to explore the correlation between key lncRNAs and cuproptosis.Results:Data from 492 patients with PCa were randomized into two groups at a 1:1 ratio.Prognostic modeling was successfully established using MLA-GNN.Survival analysis suggested that patients could be divided into high-and low-risk groups according to model scores and that there was a significant difference in disease-free survival(DFS)(P<0.01).The area under the receiver operating characteristic(ROC)curve(AUC)indicated a strong predictive performance for the model,with AUCs of 0.913,0.847,and 0.863 for the training group and 0.815,0.907,and 0.866 for the test group at 12,36,and 60 months,respectively.The immune escape score and immune microenvironment analysis suggested that the high-risk group corresponded to a stronger immune escape and a poorer immune microenvironment(P<0.05).Cellular experiments revealed that the expression of all six key lncRNAs was upregulated in the presence of copper ion carriers(P<0.05).Conclusions:This study identified cuproptosis-related lncRNAs that were strongly associated with PCa prognosis.Key lncRNAs could affect copper metabolism and may serve as new therapeutic targets.
基金This work was supported by the National Natural Science Foundation of China(Grant no.51973009)Xuzhou Natural Science Foundation in China(KC18201 and KC18108).
文摘Biomimetic scaffolds made by synthetic materials are usually used to replace the natural tissues aimed at speeding up the skin regeneration.In this study,a flexible and cytocompatible poly(glycerol sebacate)@poly-l-lactic acid(PGS@PLLA)fibrous scaffold with a core-shell structure was fabricated by coaxial electrospinning,where the shell PLLA was used to be a skeleton with pores on the fibrous surface.The fibrous morphology with pores on the surface of the prepared fibers was observed by SEM.The core-shell microstructure of PGS@PLLA fibers was confirmed by TEM and Laser Scanning Confocal Microscopy(LSCM).In addition,the prepared fibers exhibited a strong ability to repair tissues of the skin wound,where the stability of cell security and proliferation,and the lower inflammatory response were all superior to those of pure PLLA scaffold.It’s worth noting that the percentage of skin tissue was regenerated by 95%within 14 days,which suggests the potential application for electrospun-based synthetic fibrous scaffolds on wound healing.
基金partially supported by the National Science Foundation of China and Hong Kong RGC Joint Research Scheme(NSFC/RGC 11961160718)the fund of the Guangdong Provincial Key Laboratory of Computational Science and Material Design(No.2019B030301001)+1 种基金supported by the National Science Foundation of China(NSFC-11871264)the Shenzhen Natural Science Fund(RCJC20210609103819018).
文摘In this work,we study gradient-based regularization methods for neural networks.We mainly focus on two regularization methods:the total variation and the Tikhonov regularization.Adding the regularization term to the training loss is equivalent to using neural networks to solve some variational problems,mostly in high dimensions in practical applications.We introduce a general framework to analyze the error between neural network solutions and true solutions to variational problems.The error consists of three parts:the approximation errors of neural networks,the quadrature errors of numerical integration,and the optimization error.We also apply the proposed framework to two-layer networks to derive a priori error estimate when the true solution belongs to the so-called Barron space.Moreover,we conduct some numerical experiments to show that neural networks can solve corresponding variational problems sufficiently well.The networks with gradient-based regularization are much more robust in image applications.
基金supported by RG(R)-RC/17-18/02-MATHHKBU 12300819+2 种基金NSF/RGC grant N-HKBU214-19RC-FNRA-IG/19-20/SCI/01supported by Programs for Science and Technology Development of Henan Province(192102310181)。
文摘In this work,we present a new method for convex shape representation,which is regardless of the dimension of the concerned objects,using level-set approaches.To the best of our knowledge,the proposed prior is the first one which can work for high dimensional objects.Convexity prior is very useful for object completion in computer vision.It is a very challenging task to represent high dimensional convex objects.In this paper,we first prove that the convexity of the considered object is equivalent to the convexity of the associated signed distance function.Then,the second order condition of convex functions is used to characterize the shape convexity equivalently.We apply this new method to two applications:object segmentation with convexity prior and convex hull problem(especially with outliers).For both applications,the involved problems can be written as a general optimization problem with three constraints.An algorithm based on the alternating direction method of multipliers is presented for the optimization problem.Numerical experiments are conducted to verify the effectiveness of the proposed representation method and algorithm.
文摘Correction to:Radiation Detection Technology and Methods(2024)8:1-1105.https://doi.org/10.1007/s41605-024-00463-y.In this article all authors name was missing in the springer link.It has been corrected.The original article has been corrected.
基金financial support from the National Natural Science Foundation of China(NSFC)(12125507,12047503,12035008,2211530479,12475094,12135006,12075097,12375086,2022YFA1601903,12061141007,12375091,12342502,12235018,12335003,12105100,12475106,11961141015,12188102,12175245,12205171,12321005,tsqn202312052,2024HWYQ-005,12405121,12447167,12061141006,12405102,12125503,12305115,12075213,12335005,12235008)the Chinese Academy of Sciences(YSBR-101,XDB34030000)+11 种基金the National Key R&D Program of China(2022YFE0116900,2023YFA1606703,2022YFA1601901)the National Key Research and Development Program of China(2023YFA1606300)the Excellent Postdoctoral Program of Jiangsu Province(2023ZB891)the Shenzhen Science and Technology Program(202206193000001,20220816094256002)the Natural Science Foundation for Distinguished Young Scholars of Henan Province(242300421046)the Beijing Municipal Natural Science Foundation(JQ22002)the Area of Excellence(AoE/P-404/18-3)the General Research Fund(16304321)(both grants are issued by the Research Grants Council of Hong Kong S.A.R)the MOST National Key R&D Program(2023YFA1606303)the Shanghai Key Laboratory for Particle Physics and CosmologyKey Laboratory for Particle Astrophysics and Cosmology(Ministry of Education)Shanghai Jiao Tong University。
文摘We discuss the landscape of flavor physics at the Circular Electron-Positron Collider(CEPC),based on the nominal luminosity outlined in its Technical Design Report.The CEPC is designed to operate in multiple modes to address a variety of tasks.At the Z pole,the expected production of 4 Tera Z bosons will provide unique and highly precise measurements of Z boson couplings,while the substantial number of boosted heavy-flavored quarks and leptons produced in clean Z decays will facilitate investigations into their flavor physics with unprecedented precision.We investigate the prospects of measuring various physics benchmarks and discuss their implications for particle theories and phenomenological models.Our studies indicate that,with its highlighted advantages and anticipated excellent detector performance,the CEPC can explore beauty andτphysics in ways that are superior to or complementary with the Belle II and Large-Hadron-Collider-beauty experiments,potentially enabling the detection of new physics at energy scales of 10 TeV and above.This potential also extends to the observation of yet-to-be-discovered rare and exotic processes,as well as testing fundamental principles such as lepton flavor universality,lepton and baryon number conservation,etc.,making the CEPC a vibrant platform for flavor physics research.The WW threshold scan,Higgs-factory operation and top-pair productions of the CEPC further enhance its merits in this regard,especially for measuring the Cabibbo-Kobayashi-Maskawa matrix elements,and Flavor-Changing-NeutralCurrent physics of Higgs boson and top quarks.We outline the requirements for detector performance and considerations for future development to achieve the anticipated scientific goals.The role of machine learning for innovative detector design and advanced reconstruction algorithms is also stressed.The CEPC flavor physics program not only develops new capabilities for exploring flavor physics beyond existing projects but also enriches the physics opportunities of this machine.It should be remarked that,given the richness of the CEPC flavor physics,this manuscript is not meant to be a comprehensive survey,but rather an investigation of representative cases.Uncovering the full potential of flavor physics at the CEPC will require further dedicated explorations in the future.
基金This work was funded by the National Natural Science Foundation of China(Grant Nos.11702037 and 11832007)State Key Laboratory of Mechanics and Control of Mechanical Structures,Nanjing University of Aeronautics and astronautics(Grant No.MCMS-E-0522G01)+1 种基金the Open Foundation of Guangdong Provincial Key Laboratory of Materials and Technologies for Energy Conversion(Grant No.MATEC2022KF001)as well as the Cultivation Project for the Natural Science Foundation and Highlevel Talent at Chengdu University(Grant No.Z1350).
文摘High-performance Pb(Zr_(1−x)Ti_(x))O_(3)(PZT)piezoceramics are urgently desired by the market in view of their expanded operating temperature range,reduced property temperature dependence,and enhanced sensitivity and acoustic power.In this work,we reported a kind of low-cost and high-performance 0.06BiYbO_(3)–0.94Pb(Zr_(0.48)Ti_(0.52))O_(3) ternary piezoceramics;the modifying effects of La_(2)O_(3) on this perovskite system were investigated in terms of the structures,electrical properties,and thermal depolarization behaviors of ceramics.The field-dependent dielectric and conduction properties indicated that there are close correlations among oxygen vacancies(VO),conducting electrons,and intrinsic conduction process.The degradation in ferroelectric properties observed in those samples doped with more than 0.15 wt%of La_(2)O_(3) indicated that the occupying mechanisms of La^(3+)changed from the donor substitution for Pb^(2+)to the isovalent substitution for Bi^(3+).The thermally depoling micromechanisms of ceramics were revealed from the thermodynamic processes of defect dipoles and intrinsic dipoles within ferroelectric domains.The sample doped with 0.15 wt%of La_(2)O_(3) shows excellent electrical properties with TC=387℃,d33=332 pC/N,TKε=5.81×10^(−3)℃−1,Pr=20.66μC/cm^(2),Td=356℃.The significantly enhanced electrical properties and thermal depolarization temperature benefited from the donor substitution of La3+,decreasing the oxygen vacancy concentration in the lattice and possibly optimizing the ferroelectric domain structure of ceramics.
基金support from diverse funding sources,including the National Key Program for S&T Research and Development of the Ministry of Science and Technology(MOST),Yifang Wang's Science Studio of the Ten Thousand Talents Project,the CAS Key Foreign Cooperation Grant,the National Natural Science Foundation of China(NSFC)Beijing Municipal Science&Technology Commission,the CAS Focused Science Grant,the IHEP Innovation Grant,the CAS Lead Special Training Programthe CAS Center for Excellence in Particle Physics,the CAS International Partnership Program,and the CAS/SAFEA International Partnership Program for Creative Research Teams.
文摘The Circular Electron Positron Collider(CEPC)is a large scientific project initiated and hosted by China,fostered through extensive collaboration with international partners.The complex comprises four accelerators:a 30 GeV Linac,a 1.1 GeV Damping Ring,a Booster capable of achieving energies up to 180 GeV,and a Collider operating at varying energy modes(Z,W,H,and tt).The Linac and Damping Ring are situated on the surface,while the subterranean Booster and Collider are housed in a 100 km circumference underground tunnel,strategically accommodating future expansion with provisions for a potential Super Proton Proton Collider(SPPC).The CEPC primarily serves as a Higgs factory.In its baseline design with synchrotron radiation(SR)power of 30 MW per beam,it can achieve a luminosity of 5×10^(34)cm^(-2)s^(-1)per interaction point(IP),resulting in an integrated luminosity of 13 ab^(-1)for two IPs over a decade,producing 2.6 million Higgs bosons.Increasing the SR power to 50 MW per beam expands the CEPC's capability to generate 4.3 million Higgs bosons,facilitating precise measurements of Higgs coupling at sub-percent levels,exceeding the precision expected from the HL-LHC by an order of magnitude.This Technical Design Report(TDR)follows the Preliminary Conceptual Design Report(Pre-CDR,2015)and the Conceptual Design Report(CDR,2018),comprehensively detailing the machine's layout,performance metrics,physical design and analysis,technical systems design,R&D and prototyping efforts,and associated civil engineering aspects.Additionally,it includes a cost estimate and a preliminary construction timeline,establishing a framework for forthcoming engineering design phase and site selection procedures.Construction is anticipated to begin around 2027-2028,pending government approval,with an estimated duration of 8 years.The commencement of experiments and data collection could potentially be initiated in the mid-2030s.
基金funded by the National Natural Science Foundation of China(No.12372179)supported by the State Key Laboratory of Mechanics and Control of Mechanical Structures,Nanjing University of Aeronautics and Astronautics(No.MCMS-E-0522G01).
文摘As a typical Aurivillius-type compound, CaBi_(4)Ti_(4)O_(15) (CBT) is considered a strong competitor among hightemperature piezoelectric materials, but it is difficult to achieve both high piezoelectric activity and a high Curie temperaturefor CBT. In this work, the method of double-ion co-substituting at different crystalline sites was used to modify the electricalproperties of CBT. The Gd/Mn co-doped CBT ceramics with the chemical formula of Ca_(1−x)Gd_(x)Bi_(4)Ti_(4)O_(15)+0.2 wt% MnO_(2)(CBT–100xGM, x = 0–0.11) were prepared via the conventional sintering process. The phase and valence band structures,chemical compositions and microstructures, dielectric and ferroelectric properties, electrical conduction behaviors, andelectroelastic and piezoelectric properties of the ceramics were characterized. The doping concentration effects of Gd^(3+)were analyzed according to the composition-dependent structures and properties of CBT–100xGM. The donor substitutionof Gd^(3+) for Ca^(2+) at the A-site reduced the tolerance factor of the perovskite-like structure and decreased the concentration ofintrinsic oxygen vacancies. While Mn^(3+) tended to substitute for Ti4+ at the B-site, the extrinsic oxygen vacancies are limitednear the defect center of Ti(Mn) because of the formation of ( ‒MnTi')• as defect dipoles. The thermal depoling behavior ofthe CBT–100xGM ceramics between 300 and 700 ℃ was explained by the thermodynamic characteristics of the defectdipoles. The optimized composition with x = 0.08 (CBT–8GM) had a high TC ≈ 809 ℃ and a high piezoelectric coefficient(d33) ≈ 23 pC/N, as well as a piezoelectric voltage constant (g33) value of up to 21.5×10^(−3)(V·m)/N. Moreover, it can maintaina residual d33 ≈ 80% after being annealed at 700 ℃. This good anti-thermal depoling ability endows this material with greatapplication potential in high-temperature piezoelectric devices with operating temperatures exceeding 500 ℃. Thesynergistic enhancement in the piezoelectric activity and Curie temperature of CBT can be attributed mainly to the donorsubstituting effect of Gd^(3+) at the A-site, as well as the decreased elastic compliance contributed by MnO_(2) as the B-sitedopant.
基金funded by the Natural Science Foundation of Sichuan Province(Grant No.2024NSFSC0219).
文摘Recently,high-performance lead zirconate titanate(Pb(Zr_(1-x)Ti_(x))O_(3),PZT)ferroelectric ceramics have attracted intensive attention due to their wider operating temperature range,better temperature stability,as well as larger piezoelectric properties and higher energy conversion efficiency.In this study,the perovskite-type ferroelectric ceramics with a chemical formula of Pb_(0.99-x)Gd_(0.01)Sr_(x)Zr_(0.53)Ti_(0.47)O_(3)(x=0 and 0.02,abbr.PGZT and PGSZT,respectively)were prepared by the traditional solid-state reaction route.The influences of Sr-doping on the phase structure,dielectric properties,ferroelectric properties and piezoelectric properties of the PGZT ceramics were comprehensively investigated.The field-dependent P–E hysteresis loops of PGSZT were measured in the frequency range of 0.05–10 Hz and temperature range of 20–100℃.The results show that Sr-doping not only enhances the dielectric permittivity and piezoelectric coefficient of PGZT,but also decreases its dielectric loss tangent,with the d_(33) value of 473 pC/N,ε_(r) value of 1586 and tanδvalue of 0.016 found in PGSZT.Also,PGSZT shows a high Curie temperature(T_(C))of 350℃.The underlying mechanisms of the property enhancement were identified as that the introduced Sr^(2+) replaces the volatile Pb^(2+) located at the A-site of the perovskite structure,thereby reducing the concentration of lead vacancies and promoting the grain growth of the ceramics,consequently enhancing the dielectric and piezoelectric properties of PGZT.On the other hand,the frequency change in the low-frequency range(<1 Hz)played a significant impact on the remanent polarization(P_(r))and internal biased electric field(E_(i))of PGSZT,but the frequency dependence of coercive field(E_(c))tends to diminish in the high-frequency range(≥1 Hz).
基金the Natural Science Foundation of China(NSFC)(11905162,12035008,12075097,12075123,12090060,12090064,12105248,12135006,12175039,12205227,12205312,12205387,12205171,12235008,12321005,12235001,12305094,12305115,12335005,12375091,12375094,12375096,11975129,12375194,12447167,12475094,12475101,12475106,12475111,12425506,12375101,12405119,12405101,12505121,12135007,12175218,12075213,12335005,12175243,12533001,12125503,12305103,12505120,12575099,12505122,12342502,12575106,12147214,W2432006,W2441004)the National Key R&D Program of China(2024YFA1610603)+22 种基金the China Postdoctoral Science Foundation(2023M732255,2025M773403,GZC20231613)the Natural Science Foundation of Jiangsu Province(BK20210201)the Natural Science Foundation of Henan(Distinguished Young Scholars of Henan Province)(242300421046)the Natural Science Foundation of Sichuan Province(2025ZNSFSC0880)the Guangdong Major Project of Basic and Applied Basic Research(2020B0301030008)the Department of Science and Technology of Shandong province(tsqn202312052,2024HWYQ-005)the Startup Research Fund of Henan Academy of Sciences(20251820001)the Excellent Young Talents Program of Wuhan University of Technology(40122102)the research program of the Wuhan University of Technology(3120625397,2020IB024)the Fundamental Research Funds for the Central Universities(JZ2023HGTB0222,WUT:2022IVA052)the Excellent Scholar Project of Southeast University(Class A)the Big Data Computing Center of Southeast University,National Science and Technology Council,the Ministry of Education(Higher Education Sprout Project NTU-114L104022-1)the Center for Theoretical Sciences of Taiwan,and Vietnam National Foundation for Science and Technology Development(NAFOSTED)(103.01-2023.50)the Research Office of the University of the Witwatersrand and South African Department of Science and Innovation through the SA-CERN programthe self-determined research funds of Central China Normal University from the colleges'basic research and operation of MOE(CCNU24AI003)SJTU Double First Class start-up fund(WF220442604)the Innovation Capability Support Program of Shaanxi(2021KJXX-47)the Slovenian Research Agency under the research core funding No.P1-0035,the research grants J1-3013,N1-0253,CONICET,ANPCyT under project(PICT-2021-00374)Higher Education Sprout Project(NTU-114L104022-1)KIAS Individual Grants(PG086002)at the Korea Institute for Advanced Study,FAPESP(2021/09547-9)the Slovenian Research Agency under the research core funding(P1-0035)research grants J1-3013,N1-0253the bilateral project Proteus PR-12696/Projet 50194VC。
文摘I.EXECUTIVE SUMMARY next-generation,high-intensity electron-positron collider"Higgs factory",such as the Circular Electron-Positron Collider(CEPC),is among the highest priorities for the global high-energy collider physics community.The CEPC can provide unprecedented opportunities for making fundamental discoveries and providing decisive insights in the quest for a"New Standard Model(SM)"of nature's fundamental interactions.The CEPC could:·Identify the origin of matter,especially the mechanism related to the first-order phase transition in the early Universe,which could produce a detectable gravitational wave signal.