Edge defects significantly impact the forming quality of Mg/Al composite plates during the rolling process.This study aims to develop an effective rolling technique to suppress these defects.First,an enhanced Lemaitre...Edge defects significantly impact the forming quality of Mg/Al composite plates during the rolling process.This study aims to develop an effective rolling technique to suppress these defects.First,an enhanced Lemaitre damage model with a generalized stress state damage prediction mechanism was used to evaluate the key mechanical factors contributing to defect formation.Based on this evaluation,an embedded composite rolling technique was proposed.Subsequently,comparative validation was conducted at 350℃ with a 50% reduction ratio.Results showed that the plates rolled using the embedded composite rolling technique had smooth surfaces and edges,with no macroscopic cracks observed.Numerical simulation indicated that,compared to conventional processes,the proposed technique reduced the maximum edge stress triaxiality of the plates from-0.02 to-1.56,significantly enhancing the triaxial compressive stress effect at the edges,which suppressed void nucleation and growth,leading to a 96%reduction in damage values.Mechanical property evaluations demonstrated that,compared to the conventional rolling process,the proposed technique improved edge bonding strength and tensile strength by approximately 67.7%and 118%,respectively.Further microstructural characterization revealed that the proposed technique,influenced by the restriction of deformation along the transverse direction(TD),weakened the plastic flow in the TD and enhanced plastic flow along the rolling direction(RD),resulting in higher grain boundary density and stronger basal texture.This,in turn,improved the toughness and transverse homogeneity of the plates.In summary,the embedded composite rolling technique provides crucial technical guidance for the preparation of Mg-based composite plates.展开更多
Polyvinyl chloride(PVC)is one of the most widely used plastic materials worldwide,particularly in long-life applications such as construction materials.However,recycling options for PVC waste remain limited,as convent...Polyvinyl chloride(PVC)is one of the most widely used plastic materials worldwide,particularly in long-life applications such as construction materials.However,recycling options for PVC waste remain limited,as conventional methods often degrade material quality or generate environmentally hazardous byproducts.In this study,we demonstrate an efficient process to convert PVC into new polymers with variable aromatic groups,using triethylsilane as the reductant in different solvents.This approach enables the production of polymers analogous to functionalized polyethylene(PE),which are typically challenging to obtain through conventional copolymerization or direct post-modification of C-H bonds in PE.The resulting polymers exhibit tunable thermal and mechanical properties depending on the introduced aromatic groups,which not only enhance the sustainable valorization of PVC waste,but also provide an opportunity for the synthesis of new functionalized polymers.展开更多
The redshifted 21 cm line,arising from neutral hydrogen,offers a unique probe into the intergalactic medium and the first stars and galaxies formed in the early universe.However,detecting this signal is a challenging ...The redshifted 21 cm line,arising from neutral hydrogen,offers a unique probe into the intergalactic medium and the first stars and galaxies formed in the early universe.However,detecting this signal is a challenging task because of artificial radio-frequency interference(RFI)and systematic errors such as ground effects.The interior of the Antarctic continent provides an excellent location to make such observations,with minimal RFI and relatively stable foreground signals.Moreover,a flat plateau in central Antarctica,with an ice cap over 2000 m deep,will show less ground reflection of radio waves,reducing the signal complexity in the area around the probing antenna.It may be advantageous to perform cosmological 21 cm experiments in Antarctica,and a 21 cm Antarctic global spectrum experiment can potentially be deployed on the Antarctic ice cap.We have performed preliminary instrumental design,system calibration,and implementation of such an instrument optimized for extreme cold and capable of long-term autonomous operation.This system shows the ability to effectively detect the 21 cm signal,confirming Antarctica as an excellent observational site for radio cosmology.展开更多
Objective:To explore the clinical value of autologous skull transplantation in the treatment of skull defects.Methods:Sixty-six patients who underwent skull defect reconstruction treatment in our hospital from January...Objective:To explore the clinical value of autologous skull transplantation in the treatment of skull defects.Methods:Sixty-six patients who underwent skull defect reconstruction treatment in our hospital from January 2022 to March 2024 were selected and divided into an autologous skull transplantation group(n=31)and an artificial bone transplantation material group(n=35)based on different bone transplantation materials.The two groups of patients were followed up for 12 months to observe the bone healing and the incidence of postoperative complications.Results:After 9 months of treatment,the bone healing performance of the autologous skull transplantation group was better than that of the artificial bone transplantation material group(P<0.05).By the end of the last follow-up,the incidence of bony postoperative complications in the autologous skull transplantation group was lower than that in the artificial bone transplantation material group(P<0.05).Conclusion:Autologous skull repair for skull defects has good biocompatibility,can promote bone healing,and reduce the incidence of postoperative complications.展开更多
Oil and gas pipeline networks are a key link in the coordinated development of oil and gas both upstream and downstream.To improve the reliability and safety of the oil and gas pipeline network, inspections are implem...Oil and gas pipeline networks are a key link in the coordinated development of oil and gas both upstream and downstream.To improve the reliability and safety of the oil and gas pipeline network, inspections are implemented to minimize the risk of leakage, spill and theft, as well as documenting actual incidents. In recent years, unmanned aerial vehicles have been recognized as a promising option for inspection due to their high efficiency. However, the integrated optimization of unmanned aerial vehicle inspection for oil and gas pipeline networks, including physical feasibility, the performance of mission, cooperation, real-time implementation and three-dimensional(3-D) space, is a strategic problem due to its large-scale,complexity as well as the need for efficiency. In this work, a novel mixed-integer nonlinear programming model is proposed that takes into account the constraints of the mission scenario and the safety performance of unmanned aerial vehicles. To minimize the total length of the inspection path, the model is solved by a two-stage solution method. Finally, a virtual pipeline network and a practical pipeline network are set as two examples to demonstrate the performance of the optimization schemes. Moreover, compared with the traditional genetic algorithm and simulated annealing algorithm, the self-adaptive genetic simulated annealing algorithm proposed in this paper provides strong stability.展开更多
Luminescent nanoparticles(upconversion nanoparticles,carbon dots,silicon nanoparticles and nanophosphors)have the advantages of tunable photoluminescence,good biocompatibility,low cytotoxicity and chemical/physical st...Luminescent nanoparticles(upconversion nanoparticles,carbon dots,silicon nanoparticles and nanophosphors)have the advantages of tunable photoluminescence,good biocompatibility,low cytotoxicity and chemical/physical stability.Recently,the luminescent nanoparticles have been involved in the plant research for imaging plant phenotype and improving the photosynthesis efficiency.Luminescent nanoparticles are applied for the plant imaging in vivo and in vitro,while the plant photosynthesis is dependent on the specific light wavelength,providing the luminescent nanoparticles an opportunity to optimize the agriculture light.This review presents the recent developments of luminescent nanoparticles applied on the plant imaging and photosynthesis and discusses the trend for future research.展开更多
The petrol truck routing problem is an important part of the petrol supply chain.This study focuses on determining routes for distributing petrol products from a depot to petrol stations with the objective of minimizi...The petrol truck routing problem is an important part of the petrol supply chain.This study focuses on determining routes for distributing petrol products from a depot to petrol stations with the objective of minimizing the total travel cost and the fixed cost required to use the trucks.We propose a mathematical model that considers petrol trucks returning to a depot multiple times and develop a heuristic algorithm based on a local branch-and-bound search with a tabu list and the Metropolis acceptance criterion.In addition,an approach that accelerates the solution process by adding several valid inequalities is presented.In this study,the trucks are homogeneous and have two compartments,and each truck can execute at most three tasks daily.The sales company arranges the transfer amount and the time windows for each station.The performance of the proposed algorithm is evaluated by comparing its results with the optimal results.In addition,a real-world case of routing petrol trucks in Beijing is studied to demonstrate the effectiveness of the proposed approach.展开更多
To save energy and raise molding and coremaking productivity, the synthetic procedure of novolaks for the shell process was investigated. The study indicated that it was difficult to obtain fast curing novolaks under ...To save energy and raise molding and coremaking productivity, the synthetic procedure of novolaks for the shell process was investigated. The study indicated that it was difficult to obtain fast curing novolaks under strongly acidic conditions alone. A novel synthetic procedure was proposed for preparing novolaks in a two-step manner, a divalent metal salt catalyzed novolak preparation followed by a strong acid catalyzed novolak preparation. The optimum conditions for the two-step procedure were determined by orthogonal experiment design. The results showed that it was easy to prepare fast curing novolaks with cure time in the range of 20 s to 30 s and softening point in the range of 80℃ to 90℃ under complex catalysis conditions.展开更多
Timely and accurate population statistic data plays an important role in many fields.To illustrate the demographic characteristics,population density is a crucial factor in evaluating population data.With a dynamic re...Timely and accurate population statistic data plays an important role in many fields.To illustrate the demographic characteristics,population density is a crucial factor in evaluating population data.With a dynamic regional migration in population,it is a challenging job to evaluate population density without a census-based survey.We present the approach to classify satellite images in different magnitudes in population density and execute the comparative experiment to discuss the factors that influence the identification to the images with the deep learning approach.In this paper,we use satellite imagery and community population density data.With convolutional neural networks,we evaluated the performance of CNN on population estimation with satellite images,found the features that are important in population estimation,and then perform the sensitive analysis.展开更多
Biomass chemical looping gasification technology is one of the essential ways to utilize abundant biomass resources.At the same time,dimethyl carbonate can replace phosgene as an environmentfriendly organic material f...Biomass chemical looping gasification technology is one of the essential ways to utilize abundant biomass resources.At the same time,dimethyl carbonate can replace phosgene as an environmentfriendly organic material for the synthesis of polycarbonate.In this paper,a novel system coupling biomass chemical looping gasification with dimethyl carbonate synthesis with methanol as an intermediate is designed through microscopic mechanism analysis and process optimization.Firstly,reactive force field molecular dynamics simulation is performed to explore the reaction mechanism of biomass chemical looping gasification to determine the optimal gasification temperature range.Secondly,steady-state simulations of the process based on molecular dynamics simulation results are carried out to investigate the effects of temperature,steam to biomass ratio,and oxygen carrier to biomass ratio on the syngas yield and compositions.In addition,the main energy indicators of biomass chemical looping gasification process including lower heating value and cold gas efficiency are analyzed based on the above optimum parameters.Then,two synthesis stages are simulated and optimized with the following results obtained:the optimal temperature and pressure of methanol synthesis stage are 150℃ and 4 MPa;the optimal temperature and pressure of dimethyl carbonate synthesis stage are 140℃ and 0.3 MPa.Finally,the pre-separation-extraction-decantation process separates the mixture of dimethyl carbonate and methanol generated in the synthesis stage with 99.11%purity of dimethyl carbonate.Above results verify the feasibility of producing dimethyl carbonate from the perspective of multi-scale simulation and realize the multi-level utilization of biomass resources.展开更多
The development of low-cost, efficient, and high atomic economy electrocatalysts for hydrogen evolution reaction(HER) in the entire p H range for sustainable hydrogen production is of great importance but still challe...The development of low-cost, efficient, and high atomic economy electrocatalysts for hydrogen evolution reaction(HER) in the entire p H range for sustainable hydrogen production is of great importance but still challenging. Herein, we synthesize a highly dispersed N-doped carbon frames(NCFs) anchored with Co single atoms(SAs) and Co nanoparticles(NPs) catalyst by a doping-adsorption-pyrolysis strategy for electrocatalytic hydrogen evolution. The Co SAs-Co NPs/NCFs catalyst exhibits an excellent HER activity with small overpotential, low Tafel slope, high turnover frequency as well as remarkable stability. It also exhibits a superior HER performance in the entire p H range. Combining with experimental and theoretical calculation, we find that Co SAs with Co-N_(3) coordination structure and Co NPs have a strong interaction for promoting synergistic HER electrocatalytic process. The H_(2)O molecule is easily activated and dissociated on Co NPs, while the generated H^(*) is easily adsorbed on Co SAs for HER, which makes the Co SAs-Co NPs/NCFs catalyst exhibit more suitable H adsorption strength and more conducive to the activation and dissociation of H_(2)O molecules. This work not only proposes a novel idea for constructing coupling catalyst with atomic-level precision, but also provides strong reference for the development of high-efficiency HER electrocatalysts for practical application.展开更多
Nowadays,the efficient and cleaner utilization of coal have attracted wide attention due to the rich coal and rare oil/gas resources structure in China.Coal chemical looping gasification(CCLG)is a promising coal utili...Nowadays,the efficient and cleaner utilization of coal have attracted wide attention due to the rich coal and rare oil/gas resources structure in China.Coal chemical looping gasification(CCLG)is a promising coal utilization technology to achieve energy conservation and emission reduction targets for highly pure synthesis gas.As a downstream product of synthesis gas,methyl methacrylate(MMA),is widely used as raw material for synthesizing polymethyl methacrylate and resin products with excellent properties.So this paper proposes a novel system integrating MMA production and CCLG(CCLG-MMA)processes aiming at"energy saving and low emission",in which the synthesis gas produced by CCLG and purified by dry methane reforming(DMR)reaction and Rectisol process reacts with ethylene for synthesizing MMA.Firstly,the reaction mechanism of CCLG is investigated by using Reactive force field(ReaxFF)MD simulation based on atomic models of char and oxygen carrier(Fe_(2)O_(3))for obtaining optimum reaction temperature of fuel reactor(FR).Secondly,the steady-state simulation of CCLG-MMA system is carried out to verify the feasibility of MMA production.The amount of CO_(2)emitted by CCLG process and DMR reaction is 0.0028(kg CO_(2))^(-1)·(kg MMA)^(-1).The total energy consumption of the CCLG-MMA system is 45521 kJ·(kg MMA)^(-1),among which the consumption of MMA production part is 25293 k(·kg MMA)^(-1).The results show that the CCLG-MMA system meets CO_(2)emission standard and has lower energy consumption compared to conventional MMA production process.Finally,one control scheme is designed to verify the stability of CCLG-MMA system.The CCLG-MMA integration strategy aims to obtain highly pure MMA from multi-scale simulation perspectives,so this is an optimal design regarding all factors influencing cleaner MMA production.展开更多
The Global Navigation Satellite System(GNSS)has been widely used in various fields.To achieve positioning,the receiver must first lock the satellite signal.This is a complicated and expensive process that consumes a l...The Global Navigation Satellite System(GNSS)has been widely used in various fields.To achieve positioning,the receiver must first lock the satellite signal.This is a complicated and expensive process that consumes a lot of resources of the receiver.For this reason,this paper proposes a new fast acquisition algorithm with High Signal-tonoise ratio(SNR)performance based on sparse fast Fourier transform(HSFFT).The algorithm first replaces the IFFT process of the traditional parallel code phase capture algorithm with inverse sparse fast Fourier transform(ISFFT)with better computing performance,and then uses linear search combined with code phase discrimination to replace the positioning loop and the estimation loop with poor noise immunity in ISFFT.Theoretical analysis and simulation results show that,compared with the existing SFFT parallel code phase capture algorithm,the calculation amount of this algorithm is reduced by 19%,and the SNR performance is improved by about 5dB.Compared with the classic FFT parallel code phase capture algorithm,the calculation amount of the algorithm in this paper is reduced by 43%,and when the capture probability is greater than 95%,the SNR performance of the two is approximately the same.展开更多
Direct-current(DC)arc plasma has great application values in the field of the chemical industry,but it has the problem of low energy efficiency.Facing the requirement for improving the energy efficiency of the arc,thi...Direct-current(DC)arc plasma has great application values in the field of the chemical industry,but it has the problem of low energy efficiency.Facing the requirement for improving the energy efficiency of the arc,this paper proposes a unique method of pulsed modulated arc(PMA).This method uses high-frequency pulses and reduces the arc current to improve the control of electron temperature.The electrical characteristics,optical characteristics and products are tested.The test results show that during the PMA process,all of the experimental results which include voltage,current and light will significantly increase.These results are analyzed from the perspective of functionality,repeatability and energy conversion.The analysis results show that although the PMA method does not show good parameter consistency,it has potential application prospects because it increases the energy conversion rate by 4.5%and 8%from the perspective of light and products,respectively.展开更多
A rate-dependent peridynamic ceramic model,considering the brittle tensile response,compressive plastic softening and strain-rate dependence,can accurately represent the dynamic response and crack propagation of ceram...A rate-dependent peridynamic ceramic model,considering the brittle tensile response,compressive plastic softening and strain-rate dependence,can accurately represent the dynamic response and crack propagation of ceramic materials.However,it also considers the strain-rate dependence and damage accumulation caused by compressive plastic softening during the compression stage,requiring more computational resources for the bond force evaluation and damage evolution.Herein,the OpenMP parallel optimization of the rate-dependent peridynamic ceramicmodel is investigated.Also,themodules that compute the interactions betweenmaterial points and update damage index are vectorized and parallelized.Moreover,the numerical examples are carried out to simulate the dynamic response and fracture of the ceramic plate under normal impact.Furthermore,the speed-up ratio and computational efficiency by multi-threads are evaluated and discussed to demonstrate the reliability of parallelized programs.The results reveal that the totalwall clock time has been significantly reduced after optimization,showing the promise of parallelization process in terms of accuracy and stability.展开更多
1.Introduction Carbon neutrality has emerged as a global goal due to its pivotal role in addressing the challenges of global climate change.Before the United Nations Climate Summit was held in November 2020,124 countr...1.Introduction Carbon neutrality has emerged as a global goal due to its pivotal role in addressing the challenges of global climate change.Before the United Nations Climate Summit was held in November 2020,124 countries promised to reach net-zero emissions[1].Solar energy is one of the important renewable energy sources that significantly curtail carbon emissions originating from fossil fuels.展开更多
Due to the huge amount of increasing data, the requirements of people forelectronic products such as mobile phones, tablets, and notebooks are constantlyimproving. The development and design of various software applic...Due to the huge amount of increasing data, the requirements of people forelectronic products such as mobile phones, tablets, and notebooks are constantlyimproving. The development and design of various software applications attach greatimportance to users’ experiences. The rationalized UI design should allow a user not onlyenjoy the visual design experience of the new product but also operating it morepleasingly. This process is to enhance the attractiveness and performance of the newproduct and thus to promote the active usage and consuming conduct of users. In thispaper, an UI design optimization strategy for general APP in the big data environment isproposed to get better user experience while effectively obtaining information. Anexperimental example of a library APP is designed to optimize the user experience. Theexperimental results show that the user-centered UI design is the core of optimization,and user portrait based on big data platforms is the key to UI design.展开更多
基金supported by National Key Research and Development Program(2018YFA0707300)Major Program of National Natural Science Foundation of China(U22A20188).
文摘Edge defects significantly impact the forming quality of Mg/Al composite plates during the rolling process.This study aims to develop an effective rolling technique to suppress these defects.First,an enhanced Lemaitre damage model with a generalized stress state damage prediction mechanism was used to evaluate the key mechanical factors contributing to defect formation.Based on this evaluation,an embedded composite rolling technique was proposed.Subsequently,comparative validation was conducted at 350℃ with a 50% reduction ratio.Results showed that the plates rolled using the embedded composite rolling technique had smooth surfaces and edges,with no macroscopic cracks observed.Numerical simulation indicated that,compared to conventional processes,the proposed technique reduced the maximum edge stress triaxiality of the plates from-0.02 to-1.56,significantly enhancing the triaxial compressive stress effect at the edges,which suppressed void nucleation and growth,leading to a 96%reduction in damage values.Mechanical property evaluations demonstrated that,compared to the conventional rolling process,the proposed technique improved edge bonding strength and tensile strength by approximately 67.7%and 118%,respectively.Further microstructural characterization revealed that the proposed technique,influenced by the restriction of deformation along the transverse direction(TD),weakened the plastic flow in the TD and enhanced plastic flow along the rolling direction(RD),resulting in higher grain boundary density and stronger basal texture.This,in turn,improved the toughness and transverse homogeneity of the plates.In summary,the embedded composite rolling technique provides crucial technical guidance for the preparation of Mg-based composite plates.
基金the Beijing Natural Science Foundation(Z240029)the National Natural Science Foundation of China(22472004)+2 种基金China National Petroleum Corporation-Peking University Strategic Cooperation Project of Fundamental Researchthe New Cornerstone Science Foundationsupport from the Tencent Foundation through the Xplorer Prize.
文摘Polyvinyl chloride(PVC)is one of the most widely used plastic materials worldwide,particularly in long-life applications such as construction materials.However,recycling options for PVC waste remain limited,as conventional methods often degrade material quality or generate environmentally hazardous byproducts.In this study,we demonstrate an efficient process to convert PVC into new polymers with variable aromatic groups,using triethylsilane as the reductant in different solvents.This approach enables the production of polymers analogous to functionalized polyethylene(PE),which are typically challenging to obtain through conventional copolymerization or direct post-modification of C-H bonds in PE.The resulting polymers exhibit tunable thermal and mechanical properties depending on the introduced aromatic groups,which not only enhance the sustainable valorization of PVC waste,but also provide an opportunity for the synthesis of new functionalized polymers.
基金supported by the Polar Research Institute of China and the Chinese Arctic and Antarctic Administrationsupported by the Chinese Academy of Science Key Instrument(ZDKYYQ20200008)the National Natural Science Foundation of China(12473094 and 12273070).
文摘The redshifted 21 cm line,arising from neutral hydrogen,offers a unique probe into the intergalactic medium and the first stars and galaxies formed in the early universe.However,detecting this signal is a challenging task because of artificial radio-frequency interference(RFI)and systematic errors such as ground effects.The interior of the Antarctic continent provides an excellent location to make such observations,with minimal RFI and relatively stable foreground signals.Moreover,a flat plateau in central Antarctica,with an ice cap over 2000 m deep,will show less ground reflection of radio waves,reducing the signal complexity in the area around the probing antenna.It may be advantageous to perform cosmological 21 cm experiments in Antarctica,and a 21 cm Antarctic global spectrum experiment can potentially be deployed on the Antarctic ice cap.We have performed preliminary instrumental design,system calibration,and implementation of such an instrument optimized for extreme cold and capable of long-term autonomous operation.This system shows the ability to effectively detect the 21 cm signal,confirming Antarctica as an excellent observational site for radio cosmology.
文摘Objective:To explore the clinical value of autologous skull transplantation in the treatment of skull defects.Methods:Sixty-six patients who underwent skull defect reconstruction treatment in our hospital from January 2022 to March 2024 were selected and divided into an autologous skull transplantation group(n=31)and an artificial bone transplantation material group(n=35)based on different bone transplantation materials.The two groups of patients were followed up for 12 months to observe the bone healing and the incidence of postoperative complications.Results:After 9 months of treatment,the bone healing performance of the autologous skull transplantation group was better than that of the artificial bone transplantation material group(P<0.05).By the end of the last follow-up,the incidence of bony postoperative complications in the autologous skull transplantation group was lower than that in the artificial bone transplantation material group(P<0.05).Conclusion:Autologous skull repair for skull defects has good biocompatibility,can promote bone healing,and reduce the incidence of postoperative complications.
基金part of the Program of "Study on Optimization and Supply-side Reliability of Oil Product Supply Chain Logistics System" funded under the National Natural Science Foundation of China, Grant Number 51874325
文摘Oil and gas pipeline networks are a key link in the coordinated development of oil and gas both upstream and downstream.To improve the reliability and safety of the oil and gas pipeline network, inspections are implemented to minimize the risk of leakage, spill and theft, as well as documenting actual incidents. In recent years, unmanned aerial vehicles have been recognized as a promising option for inspection due to their high efficiency. However, the integrated optimization of unmanned aerial vehicle inspection for oil and gas pipeline networks, including physical feasibility, the performance of mission, cooperation, real-time implementation and three-dimensional(3-D) space, is a strategic problem due to its large-scale,complexity as well as the need for efficiency. In this work, a novel mixed-integer nonlinear programming model is proposed that takes into account the constraints of the mission scenario and the safety performance of unmanned aerial vehicles. To minimize the total length of the inspection path, the model is solved by a two-stage solution method. Finally, a virtual pipeline network and a practical pipeline network are set as two examples to demonstrate the performance of the optimization schemes. Moreover, compared with the traditional genetic algorithm and simulated annealing algorithm, the self-adaptive genetic simulated annealing algorithm proposed in this paper provides strong stability.
基金Project supported by the National Natural Science Foundations of China(21671070)the GDUPS(2018)for Prof.Bingfu LEIthe Guangzhou Science & Technology Project(201707010033,201704030086)
文摘Luminescent nanoparticles(upconversion nanoparticles,carbon dots,silicon nanoparticles and nanophosphors)have the advantages of tunable photoluminescence,good biocompatibility,low cytotoxicity and chemical/physical stability.Recently,the luminescent nanoparticles have been involved in the plant research for imaging plant phenotype and improving the photosynthesis efficiency.Luminescent nanoparticles are applied for the plant imaging in vivo and in vitro,while the plant photosynthesis is dependent on the specific light wavelength,providing the luminescent nanoparticles an opportunity to optimize the agriculture light.This review presents the recent developments of luminescent nanoparticles applied on the plant imaging and photosynthesis and discusses the trend for future research.
基金the Program of “Study on Optimization and Supply-side Reliability of Oil Product Supply Chain Logistics System” funded under the National Natural Science Foundation of China, Grant Number 51874325
文摘The petrol truck routing problem is an important part of the petrol supply chain.This study focuses on determining routes for distributing petrol products from a depot to petrol stations with the objective of minimizing the total travel cost and the fixed cost required to use the trucks.We propose a mathematical model that considers petrol trucks returning to a depot multiple times and develop a heuristic algorithm based on a local branch-and-bound search with a tabu list and the Metropolis acceptance criterion.In addition,an approach that accelerates the solution process by adding several valid inequalities is presented.In this study,the trucks are homogeneous and have two compartments,and each truck can execute at most three tasks daily.The sales company arranges the transfer amount and the time windows for each station.The performance of the proposed algorithm is evaluated by comparing its results with the optimal results.In addition,a real-world case of routing petrol trucks in Beijing is studied to demonstrate the effectiveness of the proposed approach.
文摘To save energy and raise molding and coremaking productivity, the synthetic procedure of novolaks for the shell process was investigated. The study indicated that it was difficult to obtain fast curing novolaks under strongly acidic conditions alone. A novel synthetic procedure was proposed for preparing novolaks in a two-step manner, a divalent metal salt catalyzed novolak preparation followed by a strong acid catalyzed novolak preparation. The optimum conditions for the two-step procedure were determined by orthogonal experiment design. The results showed that it was easy to prepare fast curing novolaks with cure time in the range of 20 s to 30 s and softening point in the range of 80℃ to 90℃ under complex catalysis conditions.
文摘Timely and accurate population statistic data plays an important role in many fields.To illustrate the demographic characteristics,population density is a crucial factor in evaluating population data.With a dynamic regional migration in population,it is a challenging job to evaluate population density without a census-based survey.We present the approach to classify satellite images in different magnitudes in population density and execute the comparative experiment to discuss the factors that influence the identification to the images with the deep learning approach.In this paper,we use satellite imagery and community population density data.With convolutional neural networks,we evaluated the performance of CNN on population estimation with satellite images,found the features that are important in population estimation,and then perform the sensitive analysis.
基金supported by the National Natural Science Foundation of China(22178189)the Natural Science Foundation of Shandong Province(ZR2021MB113)the Postdoctoral Science Foundation of China(2022M711746)。
文摘Biomass chemical looping gasification technology is one of the essential ways to utilize abundant biomass resources.At the same time,dimethyl carbonate can replace phosgene as an environmentfriendly organic material for the synthesis of polycarbonate.In this paper,a novel system coupling biomass chemical looping gasification with dimethyl carbonate synthesis with methanol as an intermediate is designed through microscopic mechanism analysis and process optimization.Firstly,reactive force field molecular dynamics simulation is performed to explore the reaction mechanism of biomass chemical looping gasification to determine the optimal gasification temperature range.Secondly,steady-state simulations of the process based on molecular dynamics simulation results are carried out to investigate the effects of temperature,steam to biomass ratio,and oxygen carrier to biomass ratio on the syngas yield and compositions.In addition,the main energy indicators of biomass chemical looping gasification process including lower heating value and cold gas efficiency are analyzed based on the above optimum parameters.Then,two synthesis stages are simulated and optimized with the following results obtained:the optimal temperature and pressure of methanol synthesis stage are 150℃ and 4 MPa;the optimal temperature and pressure of dimethyl carbonate synthesis stage are 140℃ and 0.3 MPa.Finally,the pre-separation-extraction-decantation process separates the mixture of dimethyl carbonate and methanol generated in the synthesis stage with 99.11%purity of dimethyl carbonate.Above results verify the feasibility of producing dimethyl carbonate from the perspective of multi-scale simulation and realize the multi-level utilization of biomass resources.
基金supported by the Taishan Scholars Program of Shandong Province(tsqn201909065)the Shandong Provincial Natural Science Foundation(ZR2020QB174)+3 种基金the Petro China Innovation Foundation(2019D-5007-0401)the National Natural Science Foundation of China(21776315,22108306)the Fundamental Research Funds for the Central Universities(19CX02008A,19CX05001A)the Postgraduate Innovation Fund of China University of Petroleum(East China)(YCX2020037)。
文摘The development of low-cost, efficient, and high atomic economy electrocatalysts for hydrogen evolution reaction(HER) in the entire p H range for sustainable hydrogen production is of great importance but still challenging. Herein, we synthesize a highly dispersed N-doped carbon frames(NCFs) anchored with Co single atoms(SAs) and Co nanoparticles(NPs) catalyst by a doping-adsorption-pyrolysis strategy for electrocatalytic hydrogen evolution. The Co SAs-Co NPs/NCFs catalyst exhibits an excellent HER activity with small overpotential, low Tafel slope, high turnover frequency as well as remarkable stability. It also exhibits a superior HER performance in the entire p H range. Combining with experimental and theoretical calculation, we find that Co SAs with Co-N_(3) coordination structure and Co NPs have a strong interaction for promoting synergistic HER electrocatalytic process. The H_(2)O molecule is easily activated and dissociated on Co NPs, while the generated H^(*) is easily adsorbed on Co SAs for HER, which makes the Co SAs-Co NPs/NCFs catalyst exhibit more suitable H adsorption strength and more conducive to the activation and dissociation of H_(2)O molecules. This work not only proposes a novel idea for constructing coupling catalyst with atomic-level precision, but also provides strong reference for the development of high-efficiency HER electrocatalysts for practical application.
基金supported by the National Natural Science Foundation of China(21576143)Foundation of State Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering(2020-KF-13)。
文摘Nowadays,the efficient and cleaner utilization of coal have attracted wide attention due to the rich coal and rare oil/gas resources structure in China.Coal chemical looping gasification(CCLG)is a promising coal utilization technology to achieve energy conservation and emission reduction targets for highly pure synthesis gas.As a downstream product of synthesis gas,methyl methacrylate(MMA),is widely used as raw material for synthesizing polymethyl methacrylate and resin products with excellent properties.So this paper proposes a novel system integrating MMA production and CCLG(CCLG-MMA)processes aiming at"energy saving and low emission",in which the synthesis gas produced by CCLG and purified by dry methane reforming(DMR)reaction and Rectisol process reacts with ethylene for synthesizing MMA.Firstly,the reaction mechanism of CCLG is investigated by using Reactive force field(ReaxFF)MD simulation based on atomic models of char and oxygen carrier(Fe_(2)O_(3))for obtaining optimum reaction temperature of fuel reactor(FR).Secondly,the steady-state simulation of CCLG-MMA system is carried out to verify the feasibility of MMA production.The amount of CO_(2)emitted by CCLG process and DMR reaction is 0.0028(kg CO_(2))^(-1)·(kg MMA)^(-1).The total energy consumption of the CCLG-MMA system is 45521 kJ·(kg MMA)^(-1),among which the consumption of MMA production part is 25293 k(·kg MMA)^(-1).The results show that the CCLG-MMA system meets CO_(2)emission standard and has lower energy consumption compared to conventional MMA production process.Finally,one control scheme is designed to verify the stability of CCLG-MMA system.The CCLG-MMA integration strategy aims to obtain highly pure MMA from multi-scale simulation perspectives,so this is an optimal design regarding all factors influencing cleaner MMA production.
文摘The Global Navigation Satellite System(GNSS)has been widely used in various fields.To achieve positioning,the receiver must first lock the satellite signal.This is a complicated and expensive process that consumes a lot of resources of the receiver.For this reason,this paper proposes a new fast acquisition algorithm with High Signal-tonoise ratio(SNR)performance based on sparse fast Fourier transform(HSFFT).The algorithm first replaces the IFFT process of the traditional parallel code phase capture algorithm with inverse sparse fast Fourier transform(ISFFT)with better computing performance,and then uses linear search combined with code phase discrimination to replace the positioning loop and the estimation loop with poor noise immunity in ISFFT.Theoretical analysis and simulation results show that,compared with the existing SFFT parallel code phase capture algorithm,the calculation amount of this algorithm is reduced by 19%,and the SNR performance is improved by about 5dB.Compared with the classic FFT parallel code phase capture algorithm,the calculation amount of the algorithm in this paper is reduced by 43%,and when the capture probability is greater than 95%,the SNR performance of the two is approximately the same.
基金supported by National Natural Science Foundation of China(No.52177135)the National Science and Technology Major Project of China(Nos.2017-Ⅲ-0007-0032,2019-Ⅲ-0013-0056)。
文摘Direct-current(DC)arc plasma has great application values in the field of the chemical industry,but it has the problem of low energy efficiency.Facing the requirement for improving the energy efficiency of the arc,this paper proposes a unique method of pulsed modulated arc(PMA).This method uses high-frequency pulses and reduces the arc current to improve the control of electron temperature.The electrical characteristics,optical characteristics and products are tested.The test results show that during the PMA process,all of the experimental results which include voltage,current and light will significantly increase.These results are analyzed from the perspective of functionality,repeatability and energy conversion.The analysis results show that although the PMA method does not show good parameter consistency,it has potential application prospects because it increases the energy conversion rate by 4.5%and 8%from the perspective of light and products,respectively.
基金supported by the National Natural Science Foundation of China(Nos.11972267,11802214 and 51932006)the Fundamental Research Funds for the Central Universities(WUT:2020lll031GX).
文摘A rate-dependent peridynamic ceramic model,considering the brittle tensile response,compressive plastic softening and strain-rate dependence,can accurately represent the dynamic response and crack propagation of ceramic materials.However,it also considers the strain-rate dependence and damage accumulation caused by compressive plastic softening during the compression stage,requiring more computational resources for the bond force evaluation and damage evolution.Herein,the OpenMP parallel optimization of the rate-dependent peridynamic ceramicmodel is investigated.Also,themodules that compute the interactions betweenmaterial points and update damage index are vectorized and parallelized.Moreover,the numerical examples are carried out to simulate the dynamic response and fracture of the ceramic plate under normal impact.Furthermore,the speed-up ratio and computational efficiency by multi-threads are evaluated and discussed to demonstrate the reliability of parallelized programs.The results reveal that the totalwall clock time has been significantly reduced after optimization,showing the promise of parallelization process in terms of accuracy and stability.
文摘1.Introduction Carbon neutrality has emerged as a global goal due to its pivotal role in addressing the challenges of global climate change.Before the United Nations Climate Summit was held in November 2020,124 countries promised to reach net-zero emissions[1].Solar energy is one of the important renewable energy sources that significantly curtail carbon emissions originating from fossil fuels.
基金Hunan Provincial Education Science 13th Five-Year Plan (Grant No.XJK016BXX001)Social Science Foundation of Hunan Province (Grant No.17YBA049)+1 种基金Open Foundation for the University Innovation Platform in the HunanProvince, grant number 16K013. This research work is implemented at the 2011Collaborative Innovation Center for Development and Utilization of Finance andEconomics Big Data Property, Universities of Hunan Province. Open project (Grant Nos.20181901CRP03, 20181901CRP04, 20181901CRP05)National Social Science Fund Project: Research on the Impact Mechanism of China’sCapital Space Flow on Regional Economic Development (Project No. 14BJL086).
文摘Due to the huge amount of increasing data, the requirements of people forelectronic products such as mobile phones, tablets, and notebooks are constantlyimproving. The development and design of various software applications attach greatimportance to users’ experiences. The rationalized UI design should allow a user not onlyenjoy the visual design experience of the new product but also operating it morepleasingly. This process is to enhance the attractiveness and performance of the newproduct and thus to promote the active usage and consuming conduct of users. In thispaper, an UI design optimization strategy for general APP in the big data environment isproposed to get better user experience while effectively obtaining information. Anexperimental example of a library APP is designed to optimize the user experience. Theexperimental results show that the user-centered UI design is the core of optimization,and user portrait based on big data platforms is the key to UI design.