Since meteorological conditions are the main factor driving the transport and dispersion of air pollutants,an accurate simulation of the meteorological field will directly affect the accuracy of the atmospheric chemic...Since meteorological conditions are the main factor driving the transport and dispersion of air pollutants,an accurate simulation of the meteorological field will directly affect the accuracy of the atmospheric chemical transport model in simulating PM_(2.5).Based on the NASM joint chemical data assimilation system,the authors quantified the impacts of different meteorological fields on the pollutant simulations as well as revealed the role of meteorological conditions in the accumulation,maintenance,and dissipation of heavy haze pollution.During the two heavy pollution processes from 10 to 24 November 2018,the meteorological fields were obtained using NCEP FNL and ERA5 reanalysis data,each used to drive the WRF model,to analyze the differences in the simulated PM_(2.5) concentration.The results show that the meteorological field has a strong influence on the concentration levels and spatial distribution of the pollution simulations.The ERA5 group had relatively small simulation errors,and more accurate PM_(2.5) simulation results could be obtained.The RMSE was 11.86𝜇g m^(-3)lower than that of the FNL group before assimilation,and 5.77𝜇g m^(-3)lower after joint assimilation.The authors used the PM_(2.5) simulation results obtained by ERA5 data to discuss the role of the wind field and circulation situation on the pollution process,to analyze the correlation between wind speed,temperature,relative humidity,and boundary layer height and pollutant concentrations,and to further clarify the key formation mechanism of this pollution process.展开更多
基金supported by the Second Tibetan Plateau Scientific Expedition and Research Program of Ministry of Science and Technology of the People's Republic of China[grant number 2022QZKK0101]the Science and Technology Department of the Tibet Program[grant number XZ202301ZY0035G]。
文摘Since meteorological conditions are the main factor driving the transport and dispersion of air pollutants,an accurate simulation of the meteorological field will directly affect the accuracy of the atmospheric chemical transport model in simulating PM_(2.5).Based on the NASM joint chemical data assimilation system,the authors quantified the impacts of different meteorological fields on the pollutant simulations as well as revealed the role of meteorological conditions in the accumulation,maintenance,and dissipation of heavy haze pollution.During the two heavy pollution processes from 10 to 24 November 2018,the meteorological fields were obtained using NCEP FNL and ERA5 reanalysis data,each used to drive the WRF model,to analyze the differences in the simulated PM_(2.5) concentration.The results show that the meteorological field has a strong influence on the concentration levels and spatial distribution of the pollution simulations.The ERA5 group had relatively small simulation errors,and more accurate PM_(2.5) simulation results could be obtained.The RMSE was 11.86𝜇g m^(-3)lower than that of the FNL group before assimilation,and 5.77𝜇g m^(-3)lower after joint assimilation.The authors used the PM_(2.5) simulation results obtained by ERA5 data to discuss the role of the wind field and circulation situation on the pollution process,to analyze the correlation between wind speed,temperature,relative humidity,and boundary layer height and pollutant concentrations,and to further clarify the key formation mechanism of this pollution process.
