To address the issues of the greenhouse effect and energy dilemma,it is a global hot topic on converting CO_(2)to valuable chemicals and useable fuels.In this review,firstly,we shortly summarize different CO_(2)conver...To address the issues of the greenhouse effect and energy dilemma,it is a global hot topic on converting CO_(2)to valuable chemicals and useable fuels.In this review,firstly,we shortly summarize different CO_(2)conversion methods including thermal catalysis,biocatalysis,electrocatalysis,photocatalysis,and plasma catalysis.Then,a comprehensive overview of the currently explored plasma driven CO_(2)conversion is presented,such as microwave discharge plasma,gliding arc discharge plasma,radiofrequency inductively coupled plasma,and dielectric barrier discharge plasma,with an emphasis on their experimental setups,achievements and limitations.Furthermore,the activation of CO_(2)conversion via the synergistic effect between the plasma and photocatalyst is discussed in detail.Finally,the associated challenges and future development trends for plasma catalytic CO_(2)conversion are briefly concluded.展开更多
基金supported by the National Natural Science Foundation of China(Grant No.22072010)Natural Science Foundation of Chongqing Municipality(Grant No.CSTB2024NSCQLZX0101)+2 种基金Natural Science Foundation of Chongqing(Grant No.cstc2021ycjh-bgzxm0181)Science and Technology Research Program of Chongqing Municipal Education Commission(Grant No.KJQN202300629)Institute for Advanced Sciences(Grant No.E011A2022325).
文摘To address the issues of the greenhouse effect and energy dilemma,it is a global hot topic on converting CO_(2)to valuable chemicals and useable fuels.In this review,firstly,we shortly summarize different CO_(2)conversion methods including thermal catalysis,biocatalysis,electrocatalysis,photocatalysis,and plasma catalysis.Then,a comprehensive overview of the currently explored plasma driven CO_(2)conversion is presented,such as microwave discharge plasma,gliding arc discharge plasma,radiofrequency inductively coupled plasma,and dielectric barrier discharge plasma,with an emphasis on their experimental setups,achievements and limitations.Furthermore,the activation of CO_(2)conversion via the synergistic effect between the plasma and photocatalyst is discussed in detail.Finally,the associated challenges and future development trends for plasma catalytic CO_(2)conversion are briefly concluded.