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Optimization of the prompt fission neutron spectra of ^(239)Pu(n,f)via criticality benchmarking
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作者 Jia-Hao Chen Bo Yang +5 位作者 Qing-Gang Jia Rui Li Wen-Di Chen hai-rui guo Wei-Li Sun Tao Ye 《Nuclear Science and Techniques》 2025年第9期139-149,共11页
Prompt fission neutron spectra(PFNS)have a significant role in nuclear science and technology.In this study,the PFNS for^(239)Pu are evaluated using both differential and integral experimental data.A method that lever... Prompt fission neutron spectra(PFNS)have a significant role in nuclear science and technology.In this study,the PFNS for^(239)Pu are evaluated using both differential and integral experimental data.A method that leverages integral criticality benchmark experiments to constrain the PFNS data is introduced.The measured central values of the PFNS are perturbed by constructing a covariance matrix.The PFNS are sampled using two types of covariance matrices,either generated with an assumed correlation matrix and incorporating experimental uncertainties or derived directly from experimental reports.The joint Monte Carlo transport code is employed to perform transport simulations on five criticality benchmark assemblies by utilizing perturbed PFNS data.Extensive simulations result in an optimized PFNS that shows improved agreement with the integral criticality benchmark experiments.This study introduces a novel approach for optimizing differential experimental data through integral experiments,particularly when a covariance matrix is not provided. 展开更多
关键词 Prompt fission neutron spectra Differential nuclear data Criticality benchmark Random sample Transport simulation
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Study of ^(6)Li+^(7)Li anomalous large-angle scattering
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作者 Zhi-Hao Sun Hao-Yang Fan +9 位作者 Yi-Ting E hai-rui guo Tao Ye Wei-Li Sun Xu Han Wen-Di Chen Yang-Jun Ying Yong-Li Xu Dong-Hong Zhang Yin-Lu Han 《Nuclear Science and Techniques》 2025年第8期211-221,共11页
This study investigates the mechanism of ^(6)Li+^(7)Li anomalous large-angle scattering.First,elastic scattering is analyzed using an optical model with the São Paulo potential,and inelastic scattering to the fir... This study investigates the mechanism of ^(6)Li+^(7)Li anomalous large-angle scattering.First,elastic scattering is analyzed using an optical model with the São Paulo potential,and inelastic scattering to the first excited state of ^(7)Li is analyzed by distorted wave born approximation method.The experimental data of the elastic scattering angular distributions could be described reasonably well by the optical model at forward angles;however,anomalous large-angle scattering is observed in the angular distributions of both the elastic and inelastic channels for all measured energies.Elastic and inelastic scatterings are investigated using the coupled reaction channel method.The elastic and inelastic scattering,transfer reactions for the ground and excited states,and their coupling effects are considered in the coupled reaction channel scheme.In addition,the influence of the breakup effects of the weakly bound ^(6)Li and ^(7)Li is investigated by including three resonance states of ^(6)Li and two resonance states of ^(7)Li in the coupled reaction channel framework.The observed anomalous large-angle scattering is explained using the transfer reaction mechanism and breakup effect,and the calculated results reproduce the experimental data reasonably well. 展开更多
关键词 Anomalous large-angle scattering Coupled reaction channel Transfer reaction Breakup effect
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Theoretical analysis of the double-differential cross-sections of neutron,proton,deuteron,^(3)He,andαfor the p+^(6) Li reaction
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作者 Fang-Lei Zou Xiao-Jun Sun +10 位作者 Jing-Shang Zhang hai-rui guo Yin-Lu Han Rui-Rui Xu Xi Tao Ji-Min Wang Xiao-Dong Sun Yuan Tian Tao Ye Yong-Li Xu Chun-Tian Liang 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第3期181-197,共17页
Based on the unified Hauser–Feshbach and exciton model,which can describe the particle emission processes between discrete energy levels with energy,angular momentum,and parity conservations,a statistical theory of l... Based on the unified Hauser–Feshbach and exciton model,which can describe the particle emission processes between discrete energy levels with energy,angular momentum,and parity conservations,a statistical theory of light nucleus reaction(STLN)is developed to calculate the double-differential cross-sections of the outgoing neutron and light charged particles for the proton-induced^(6) Li reaction.A significant difference is observed between the p+^(6) Li and p+^(7) Li reactions owing to the discrepancies in the energy-level structures of the targets.The reaction channels,including sequential and simultaneous emission processes,are analyzed in detail.Taking the double-differential cross-sections of the outgoing proton as an example,the influence of contaminations(such as^(1) H,^(7)Li,^(12)C,and^(16)O)on the target is identified in terms of the kinetic energy of the first emitted particles.The optical potential parameters of the proton are obtained by fitting the elastic scattering differential cross-sections.The calculated total double-differential cross-sections of the outgoing proton and deuteron at E_(p)=14 MeV agree well with the experimental data for different outgoing angles.Simultaneously,the mixed double differential cross-sections of^(3) He andαare in good agreement with the measurements.The agreement between the measured data and calculated results indicates that the two-body and three-body breakup reactions need to be considered,and the pre-equilibrium reaction mechanism dominates the reaction processes.Based on the STLN model,a PLUNF code for the p+^(6) Li reaction is developed to obtain an ENDF-6-formatted file of the double-differential cross-sections of the nucleon and light composite charged particles. 展开更多
关键词 Statistical theory of light nucleus reaction p+^(6)Li reaction Light composite charged particle Double-differential cross-sections Two-body breakup Three-body breakup
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Correction to:Theoretical analysis of the double-differential cross-sections of neutron,proton,deuteron,^(3)He,and α for the p+^(6)Li reaction
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作者 Fang-Lei Zou Xiao-Jun Sun +10 位作者 Jing-Shang Zhang hai-rui guo Yin-Lu Han Rui-Rui Xu Xi Tao Ji-Min Wang Xiao-Dong Sun Yuan Tian Tao Ye Yong-Li Xu Chun-Tian Liang 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2024年第11期139-139,共1页
Correction to:Nuclear Science and Techniques(2024)35:61 https://doi.org/10.1007/s41365-024-01421-5 In this article,the figures were wrongly numbered.The Fig.7 and 8 should have been Fig.11 and 12.The Fig.9,10,11,and 1... Correction to:Nuclear Science and Techniques(2024)35:61 https://doi.org/10.1007/s41365-024-01421-5 In this article,the figures were wrongly numbered.The Fig.7 and 8 should have been Fig.11 and 12.The Fig.9,10,11,and 12 should have been 7,8,9 and 10.The original article has been corrected. 展开更多
关键词 corrected double differential
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Ho^(3+)和Yb^(3+)共掺杂La_(7)P_(3)O_(18)荧光粉的合成及上转换发光性能 被引量:1
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作者 朱浩天 郭海瑞 +4 位作者 郑启泾 官春艳 朱莉萍 李海斌 杨锦瑜 《Transactions of Nonferrous Metals Society of China》 SCIE EI CAS CSCD 2023年第4期1205-1213,共9页
通过高温固相技术合成Ho^(3+)和Yb^(3+)共掺杂La_(7)P_(3)O_(18)上转换荧光粉。XRD结果表明,合成样品是空间群为P21/n的单斜结构的La_(7)P_(3)O_(18)晶体和少量La PO4晶体的混合物。紫外可见漫反射光谱结果证实La_(7)P_(3)O_(18)晶体是... 通过高温固相技术合成Ho^(3+)和Yb^(3+)共掺杂La_(7)P_(3)O_(18)上转换荧光粉。XRD结果表明,合成样品是空间群为P21/n的单斜结构的La_(7)P_(3)O_(18)晶体和少量La PO4晶体的混合物。紫外可见漫反射光谱结果证实La_(7)P_(3)O_(18)晶体是一种光学带隙为4.10 e V的间接半导体。经980 nm激光激发,Ho^(3+)和Yb^(3+)共掺杂La_(7)P_(3)O_(18)荧光粉发射出Ho^(3+)离子特征的蓝色(486 nm)、绿色(550 nm)和红色(661 nm)特征峰,其中,661 nm处发射峰在样品上转换发光光谱中占主导地位。此外,随着Ho^(3+)和Yb^(3+)掺杂量的增加,样品上转换发光强度先增大后减小。当Ho^(3+)和Yb^(3+)的掺杂量分别达到1%和10%(摩尔分数)时,样品出现浓度猝灭现象,其机制为电四极-电四极相互作用。泵浦功率和发光强度关系表明,样品的绿光和红光发射均源于双光子吸收过程激发。Ho^(3+)和Yb^(3+)共掺杂La_(7)P_(3)O_(18)晶体上转换发光色坐标位于橙红色区域。 展开更多
关键词 La_(7)P_(3)O_(18) Ho^(3+) Yb^(3+) 上转换发光
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Measurement of the ^(232)Th(n,f)cross section in the 1-200 MeV range at the CSNS Back-n 被引量:5
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作者 Zhi-Zhou Ren Yi-Wei Yang +77 位作者 Yong-Hao Chen Rong Liu Bang-Jiao Ye Jie Wen hai-rui guo Zi-Jie Han Qi-Ping Chen Zhong-Wei Wen Wei-Li Sun Han Yi Xing-Yan Liu Tao Ye Jiang-Bo Bai Qi An Jie Bao Yu Bao Ping Cao Hao-Lei Chen Zhen Chen Zeng-Qi Cui Rui-Rui Fan Chang-Qing Feng Ke-Qing Gao Xiao-Long Gao Min-Hao Gu Chang-Cai Han guo-Zhu He Yong-Cheng He Yang Hong Yi-Wei Hu Han-Xiong Huang Xi-Ru Huang Hao-Yu Jiang Wei Jiang Zhi-Jie Jiang Han-Tao Jing Ling Kang Bo Li Chao Li Jia-Wen Li Qiang Li Xiao Li Yang Li Jie Liu Shu-Bin Liu Ze Long Guang-Yuan Luan Chang-Jun Ning Meng-Chen Niu Bin-Bin Qi Jie Ren Xi-Chao Ruan Zhao-Hui Song Kang Sun Zhi-Jia Sun Zhi-Xin Tan Jing-Yu Tang Xin-Yi Tang Bin-Bin Tian Li-Jiao Wang Peng-Cheng Wang Zhao-Hui Wang Xiao-Guang Wu Xuan Wu Li-Kun Xie Xiao-Yun Yang Li Yu Tao Yu Yong-Ji Yu guo-Hui Zhang Lin-Hao Zhang Qi-Wei Zhang Xian-Peng Zhang Yu-Liang Zhang Zhi-Yong Zhang Lu-Ping Zhou Zhi-Hao Zhou Ke-Jun Zhu 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2023年第8期142-153,共12页
The ^(232)Th(n,f)cross section is very important in basic nuclear physics and applications based on the Th/U fuel cycle.Using the time-of-flight method and a multi-cell fast-fission ionization chamber,a novel measurem... The ^(232)Th(n,f)cross section is very important in basic nuclear physics and applications based on the Th/U fuel cycle.Using the time-of-flight method and a multi-cell fast-fission ionization chamber,a novel measurement of the^(232)Th(n,f)cross sec-tion relative to^(235)U in the 1–200 MeV range was performed at the China Spallation Neutron Source Back-n white neutron source(Back-n).The fission event-neutron energy spectra of^(232)Th and^(235)U fission cells were measured in the single-bunch mode.Corrected 232Th/235U fission cross-sectional ratios were obtained,and the measurement uncertainties were 2.5–3.7%for energies in the 2–20 MeV range and 3.6–6.2%for energies in the 20–200 MeV range.The^(232)Th(n,f)cross section was obtained by introducing the standard cross section of^(235)U(n,f).The results were compared with those of previous theoreti-cal calculations,measurements,and evaluations.The measured 232Th fission cross section agreed with the main evaluation results in terms of the experimental uncertainty,and 232Th fission resonances were observed in the 1–3 MeV range.The present results provide^(232)Th(n,f)cross-sectional data for the evaluation and design of Th/U cycle nuclear systems. 展开更多
关键词 232Th(n f)cross section Fast-fission ionization chamber Back-n white neutron source
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Theoretical calculation and evaluation of n +^(240,242,244)Pu reactions 被引量:3
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作者 hai-rui guo Yin-Lu Han Chong-Hai Cai 《Nuclear Science and Techniques》 SCIE CAS CSCD 2019年第1期79-88,共10页
The nuclear data of n+^(240;242;244)Pu reactions for incident energy below 200 MeV are calculated and evaluated to meet the requirement in the design of an accelerator-driven subcritical system. The optical model is u... The nuclear data of n+^(240;242;244)Pu reactions for incident energy below 200 MeV are calculated and evaluated to meet the requirement in the design of an accelerator-driven subcritical system. The optical model is used to calculate the total, nonelastic, shape elastic cross sections, shape elastic scattering angular distributions, and transmission coefficients. The distorted-wave Born approximation is applied to calculate the direct inelastic scatterings to the discrete excited states. The nuclear reaction statistical models and fission theory are applied to describe neutron, proton, deuteron, triton, helium-3, alpha and c emissions, and fission consistently. The results thus obtained are compared with experimental data and the evaluated data obtained from ENDF/B-VII.1 and JENDL-4.0. 展开更多
关键词 n+240 242 244pu REACTIONS THEORETICAL calculation of NUCLEAR reaction NUCLEAR data for E≤200 MEV
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Favorable surface reconstruction with strong reducibility on the high-entropy sulfide for efficient electrochemical oxidation of 5-hydroxymethylfurfural at high concentrations
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作者 Yu-Ting Fang hai-rui guo +3 位作者 Gui-Cai Lv Cheng Wang Meng-Meng Zhen Hui-Ling Liu 《Rare Metals》 2025年第10期7404-7417,共14页
Electrochemical oxidation of 5-hydroxymethylfurfural(HMFOR),featuring favorable thermodynamics,presents a promising alternative to the conventional oxygen evolution reaction for energy-saving hydrogen(H_(2))production... Electrochemical oxidation of 5-hydroxymethylfurfural(HMFOR),featuring favorable thermodynamics,presents a promising alternative to the conventional oxygen evolution reaction for energy-saving hydrogen(H_(2))production coupled with biomass upgrading.However,the multiple proton-coupled electron transfer steps in HMFOR result in sluggish kinetics,highlighting the development of highly efficient electrocatalysts.Herein,a high-entropy amorphous MoCrCoNiZn-S grown on nickel foam(HEAS@NF)is constructed via a metal organic framework-derived strategy to efficiently convert HMF to 2,5-furandicarboxylic acid(FDCA).The abundant active sites on the HEAS@NF facilitate the structural evolution to oxyhydroxides that possess strong reducibility for HMF dehydrogenation,leading to superior HMFOR performance compared to sulfides with fewer metal elements.In situ electrochemical impedance spectroscopy results confirm significantly favored kinetics to HMFOR over OER on the HEAS@NF,resulting in a remarkable98%HMF conversion,with FDCA yield and Faradaic efficiency of 98%and 94%even at a concentrated 100 mM HMF.A two-electrode flow electrolyzer equipped with the bifunctional HEAS@NF enables simultaneous cathodic H2and anodic FDCA production with an electricity saving of 10.8%.This study presents an effective strategy to inspire the exploration of high-entropy catalysts for biomass-assisted H2production. 展开更多
关键词 High-entropy sulfide H_(2)production 5-Hydroxymethylfurfural oxidation Biomass upgrading Electrocatalysis
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Applicability of 9Be global optical potential to reactions of 7,10,11,12Be
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作者 Yong-Li Xu Yin-Lu Han +3 位作者 Hai-Ying Liang Zhen-Dong Wu hai-rui guo Chong-Hai Cai 《Chinese Physics C》 SCIE CAS CSCD 2019年第9期55-61,共7页
Elastic scattering angular distributions and total reaction cross-sections of 7,10,11,12Be projectiles are predicted by the systematic 9Be global phenomenological optical model potential for target mass numbers rangin... Elastic scattering angular distributions and total reaction cross-sections of 7,10,11,12Be projectiles are predicted by the systematic 9Be global phenomenological optical model potential for target mass numbers ranging from 24 to 209.These predictions provide a detailed analysis by their comparison with the available experimental data.Furthermore,these elastic scattering observables are also predicted for some targets out of the mass number range.The results are in reasonable agreement with the existing experimental data,and they are presented in this study. 展开更多
关键词 global PHENOMENOLOGICAL optical model potential elastic scattering ANGULAR DISTRIBUTIONS total reaction cross SECTIONS
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Microscopic study of 7Li-nucleus potential
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作者 Wen-Di Chen hai-rui guo +4 位作者 Wei-Li Sun Tao Ye Yang-Jun Ying Yin-Lu Han Qing-Biao Shen 《Chinese Physics C》 SCIE CAS CSCD 2020年第5期106-113,共8页
A microscopic approach is employed to study the optical potential for the 7Li-nucleus interaction system without any free parameters.It is obtained by folding the microscopic optical potentials of the constituent nucl... A microscopic approach is employed to study the optical potential for the 7Li-nucleus interaction system without any free parameters.It is obtained by folding the microscopic optical potentials of the constituent nucleons of 7Li over their density distributions.We employ an isospin-dependent nucleon microscopic optical potential,which is based on the Skyrme nucleon-nucleon effective interaction and derived using the Green's function method,as the nucleon optical potential.The harmonic oscillator shell model is used to describe the internal wave function of 7Li and obtain the nucleon density distribution.The 7Li microscopic optical potential is used to predict the reaction cross-sections and elastic scattering angular distributions for the target range from 27Al to 208Pb and energy range below 450 MeV.Generally,the results can reproduce the measured data reasonably well.In addition,the microscopic optical potential is comparable to a global phenomenological optical potential by fitting the presently existing measured data. 展开更多
关键词 7 LI MICROSCOPIC optical POTENTIAL 7 LI ELASTIC scattering FOLDING model
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Double differential cross sections of light charged particle production for the n+^238U reaction
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作者 hai-rui guo Yin-Lu Han Chong-Hai Cai 《Chinese Physics C》 SCIE CAS CSCD 2018年第12期90-99,共10页
Production of light complex particles from the n+^238u reaction is analyzed with the exciton model including the improved Iwamoto-Harada pickup mechanism for the preequilibrium process. It is allowed that some of the... Production of light complex particles from the n+^238u reaction is analyzed with the exciton model including the improved Iwamoto-Harada pickup mechanism for the preequilibrium process. It is allowed that some of the nucleons forming the complex ejectile come from levels below the Fermi energy, and the intrinsic structure of the emitted particle is taken into account. The equilibrium-state emissions are also considered by using Hauser- Feshbach theory with the width fluctuation correction and the evaporation model angular distributions, energy spectra and double differential cross sections of neutron, alpha emissions for the n+^238U reaction are consistently calculated and analyzed with the energy range En ≤150 MeV. ENDF-formatted nuclear data including information charged particles are obtained. Moreover, all cross sections, proton, deuteron, triton and nuclear theoretical models in about the production of light 展开更多
关键词 light charged particle production nuclear reaction theoretical model n+^238U reaction nuclear data at En≤ 150 MeV
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Description of elastic scattering induced by the unstable nuclei^(9,10,11,13,14)C
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作者 Yong-Li Xu Yin-Lu Han +4 位作者 Xin-Wu Su Xiao-Jun Sun Hai-Ying Liang hai-rui guo Chong-Hai Cai 《Chinese Physics C》 SCIE CAS CSCD 2021年第11期122-127,共6页
The elastic-scattering angular distributions and total reaction cross sections of ^(9,10,11,13,14)C projectiles were predicted using the obtained ^(12)C and ^(9)Be global optical model potentials,respectively.The pred... The elastic-scattering angular distributions and total reaction cross sections of ^(9,10,11,13,14)C projectiles were predicted using the obtained ^(12)C and ^(9)Be global optical model potentials,respectively.The predictions were analyzed in detail by comparison with the available experimental data.The results indicate that the ^(12)C and ^(9)Be global optical model potentials provide a satisfactory description of the elastic scattering data for the reactions induced by the ^(9,10,11,13)C.For the neutron-rich carbon isotope ^(14)C,the elastic scattering can be well described by changing the real part radius parameter of the ^(12)C global optical model potential.Possible physical explanations for the observed differences are further discussed. 展开更多
关键词 optical model potential elastic-scattering angular distribution reaction cross section
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Global optical model potential describing 12C-nucleus elastic scattering
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作者 Yong-Li Xu Yin-Lu Han +4 位作者 Xin-Wu Su Xiao-Jun Sun Hai-Ying Liang hai-rui guo Chong-Hai Cai 《Chinese Physics C》 SCIE CAS CSCD 2020年第12期123-132,共10页
We construct a new global optical model potential to describe the elastic scattering of 12C.The experimental data of elastic-scattering angular distributions and total reaction cross sections for targets from 24Mg to ... We construct a new global optical model potential to describe the elastic scattering of 12C.The experimental data of elastic-scattering angular distributions and total reaction cross sections for targets from 24Mg to 209Bi are considered below 200 MeV within the framework of the optical model.The results calculated using the derived global optical potential are then compared with the existing experimental data.The reliability of the global optical potential is further tested by predicting the elastic scattering data out of the mass and energy ranges,within which the global potential parameters are determined,and reasonable results are also obtained. 展开更多
关键词 optical model potential elastic-scattering angular distribution reaction cross section
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Applicability of 9Be global optical potential to description of 8,10,11B elastic scattering
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作者 Yong-Li Xu Yin-Lu Han +3 位作者 Hai-Ying Liang Zhen-Dong Wu hai-rui guo Chong-Hai Cai 《Chinese Physics C》 SCIE CAS CSCD 2020年第3期65-72,共8页
We achieved a set of 9Be global phenomenological optical model potentials by fitting a large experimental dataset of the elastic scattering observable for target mass numbers from 24 to 209.The obtained 9Be global opt... We achieved a set of 9Be global phenomenological optical model potentials by fitting a large experimental dataset of the elastic scattering observable for target mass numbers from 24 to 209.The obtained 9Be global optical model potential was applied to predict elastic-scattering angular distributions and total reaction cross-sections of 8,10,11B projectiles.The predictions are made by performing a detailed analysis comparing with the available experimental data.Furthermore,these elastic scattering observables are also predicted for some lighter targets outside of the given mass number range,and reasonable results are obtained.Possible physical explanations for the observed differences are also discussed. 展开更多
关键词 optical model potential elastic-scattering angular distribution total reaction cross section
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