This research explores the prospect of fabricating a face-centered cubic(fcc) Ni-base alloy cladding(Inconel 690) on an fcc Fe-base alloy(316 L stainless-steel) having improved mechanical properties and reduced sensit...This research explores the prospect of fabricating a face-centered cubic(fcc) Ni-base alloy cladding(Inconel 690) on an fcc Fe-base alloy(316 L stainless-steel) having improved mechanical properties and reduced sensitivity to corrosion through grain boundary and microstructure engineering concepts enabled by additive manufacturing(AM) utilizing electron-beam powder bed fusion(EPBF). The unique solidification and associated constitutional supercooling phenomena characteristic of EPBF promotes[100] textured and extended columnar grains having lower energy grain boundaries as opposed to random, high-angle grain boundaries, but no coherent {111} twin boundaries characteristic of conventional thermo-mechanically processed fcc metals and alloys, including Inconel 690 and 316 L stainless-steel.In addition to [100] textured grains, columnar grains were produced by EPBF fabrication of Inconel 690 claddings on 316 L stainless-steel substrates. Also, irregular 2–3 μm diameter, low energy subgrains were formed along with dislocation densities varying from 108 to 109 cm^2, and a homogeneous distribution of Cr_(23)C_6 precipitates. Precipitates were formed within the grains(with ~3 μm interparticle spacing),but not in the subgrain or columnar grain boundaries. These inclusive, hierarchical microstructures produced a tensile yield strength of 0.527 GPa, elongation of 21%, and Vickers microindentation hardness of 2.33 GPa for the Inconel 690 cladding in contrast to a tensile yield strength of 0.327 GPa, elongation of 53%, and Vickers microindentation hardness of 1.78 GPa, respectively for the wrought 316 L stainlesssteel substrate. Aging of both the Inconel 690 cladding and the 316 L stainless-steel substrate at 685?C for50 h precipitated Cr_(23)C_6 carbides in the Inconel 690 columnar grain boundaries, but not in the low-angle(and low energy) subgrain boundaries. In contrast, Cr_(23)C_6 carbides precipitated in the 316 L stainless-steel grain boundaries, but not in the low energy coherent {111} twin boundaries. Consequently, the Inconel690 subgrain boundaries essentially serve as surrogates for coherent twin boundaries with regard to avoiding carbide precipitation and corrosion sensitization.展开更多
Existing droplet evaporation/combustion mod- els in computational fluid dynamics (CFD) simulation of spray combustion are based on simplified 1-D models. Both these models and recently developed 3-D models of single...Existing droplet evaporation/combustion mod- els in computational fluid dynamics (CFD) simulation of spray combustion are based on simplified 1-D models. Both these models and recently developed 3-D models of single- droplet combustion do not give the conditions for the different existing droplet combustion modes. In this paper, droplet evaporation and combustion are studied both analytically and numerically. In the analytical solution, a 2-D axisymmetric flow surrounding an evaporating and combusting droplet was considered. The governing equations were solved using an integral method, similar to the Karman-Pohlhausen method for solving boundary-layer flows with pressure gradient. The results give a local evaporation rate and flame radius in agree- ment with experimental results. In numerical simulation, 3-D combusting gas flows surrounding an ethanol droplet were studied. The prediction results show three modes of droplet combustion under different relative velocities, explaining the change in the evaporation constant with an increase in relative velocity observed in experiments. This implies that different droplet combustion models should be developed in simu- lating spray combustion. The predicted local evaporation rate and flame radius by numerical simulation are in agree- ment with the analytical solution in the range of azimuthal angles 0° 〈 θ 〈 90°. The numerical results indicate that the drag force of an evaporating and combusting droplet is much smaller than that of a cold solid particle, and thus the currently used drag models should be modified.展开更多
<001>textured Pb(Ni_(1/3)Nb_(2/3))O_(3)-PbZrO_(3)-PbTiO_(3)(PNN-PZT)ceramics were prepared by templated grain growth(TGG)technique using 0.36PNN-x PZ-(0.64-x)PT(x=0.23,0.25 and 0.27)powder matrix.Optimum templat...<001>textured Pb(Ni_(1/3)Nb_(2/3))O_(3)-PbZrO_(3)-PbTiO_(3)(PNN-PZT)ceramics were prepared by templated grain growth(TGG)technique using 0.36PNN-x PZ-(0.64-x)PT(x=0.23,0.25 and 0.27)powder matrix.Optimum template content was derived to achieve the best electromechanical properties of textured ceramics.The piezoelectric coefficient d33=1165 pC/N,Curie temperature T_(C)=197℃,longitudinal mode electrome-chanical coupling factor k33=0.86 and a very large effective piezoelectric strain coefficient d_(33)^(*)=2041 pm/V were simultaneously achieved at the morphotropic phase boundary(MPB)composition(x=0.25)with 3 vol.%BaTiO_(3)(BT)templates.Domain structures of textured ceramics were analyzed in detail to reveal the origin of these high piezoelectric and electromechanical properties.展开更多
An electrolyte model for the solid oxide fuel cell (SOFC) with proton conducting perovskite electrolyte is developed in this study, in which four types of charge carriers including proton, oxygen vacancy (oxide ion), ...An electrolyte model for the solid oxide fuel cell (SOFC) with proton conducting perovskite electrolyte is developed in this study, in which four types of charge carriers including proton, oxygen vacancy (oxide ion), free electron and electron hole are taken into consideration. The electrochemical process within the SOFC with hydrogen as the fuel is theoretically analyzed. With the present model, the effects of some parameters, such as the thickness of electrolyte, operating temperature and gas composition, on the ionic transport (or gas permeation) through the electrolyte and the electrical performance, i.e., the electromotive force (EMF) and internal resistance of the cell, are investigated in detail. The theoretical results are tested partly by comparing with the experimental data obtained from SrCe0.95M0.05O3-α, (M=Yb, Y) cells.展开更多
Proton-hole mixed conductor, SrCeo.95Yb0.05O3-α(SCYb), has the potential to be used as a membrane for dehydrogenation reactions such as methane coupling due to its high C2-selectivity and its simplicity for fabricati...Proton-hole mixed conductor, SrCeo.95Yb0.05O3-α(SCYb), has the potential to be used as a membrane for dehydrogenation reactions such as methane coupling due to its high C2-selectivity and its simplicity for fabricating reactor systems. In addition, the mixed conducting membrane in the hollow fibre geometry is capable of providing high surface area per unit volume. In this study, mechanism of methane coupling reaction on the SCYb membrane was proposed and the kinetic parameters were obtained by regression of experimental data. A mathematical model describing the methane coupling in the SCYb hollow fibre membrane reactor was also developed. With this mathematical model, various operating conditions such as the operation mode, operation pressure and feed concentrations affecting performance of the reactor were investigated. The simulation results show that the cocurrent flow in the reactor exhibits higher conversion of methane and higher yield of ethylene compared to the countercurrent flow. In order to achieve the highest C2 yield, especially of ethylene, pure methane should be used as feed and the operating pressure be 300 kPa. Air can be used as the source of oxygen for the reaction and its optimum feed velocity is twice of the methane feed velocity. The air pressure in the lumen side should be kept the same as or slightly lower than the pressure of shell side.展开更多
Based on the main characteristics of the tectonic-magmatic evolution of region and Tanlu fault zone,we have discussed ore-bearing magmatic rocks petrochemistry,strontium and lead isotope,and the source of ore-forming ...Based on the main characteristics of the tectonic-magmatic evolution of region and Tanlu fault zone,we have discussed ore-bearing magmatic rocks petrochemistry,strontium and lead isotope,and the source of ore-forming materials in Yinan skarn deposit in this paper.展开更多
In this paper,we report the detection of the very-high-energy(VHE,100 GeV<E<100 TeV)and ultra-high-energy(UHE,E>100 TeV)y-ray emissions from the direction of the young star-forming region W43,observed by the ...In this paper,we report the detection of the very-high-energy(VHE,100 GeV<E<100 TeV)and ultra-high-energy(UHE,E>100 TeV)y-ray emissions from the direction of the young star-forming region W43,observed by the Large High Altitude Air Shower Observation(LHAASO).The extendedγ-ray source was detected with a significance of~16σby KM2A and~17σby WCDA,respectively.The angular extension of this y-ray source is about 0.5 degrees,corresponding to a physical size of about 50pc.We discuss the origin of theγ-ray emission and possible cosmic ray acceleration in the W43 region using multi-wavelength data.Our findings suggest that W43 is likely another young star cluster capable of accelerating cosmic rays(CRs)to at least several hundred TeV.展开更多
We report the detection of an extended very-high-energy(VHE)γ-ray source coincident with the location of middle-aged(62.4 kyr)pulsar PSR J0248+6021,by using the LHAASO-WCDA data of live 796 d and LHAASO-KM2A data of ...We report the detection of an extended very-high-energy(VHE)γ-ray source coincident with the location of middle-aged(62.4 kyr)pulsar PSR J0248+6021,by using the LHAASO-WCDA data of live 796 d and LHAASO-KM2A data of live 1216d.A significant excess of y-ray induced showers is observed both by WCDA in energy bands of 1-25 TeV and KM2A in energy bands of>25 TeV with 7.3σand 13.5σ,respectively.The best-fit position derived through WCDA data is R.A.=42.06°±0.12°and Dec.=60.24°±0.13°with an extension of 0.69°±0.15°and that of the KM2A data is R.A.=42.29°±0.13°and Dec.=60.38°±0.07°with an extension of 0.37°±0.07°.No clear extended multiwavelength counterpart of this LHAASO source has been found from the radio band to the GeV band.The most plausible explanation of the VHEγ-ray emission is the inverse Compton process of highly relativistic electrons and positrons injected by the pulsar.These electrons/positrons are hypothesized to be either confined within the pulsar wind nebula or to have already escaped into the interstellar medium,forming a pulsar halo.展开更多
We report a dedicated study of the newly discovered extended UHEγ-ray source 1LHAASO J0056+6346u.Analyzing 979 d of LHAASO-WCDA data and 1389 d of LHAASO-KM2A data,we observed a significant excess ofγ-ray events wit...We report a dedicated study of the newly discovered extended UHEγ-ray source 1LHAASO J0056+6346u.Analyzing 979 d of LHAASO-WCDA data and 1389 d of LHAASO-KM2A data,we observed a significant excess ofγ-ray events with both WCDA and KM2A.Assuming a point power-law source with a fixed spectral index,the significance maps reveal excesses of 12.65σ,22.18σ,and 10.24σin the energy ranges of 1-25,25-100,and>100 TeV,respectively.We use a 3D likelihood algorithm to derive the morphological and spectral parameters,and the source is detected with significances of 13.72σby WCDA and 25.27σby KM2A.The best-fit positions derived from WCDA and KM2A data are(R.A.=13.96°±0.09°,Decl.=63.92°±0.05°)and(R.A.=14.00°±0.05°,Decl.=63.79°±0.02°),respectively.The angular size(r_(39))of 1LHAASO J0056+6346u is 0.34°±0.04°at 1-25 TeV and 0.24°±0.02°at>25 TeV.The differential flux of this UHEγ-ray source can be described by an exponential cutoff power-law function:(2.67±0.25)×10^(-15)(E/20 TeV)^((-1.97±0.10))e^(-E/(55.1±7.2)TeV)TeV^(-1)cm^(-2)s^(-1).To explore potential sources ofγ-ray emission,we investigated the gas distribution around 1LHAASO J0056+6346u.1LHAASO J0056+6346u is likely to be a TeV PWN powered by an unknown pulsar,which would naturally explain both its spatial and spectral properties.Another explanation is that this UHEγ-ray source might be associated with gas content illuminated by a nearby CR accelerator,possibly the SNR candidate G124.0+1.4.展开更多
By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0...By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) events.The mass of χ_(c 0) is determined to be M (χ_(c 0))=(3415.63±0.07±0.07±0.07)MeV/c^(2),and its full width is F (χ_(c 0))=(12.52±0.12±0.13)MeV,where the first uncertainty is statistical,the second systematic,and the third for mass comes from χ_(c 2) mass uncertainty.These measurements improve the precision of χ_(c 0) mass by a factor of four and width by one order of magnitude over the previous individual measurements,and significantly boost our knowledge about the charmonium spectrum.Together with additional (345.4±2.6)×10^(6)(3686) data events taken in 2012,the decay branching fractions of χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) are measured as well,with precision improved by a factor of three compared to previous measurements.These χ_(c 0) decay branching fractions provide important inputs for the study of glueballs.展开更多
Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limi...Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.展开更多
Using an electron-positron collision data sample corresponding to(1.0087±0.0044)×10^(10)events collected using the BESIII detector at the BEPCII collider,we firstly search for the lepton number violation de...Using an electron-positron collision data sample corresponding to(1.0087±0.0044)×10^(10)events collected using the BESIII detector at the BEPCII collider,we firstly search for the lepton number violation decayφ→π^(+)π^(+)e^(-)e^(-)via J/ψ→φη.No obviously signals are found.The upper limit on the branching fraction ofφ→π^(+)π^(+)e^(-)e^(-)is set to be 1.3×10^(-5)at the 90%confidence level.展开更多
The ultra-high-energy(UHE)gamma-ray source 1LHAASO J0007+7303u is positionally associated with the composite SNR CTA1 that is located at high Galactic Latitude b≈10.5°.This provides a rare opportunity to spatial...The ultra-high-energy(UHE)gamma-ray source 1LHAASO J0007+7303u is positionally associated with the composite SNR CTA1 that is located at high Galactic Latitude b≈10.5°.This provides a rare opportunity to spatially resolve the component of the pulsar wind nebula(PWN)and supernova remnant(SNR)at UHE.This paper conducted a dedicated data analysis of 1LHAASO J0007+7303u using the data collected from December 2019 to July 2023.This source is well detected with significances of 21σand 17σat 8-100 TeV and>100 TeV,respectively.The corresponding extensions are determined to be 0.23°±0.03°and 0.17°±0.03°.The emission is proposed to originate from the relativistic electrons accelerated within the PWN of PSR J0007+7303.The energy spectrum is well described by a power-law with an exponential cutoff function dN/dE=(42.4±4.1)(E/20TeV)^(-2.31+0.11)exp(-E/(110±25Tev))TeV-1 cm^(-2)s^(-1)in the energy range from 8 to 300 TeV,implying a steady-state parent electron spectrum dN_(e)/dE_(e)∝(E_(e)/100TeV)^(-3.13±0.16)exp[(-E_(e)/(373±70TeV))^(2)]at energies above≈50 TeV.The cutoff energy of the electron spectrum is roughly equal to the expected current maximum energy of particles accelerated at the PWN terminal shock.Combining the X-ray and gamma-ray emission,the current space-averaged magnetic field can be limited to≈4.5μG.To satisfy the multi-wavelength spectrum and the y-ray extensions,the transport of relativistic particles within the PWN is likely dominated by the advection process under the free-expansion phase assumption.展开更多
Based on a sample of 2.7x 10^(9)ψ(3686)events collected by the BESIII detector operating at the BEP-CII collider,the decay 4(3686)→YX_(cJ),X_(cJ)→ηηη’is analyzed.The decay modes X_(c1)and X_(c2)→ηηη’are ob...Based on a sample of 2.7x 10^(9)ψ(3686)events collected by the BESIII detector operating at the BEP-CII collider,the decay 4(3686)→YX_(cJ),X_(cJ)→ηηη’is analyzed.The decay modes X_(c1)and X_(c2)→ηηη’are observed for the first time,and their corresponding branching fractions are determined to be B(X_(c1)→ηηη’)=(1.40±0.13(stat.)±0.09(sys.))×10^(-4)and B(X_(c2)→ηηη’)=(4.18±0.84(stat.)±0.48(sys.))×10^(-5).An upper limit on the branching fraction of x_(co)→ηηη’is set as 2.59×10^(-5)at a 90%confidence level(CL).A partial wave analys-is(PWA)of the decay X_(c1)→ηηη’is performed to search for the 1^(-+)exotic stateη1(1855).The PWA result indic-ates that the structure in theηη’mass spectrum is attributed to f_(0)(1500),while in the m mass spectrum,it is attrib-uted to the 0^(++)phase space.The upper limit of B(x_(cl)→η1(1855)η)·B(η1(1855)→ηη')<9.79×10^(-5)is set based on the PWA at 90%CL.展开更多
Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No s...Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).展开更多
We search for the leptonic decay D^(+)→e^(+)ν_(e)using an e+e-collision data sample with an integrated luminosity of 20.3 fb-1collected with the BESIII detector at a center-of-mass energy of 3.773 GeV.Significant si...We search for the leptonic decay D^(+)→e^(+)ν_(e)using an e+e-collision data sample with an integrated luminosity of 20.3 fb-1collected with the BESIII detector at a center-of-mass energy of 3.773 GeV.Significant signal is not observed,and an upper limit on the branching fraction of D^(+)→e^(+)ν_(e)is set as 9.7×10^(-7),at a confidence level of 90%.Our upper limit is an order of magnitude smaller than the previous limit for this decay mode.展开更多
Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed h...Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed hadronic decaysΛ_(c)^(+)→Σ^(0)K^(+)π^(0)andΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−)and with a single-tag method.No significant signals were observed for both decays.The upper limits on the branching fractions at the 90%confidence level were determined to be 5.0×10^(-4)for and forΛ_(c)^(+)→Σ^(0)K^(+)π^(0)and 6.5×10^(-4)forΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−).展开更多
基金Support for this project was provided by US Department of Energy grant DE-SC0011826
文摘This research explores the prospect of fabricating a face-centered cubic(fcc) Ni-base alloy cladding(Inconel 690) on an fcc Fe-base alloy(316 L stainless-steel) having improved mechanical properties and reduced sensitivity to corrosion through grain boundary and microstructure engineering concepts enabled by additive manufacturing(AM) utilizing electron-beam powder bed fusion(EPBF). The unique solidification and associated constitutional supercooling phenomena characteristic of EPBF promotes[100] textured and extended columnar grains having lower energy grain boundaries as opposed to random, high-angle grain boundaries, but no coherent {111} twin boundaries characteristic of conventional thermo-mechanically processed fcc metals and alloys, including Inconel 690 and 316 L stainless-steel.In addition to [100] textured grains, columnar grains were produced by EPBF fabrication of Inconel 690 claddings on 316 L stainless-steel substrates. Also, irregular 2–3 μm diameter, low energy subgrains were formed along with dislocation densities varying from 108 to 109 cm^2, and a homogeneous distribution of Cr_(23)C_6 precipitates. Precipitates were formed within the grains(with ~3 μm interparticle spacing),but not in the subgrain or columnar grain boundaries. These inclusive, hierarchical microstructures produced a tensile yield strength of 0.527 GPa, elongation of 21%, and Vickers microindentation hardness of 2.33 GPa for the Inconel 690 cladding in contrast to a tensile yield strength of 0.327 GPa, elongation of 53%, and Vickers microindentation hardness of 1.78 GPa, respectively for the wrought 316 L stainlesssteel substrate. Aging of both the Inconel 690 cladding and the 316 L stainless-steel substrate at 685?C for50 h precipitated Cr_(23)C_6 carbides in the Inconel 690 columnar grain boundaries, but not in the low-angle(and low energy) subgrain boundaries. In contrast, Cr_(23)C_6 carbides precipitated in the 316 L stainless-steel grain boundaries, but not in the low energy coherent {111} twin boundaries. Consequently, the Inconel690 subgrain boundaries essentially serve as surrogates for coherent twin boundaries with regard to avoiding carbide precipitation and corrosion sensitization.
基金supported by the National Natural Science Foundation of China(Grants 51390493 and 51266008)
文摘Existing droplet evaporation/combustion mod- els in computational fluid dynamics (CFD) simulation of spray combustion are based on simplified 1-D models. Both these models and recently developed 3-D models of single- droplet combustion do not give the conditions for the different existing droplet combustion modes. In this paper, droplet evaporation and combustion are studied both analytically and numerically. In the analytical solution, a 2-D axisymmetric flow surrounding an evaporating and combusting droplet was considered. The governing equations were solved using an integral method, similar to the Karman-Pohlhausen method for solving boundary-layer flows with pressure gradient. The results give a local evaporation rate and flame radius in agree- ment with experimental results. In numerical simulation, 3-D combusting gas flows surrounding an ethanol droplet were studied. The prediction results show three modes of droplet combustion under different relative velocities, explaining the change in the evaporation constant with an increase in relative velocity observed in experiments. This implies that different droplet combustion models should be developed in simu- lating spray combustion. The predicted local evaporation rate and flame radius by numerical simulation are in agree- ment with the analytical solution in the range of azimuthal angles 0° 〈 θ 〈 90°. The numerical results indicate that the drag force of an evaporating and combusting droplet is much smaller than that of a cold solid particle, and thus the currently used drag models should be modified.
基金supported in part by the Natural Science Foun-dation of Heilongjiang Province(No.LH2022E048)Postdoctoral Science Foundation of Heilongjiang Province(No.LBH-Z22138)China National Postdoctoral Program for Innovative Talents(No.BX20490103).
文摘<001>textured Pb(Ni_(1/3)Nb_(2/3))O_(3)-PbZrO_(3)-PbTiO_(3)(PNN-PZT)ceramics were prepared by templated grain growth(TGG)technique using 0.36PNN-x PZ-(0.64-x)PT(x=0.23,0.25 and 0.27)powder matrix.Optimum template content was derived to achieve the best electromechanical properties of textured ceramics.The piezoelectric coefficient d33=1165 pC/N,Curie temperature T_(C)=197℃,longitudinal mode electrome-chanical coupling factor k33=0.86 and a very large effective piezoelectric strain coefficient d_(33)^(*)=2041 pm/V were simultaneously achieved at the morphotropic phase boundary(MPB)composition(x=0.25)with 3 vol.%BaTiO_(3)(BT)templates.Domain structures of textured ceramics were analyzed in detail to reveal the origin of these high piezoelectric and electromechanical properties.
文摘An electrolyte model for the solid oxide fuel cell (SOFC) with proton conducting perovskite electrolyte is developed in this study, in which four types of charge carriers including proton, oxygen vacancy (oxide ion), free electron and electron hole are taken into consideration. The electrochemical process within the SOFC with hydrogen as the fuel is theoretically analyzed. With the present model, the effects of some parameters, such as the thickness of electrolyte, operating temperature and gas composition, on the ionic transport (or gas permeation) through the electrolyte and the electrical performance, i.e., the electromotive force (EMF) and internal resistance of the cell, are investigated in detail. The theoretical results are tested partly by comparing with the experimental data obtained from SrCe0.95M0.05O3-α, (M=Yb, Y) cells.
基金Supported by the National Natural Science Foundation of China(No.20076025).
文摘Proton-hole mixed conductor, SrCeo.95Yb0.05O3-α(SCYb), has the potential to be used as a membrane for dehydrogenation reactions such as methane coupling due to its high C2-selectivity and its simplicity for fabricating reactor systems. In addition, the mixed conducting membrane in the hollow fibre geometry is capable of providing high surface area per unit volume. In this study, mechanism of methane coupling reaction on the SCYb membrane was proposed and the kinetic parameters were obtained by regression of experimental data. A mathematical model describing the methane coupling in the SCYb hollow fibre membrane reactor was also developed. With this mathematical model, various operating conditions such as the operation mode, operation pressure and feed concentrations affecting performance of the reactor were investigated. The simulation results show that the cocurrent flow in the reactor exhibits higher conversion of methane and higher yield of ethylene compared to the countercurrent flow. In order to achieve the highest C2 yield, especially of ethylene, pure methane should be used as feed and the operating pressure be 300 kPa. Air can be used as the source of oxygen for the reaction and its optimum feed velocity is twice of the methane feed velocity. The air pressure in the lumen side should be kept the same as or slightly lower than the pressure of shell side.
文摘Based on the main characteristics of the tectonic-magmatic evolution of region and Tanlu fault zone,we have discussed ore-bearing magmatic rocks petrochemistry,strontium and lead isotope,and the source of ore-forming materials in Yinan skarn deposit in this paper.
基金supported by the National Natural Science Foundation of China(Grant Nos.12393854,12175121,12393851,12393852,12393853,12205314,12105301,12305120,12261160362,12105294,U1931201,12375107,and 12173039)the Department of Science and Technology of Sichuan Province,China(Grant No.24NSFSC2319)+2 种基金Project for Young Scientists in Basic Research of Chinese Academy of Sciences(Grant No.YSBR-061)in Thailand by the National Science and Technology Development Agency(NSTDA)the National Research Council of Thailand(NRCT)under the High-Potential Research Team Grant Program(Grant No.N42A650868)。
文摘In this paper,we report the detection of the very-high-energy(VHE,100 GeV<E<100 TeV)and ultra-high-energy(UHE,E>100 TeV)y-ray emissions from the direction of the young star-forming region W43,observed by the Large High Altitude Air Shower Observation(LHAASO).The extendedγ-ray source was detected with a significance of~16σby KM2A and~17σby WCDA,respectively.The angular extension of this y-ray source is about 0.5 degrees,corresponding to a physical size of about 50pc.We discuss the origin of theγ-ray emission and possible cosmic ray acceleration in the W43 region using multi-wavelength data.Our findings suggest that W43 is likely another young star cluster capable of accelerating cosmic rays(CRs)to at least several hundred TeV.
基金supported by the National Natural Science Foundation of China(Grant Nos.12393854,12393851,12393852,12393853,12205314,12105301,12305120,12261160362,12105294,U1931201,12375107,and 12173039)the Department of Science and Technology of Sichuan Province,China(Grant No.24NSFSC2319)+2 种基金the Project for Young Scientists in Basic Research of Chinese Academy of Sciences(Grant No.YSBR-061)in Thailand by the National Science and Technology Development Agency(NSTDA)the National Research Council of Thailand(NRCT)under the High-Potential Research Team Grant Program(Grant No.N42A650868)。
文摘We report the detection of an extended very-high-energy(VHE)γ-ray source coincident with the location of middle-aged(62.4 kyr)pulsar PSR J0248+6021,by using the LHAASO-WCDA data of live 796 d and LHAASO-KM2A data of live 1216d.A significant excess of y-ray induced showers is observed both by WCDA in energy bands of 1-25 TeV and KM2A in energy bands of>25 TeV with 7.3σand 13.5σ,respectively.The best-fit position derived through WCDA data is R.A.=42.06°±0.12°and Dec.=60.24°±0.13°with an extension of 0.69°±0.15°and that of the KM2A data is R.A.=42.29°±0.13°and Dec.=60.38°±0.07°with an extension of 0.37°±0.07°.No clear extended multiwavelength counterpart of this LHAASO source has been found from the radio band to the GeV band.The most plausible explanation of the VHEγ-ray emission is the inverse Compton process of highly relativistic electrons and positrons injected by the pulsar.These electrons/positrons are hypothesized to be either confined within the pulsar wind nebula or to have already escaped into the interstellar medium,forming a pulsar halo.
基金supported by the National Natural Science Foundation of China(Grant Nos.12393854,12393851,12393852,12393853,12205314,12105301,12305120,12261160362,12105294,U1931201,12375107,and 12173039)the Department of Science and Technology of Sichuan Province,China(Grant Nos.24NSFSC2319,and 2024NSFSC0449)+5 种基金the Project for Young Scientists in Basic Research of Chinese Academy of Sciences(Grant No.YSBR-061)in Thailand by the National Science and Technology Development Agency(NSTDA)the National Research Council of Thailand(NRCT)under the High-Potential Research Team Grant Program(Grant No.N42A650868)supported by the National Key R&D Program of China(Grant Nos.2023YFA1608000,and 2017YFA0402701)the CAS Key Research Program of Frontier Sciences(Grant No.QYZDJ-SSW-SLH047)used data from the Canadian Galactic Plane Survey,a Canadian project with international partners,supported by the Natural Sciences and Engineering Research Council。
文摘We report a dedicated study of the newly discovered extended UHEγ-ray source 1LHAASO J0056+6346u.Analyzing 979 d of LHAASO-WCDA data and 1389 d of LHAASO-KM2A data,we observed a significant excess ofγ-ray events with both WCDA and KM2A.Assuming a point power-law source with a fixed spectral index,the significance maps reveal excesses of 12.65σ,22.18σ,and 10.24σin the energy ranges of 1-25,25-100,and>100 TeV,respectively.We use a 3D likelihood algorithm to derive the morphological and spectral parameters,and the source is detected with significances of 13.72σby WCDA and 25.27σby KM2A.The best-fit positions derived from WCDA and KM2A data are(R.A.=13.96°±0.09°,Decl.=63.92°±0.05°)and(R.A.=14.00°±0.05°,Decl.=63.79°±0.02°),respectively.The angular size(r_(39))of 1LHAASO J0056+6346u is 0.34°±0.04°at 1-25 TeV and 0.24°±0.02°at>25 TeV.The differential flux of this UHEγ-ray source can be described by an exponential cutoff power-law function:(2.67±0.25)×10^(-15)(E/20 TeV)^((-1.97±0.10))e^(-E/(55.1±7.2)TeV)TeV^(-1)cm^(-2)s^(-1).To explore potential sources ofγ-ray emission,we investigated the gas distribution around 1LHAASO J0056+6346u.1LHAASO J0056+6346u is likely to be a TeV PWN powered by an unknown pulsar,which would naturally explain both its spatial and spectral properties.Another explanation is that this UHEγ-ray source might be associated with gas content illuminated by a nearby CR accelerator,possibly the SNR candidate G124.0+1.4.
基金Supported in part by National Key R&D Program of China(2020YFA0406300,2020YFA0406400,2023YFA1606000)National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+17 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)100 Talents Program of CAS(ZR2022JQ02,ZR2024QA151)supported by Shandong Provincial Natural Science Foundationsupported by the China Postdoctoral Science Foundation(2023M742100)The Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyGerman Research Foundation DFG(FOR5327,GRK 2149)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B16F640076,B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) events.The mass of χ_(c 0) is determined to be M (χ_(c 0))=(3415.63±0.07±0.07±0.07)MeV/c^(2),and its full width is F (χ_(c 0))=(12.52±0.12±0.13)MeV,where the first uncertainty is statistical,the second systematic,and the third for mass comes from χ_(c 2) mass uncertainty.These measurements improve the precision of χ_(c 0) mass by a factor of four and width by one order of magnitude over the previous individual measurements,and significantly boost our knowledge about the charmonium spectrum.Together with additional (345.4±2.6)×10^(6)(3686) data events taken in 2012,the decay branching fractions of χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) are measured as well,with precision improved by a factor of three compared to previous measurements.These χ_(c 0) decay branching fractions provide important inputs for the study of glueballs.
基金supported in part by National Key R&D Program of China(2020YFA0406400,2023YFA1606000,2020YFA0406300)National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+18 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)CAS(YSBR-101)100 Talents Program of CASCAS Project for Young Scientists in Basic Research(YSBR-117)The Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID),Chile(ANID PIA/APOYO AFB230003)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Using 20.3 fb^(-1)of e^(+)e^(-)annihilation data collected at a center-of-mass energy of 3.773 GeV with the BESⅢdetector,we report on an improved search for the radiative leptonic decay D^(+)→γe^(+)ve.An upper limit on its partial branching fraction for photon energies E_(γ)>10 MeV was determined to be 1.2×10^(-5)at a 90%confidence level;this excludes most current theoretical predictions.A sophisticated deep learning approach,which includes thorough validation and is based on the Transformer architecture,was implemented to efficiently distinguish the signal from massive backgrounds.
基金supported in part by the National Key R&D Program of China(2020YFA0406300,2020YFA0406400)National Natural Science Foundation of China(NSFC)(12035009,11635010,11735014,11835012,11935015,11935016,11935018,11961141012,12025502,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017)+17 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)CAS Key Research Program of Frontier Sciences(QYZDJ-SSW-SLH003,QYZDJ-SSW-SLH040)100 Talents Program of CASthe Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and Cosmologythe European Union's Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant agreement(894790)the German Research Foundation DFG(455635585),the Collaborative Research Center CRC 1044,FOR5327,GRK 2149Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF2022R1A2C1092335)National Science and Technology Fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B16F640076)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)the Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)the U.S.Department of Energy(DE-FG02-05ER41374).
文摘Using an electron-positron collision data sample corresponding to(1.0087±0.0044)×10^(10)events collected using the BESIII detector at the BEPCII collider,we firstly search for the lepton number violation decayφ→π^(+)π^(+)e^(-)e^(-)via J/ψ→φη.No obviously signals are found.The upper limit on the branching fraction ofφ→π^(+)π^(+)e^(-)e^(-)is set to be 1.3×10^(-5)at the 90%confidence level.
基金in China by the National Natural Science Foundation of China(Grant Nos.12393851,12393854,12393852,12393853,12022502,12205314,12105301,12261160362,12105294,U1931201,and 2024NSFJQ0060)in Thailand by the National Science and Technology Development Agency(NSTDA)the National Research Council of Thailand(NRCT)under the High-Potential Research Team Grant Program(Grant No.N42A650868)。
文摘The ultra-high-energy(UHE)gamma-ray source 1LHAASO J0007+7303u is positionally associated with the composite SNR CTA1 that is located at high Galactic Latitude b≈10.5°.This provides a rare opportunity to spatially resolve the component of the pulsar wind nebula(PWN)and supernova remnant(SNR)at UHE.This paper conducted a dedicated data analysis of 1LHAASO J0007+7303u using the data collected from December 2019 to July 2023.This source is well detected with significances of 21σand 17σat 8-100 TeV and>100 TeV,respectively.The corresponding extensions are determined to be 0.23°±0.03°and 0.17°±0.03°.The emission is proposed to originate from the relativistic electrons accelerated within the PWN of PSR J0007+7303.The energy spectrum is well described by a power-law with an exponential cutoff function dN/dE=(42.4±4.1)(E/20TeV)^(-2.31+0.11)exp(-E/(110±25Tev))TeV-1 cm^(-2)s^(-1)in the energy range from 8 to 300 TeV,implying a steady-state parent electron spectrum dN_(e)/dE_(e)∝(E_(e)/100TeV)^(-3.13±0.16)exp[(-E_(e)/(373±70TeV))^(2)]at energies above≈50 TeV.The cutoff energy of the electron spectrum is roughly equal to the expected current maximum energy of particles accelerated at the PWN terminal shock.Combining the X-ray and gamma-ray emission,the current space-averaged magnetic field can be limited to≈4.5μG.To satisfy the multi-wavelength spectrum and the y-ray extensions,the transport of relativistic particles within the PWN is likely dominated by the advection process under the free-expansion phase assumption.
基金National Key R&D Program of China(2023YFA1606000,2023YFA1606704)National Natural Science Foundation of China(NSFC)(11635010,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+14 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility ProgramCAS(YSBR-101)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID),Chile(ANID PIA/APOYO AFB230003)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources Institutional Development,Research and Innovation of Thailand(B50G670107)Polish National Science Centre(2024/53/B/ST2/00975)Swedish Research Council(2019.04595)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Based on a sample of 2.7x 10^(9)ψ(3686)events collected by the BESIII detector operating at the BEP-CII collider,the decay 4(3686)→YX_(cJ),X_(cJ)→ηηη’is analyzed.The decay modes X_(c1)and X_(c2)→ηηη’are observed for the first time,and their corresponding branching fractions are determined to be B(X_(c1)→ηηη’)=(1.40±0.13(stat.)±0.09(sys.))×10^(-4)and B(X_(c2)→ηηη’)=(4.18±0.84(stat.)±0.48(sys.))×10^(-5).An upper limit on the branching fraction of x_(co)→ηηη’is set as 2.59×10^(-5)at a 90%confidence level(CL).A partial wave analys-is(PWA)of the decay X_(c1)→ηηη’is performed to search for the 1^(-+)exotic stateη1(1855).The PWA result indic-ates that the structure in theηη’mass spectrum is attributed to f_(0)(1500),while in the m mass spectrum,it is attrib-uted to the 0^(++)phase space.The upper limit of B(x_(cl)→η1(1855)η)·B(η1(1855)→ηη')<9.79×10^(-5)is set based on the PWA at 90%CL.
基金Supported in part by National Key R&D Program of China(2023YFA1606000,2023YFA1606704)National Natural Science Foundation of China(NSFC)(12035009,11875170,11635010,11935015,11935016,11935018,12025502,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+16 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Program,CAS(YSBR-101)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)Shanghai Key Laboratory for Particle Physics and CosmologyAgencia Nacional de Investigación y Desarrollo de Chile(ANID)Chile(ANID PIA/APOYO AFB230003)ERC(758462)German Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaPolish National Science Centre(2024/53/B/ST2/00975)STFC(United Kingdom)Swedish Research Council(2019.04595)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Lepton number violation decayω→π^(+)π^(+)e^(-)e^(-)+c.c.is searched for via J/ψ→ωηusing a data sample of(1.0087±0.0044)×10^(10)J/ψevents collected via the BESIII detector at the BEPCII collider.No significant signal is observed,and the upper limit on the branching fraction ofω→π^(+)π^(+)e^(-)e^(-)+c.c.at the 90%confidence level is determined for the first time to be 2.8×10^(-6).
基金Supported in part by the National Key R&D Program of China(2023YFA1606000,2020YFA0406400,2020YFA0406300)the National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11875054,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+12 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)the Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U2032104,U1832207)the 100 Talents Program of CAS,the Excellent Youth Foundation of Henan Scientific Commitee(242300421044)the Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and Cosmology,the German Research Foundation DFG(FOR5327)the Istituto Nazionale di Fisica Nucleare,Italy,the Knut and Alice Wallenberg Foundation(2021.0174,2021.0299)the Ministry of Development of Turkey(DPT2006K-120470),the National Research Foundation of Korea(NRF-2022R1A2C1092335)the National Science and Technology Fund of Mongoliathe National Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research,and Innovation of Thailand(B16F640076,B50G670107)the Polish National Science Center(2019/35/O/ST2/02907)the Swedish Research Council(2019.04595)the Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)the US Department of Energy(DE-FG02-05ER41374)。
文摘We search for the leptonic decay D^(+)→e^(+)ν_(e)using an e+e-collision data sample with an integrated luminosity of 20.3 fb-1collected with the BESIII detector at a center-of-mass energy of 3.773 GeV.Significant signal is not observed,and an upper limit on the branching fraction of D^(+)→e^(+)ν_(e)is set as 9.7×10^(-7),at a confidence level of 90%.Our upper limit is an order of magnitude smaller than the previous limit for this decay mode.
基金supported in part by National Key R&D Program of China(2020YFA0406300,2020YFA0406400,2023YFA1606000)National Natural Science Foundation of China(NSFC)(12205141,11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+16 种基金Natural Science Foundation of Hunan Province(2024JJ2044)the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)100 Talents Program of CASThe Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyGerman Research Foundation DFG(FOR5327)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B16F640076,B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘Utilizing 4.5 fb^(-1)ofe^(+)e^(-)annihilation data collected at center-of-mass energies ranging from 4599.53 MeV to 4698.82 MeV by the BESIII detector at the BEPCII collider,we searched for singly Cabibbo-suppressed hadronic decaysΛ_(c)^(+)→Σ^(0)K^(+)π^(0)andΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−)and with a single-tag method.No significant signals were observed for both decays.The upper limits on the branching fractions at the 90%confidence level were determined to be 5.0×10^(-4)for and forΛ_(c)^(+)→Σ^(0)K^(+)π^(0)and 6.5×10^(-4)forΛ_(c)^(+)→Σ^(0)K^(+)π^(+)π^(−).