A 2-dimensional atmospheric transport model is deployed in a simplified CO 2 inverse study. Calculated carbon flux distribution for the interval from 1981 to 1997 confirms the existence of a terrestrial carbon sink i...A 2-dimensional atmospheric transport model is deployed in a simplified CO 2 inverse study. Calculated carbon flux distribution for the interval from 1981 to 1997 confirms the existence of a terrestrial carbon sink in mid-high latitude area of North Hemisphere. Strong interannual variability exists in carbon flux patterns, implying a possible link with ENSO and other natural episodes such as Pinatubo volcano eruption in 1991. Mechanism of this possible link was investigated with statistic method. Correlation analysis indicated that in North Hemisphere, climatic factors such as temperature and precipitation, to some extend, could influence the carbon cycle process of land and ocean, thus cause considerable change in carbon flux distribution. In addition, correlation study also demonstrated the possible important role of Asian terrestrial ecosystems in carbon cycle.展开更多
Uniform shape platinum nanocrystals with narrow size distribution and controlled average dimension are successfully embedded in a polymeric matrix and sup-ported on zeolite Beta. The surface structure and reactivity o...Uniform shape platinum nanocrystals with narrow size distribution and controlled average dimension are successfully embedded in a polymeric matrix and sup-ported on zeolite Beta. The surface structure and reactivity of nanometalclusters are investigated by TEM, EXAFS, CO adsorption and methane activation. The results indicate that nanometalparticles in PVP-Pt/Beta materials have high sur-face activity and reactivity to activate methane even at tem-perature of 373K.展开更多
文摘A 2-dimensional atmospheric transport model is deployed in a simplified CO 2 inverse study. Calculated carbon flux distribution for the interval from 1981 to 1997 confirms the existence of a terrestrial carbon sink in mid-high latitude area of North Hemisphere. Strong interannual variability exists in carbon flux patterns, implying a possible link with ENSO and other natural episodes such as Pinatubo volcano eruption in 1991. Mechanism of this possible link was investigated with statistic method. Correlation analysis indicated that in North Hemisphere, climatic factors such as temperature and precipitation, to some extend, could influence the carbon cycle process of land and ocean, thus cause considerable change in carbon flux distribution. In addition, correlation study also demonstrated the possible important role of Asian terrestrial ecosystems in carbon cycle.
文摘Uniform shape platinum nanocrystals with narrow size distribution and controlled average dimension are successfully embedded in a polymeric matrix and sup-ported on zeolite Beta. The surface structure and reactivity of nanometalclusters are investigated by TEM, EXAFS, CO adsorption and methane activation. The results indicate that nanometalparticles in PVP-Pt/Beta materials have high sur-face activity and reactivity to activate methane even at tem-perature of 373K.
