Wastewater from the spray absorption treatment of sludge drying gas is a kind of refractory wastewater with poor biodegradability.In this study,the free radicals generated from the double dielectric barrier were innov...Wastewater from the spray absorption treatment of sludge drying gas is a kind of refractory wastewater with poor biodegradability.In this study,the free radicals generated from the double dielectric barrier were innovatively used for the degradation of simulated spray wastewater.The effects of residence time,input power,initial pH,aeration rate,and discharge area on the degradation rate and COD(chemical oxygen demand)removal rate were investigated.The optimal conditions were as follows:residence time=120 min,input power=170.0 W,initial pH=5.54,aeration rate=0.9 mL/min,discharge area=10.8 cm^(2),and the initial concentrations of NH_(3),H_(2)S,methanethiol,trimethylamine,benzene and toluene were 250,250,50,50,50 and 100 mg/L,respectively.Meanwhile,it was also found that hydroxyl radical(⋅OH)played an important role in the degradation process.展开更多
The coal-fired flue gas spraying wastewater is a kind of refractory mixed wastewater with poor biodegradability.In this study,the degradation of model coal-fired flue gas spraying wastewater was studied by using disch...The coal-fired flue gas spraying wastewater is a kind of refractory mixed wastewater with poor biodegradability.In this study,the degradation of model coal-fired flue gas spraying wastewater was studied by using discharge free radicals produced by double-dielectric barrier discharge.The degradation rate of pollutants,chemical oxygen demand removal rate and other indicators were detected,and the influence of different conditions on the degradation effect was analyzed.The optimal parameters are as follows:residence time 120 min,input power 170.0 W,initial pH value 3.79,and aeration rate 1.8 mL/min.The initial concentrations of acetone,formaldehyde,chloroform,benzene and toluene were 100,100,100,and 100 mg/L,respectively.Furthermore,it is proved that the discharge area is independent of the degradation rate.Through the analysis of the mechanism,it is found that·OH is an important factor affecting the degradation rate of pollutants in model coal-fired flue gas spraying wastewater.展开更多
基金supported by the National Natural Science Foundation of China(No.61871409)Zhejiang Natural Science Foundation of China(No.LZ20F010001).
文摘Wastewater from the spray absorption treatment of sludge drying gas is a kind of refractory wastewater with poor biodegradability.In this study,the free radicals generated from the double dielectric barrier were innovatively used for the degradation of simulated spray wastewater.The effects of residence time,input power,initial pH,aeration rate,and discharge area on the degradation rate and COD(chemical oxygen demand)removal rate were investigated.The optimal conditions were as follows:residence time=120 min,input power=170.0 W,initial pH=5.54,aeration rate=0.9 mL/min,discharge area=10.8 cm^(2),and the initial concentrations of NH_(3),H_(2)S,methanethiol,trimethylamine,benzene and toluene were 250,250,50,50,50 and 100 mg/L,respectively.Meanwhile,it was also found that hydroxyl radical(⋅OH)played an important role in the degradation process.
基金supported by enterprise projects(No.YT2017,No.YG1908).
文摘The coal-fired flue gas spraying wastewater is a kind of refractory mixed wastewater with poor biodegradability.In this study,the degradation of model coal-fired flue gas spraying wastewater was studied by using discharge free radicals produced by double-dielectric barrier discharge.The degradation rate of pollutants,chemical oxygen demand removal rate and other indicators were detected,and the influence of different conditions on the degradation effect was analyzed.The optimal parameters are as follows:residence time 120 min,input power 170.0 W,initial pH value 3.79,and aeration rate 1.8 mL/min.The initial concentrations of acetone,formaldehyde,chloroform,benzene and toluene were 100,100,100,and 100 mg/L,respectively.Furthermore,it is proved that the discharge area is independent of the degradation rate.Through the analysis of the mechanism,it is found that·OH is an important factor affecting the degradation rate of pollutants in model coal-fired flue gas spraying wastewater.
