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铵根插层二硫化钼的电催化析氢性能研究 被引量:1
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作者 费成玮 古莉娜 《化工新型材料》 CAS CSCD 北大核心 2019年第S01期124-128,133,共6页
通过简单的水热法,制备了一种铵根插层的MoS2纳米电催化剂。通过铵根插层后,MoS2的层间距增大,使催化活性位点密度增加,促进了电荷转移,并表现出优异的电催化析氢反应活性。电化学测试结果表明,添加适量(3mL)氨水所合成的铵根插层MoS2... 通过简单的水热法,制备了一种铵根插层的MoS2纳米电催化剂。通过铵根插层后,MoS2的层间距增大,使催化活性位点密度增加,促进了电荷转移,并表现出优异的电催化析氢反应活性。电化学测试结果表明,添加适量(3mL)氨水所合成的铵根插层MoS2具有优异的电催化析氢性能,在-10mA/cm^2处的过电位由纯MoS2的388mV降至278mV,塔菲尔斜率也由118mV/dec降至62mV/dec,电催化析氢性能明显提升。此外,铵根插层也可以改善MoS2催化剂的电化学制氢稳定性。 展开更多
关键词 二硫化钼 水热法 电催化 析氢反应 铵根插层
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Distributed Collaborative Response Surface Method for Mechanical Dynamic Assembly Reliability Design 被引量:24
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作者 BAI Guangchen fei chengwei 《Chinese Journal of Mechanical Engineering》 SCIE EI CAS CSCD 2013年第6期1160-1168,共9页
Because of the randomness of many impact factors influencing the dynamic assembly relationship of complex machinery, the reliability analysis of dynamic assembly relationship needs to be accomplished considering the r... Because of the randomness of many impact factors influencing the dynamic assembly relationship of complex machinery, the reliability analysis of dynamic assembly relationship needs to be accomplished considering the randomness from a probabilistic perspective. To improve the accuracy and efficiency of dynamic assembly relationship reliability analysis, the mechanical dynamic assembly reliability(MDAR) theory and a distributed collaborative response surface method(DCRSM) are proposed. The mathematic model of DCRSM is established based on the quadratic response surface function, and verified by the assembly relationship reliability analysis of aeroengine high pressure turbine(HPT) blade-tip radial running clearance(BTRRC). Through the comparison of the DCRSM, traditional response surface method(RSM) and Monte Carlo Method(MCM), the results show that the DCRSM is not able to accomplish the computational task which is impossible for the other methods when the number of simulation is more than 100 000 times, but also the computational precision for the DCRSM is basically consistent with the MCM and improved by 0.40-4.63% to the RSM, furthermore, the computational efficiency of DCRSM is up to about 188 times of the MCM and 55 times of the RSM under 10000 times simulations. The DCRSM is demonstrated to be a feasible and effective approach for markedly improving the computational efficiency and accuracy of MDAR analysis. Thus, the proposed research provides the promising theory and method for the MDAR design and optimization, and opens a novel research direction of probabilistic analysis for developing the high-performance and high-reliability of aeroengine. 展开更多
关键词 machinery dynamic assembly reliability analysis distributed collaborative response surface method blade-tip radial running clearance
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Advanced multiple response surface method of sensitivity analysis for turbine blisk reliability with multi-physics coupling 被引量:7
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作者 Zhang Chunyi Song Lukai +2 位作者 fei chengwei Lu Cheng Xie Yongmei 《Chinese Journal of Aeronautics》 SCIE EI CAS CSCD 2016年第4期962-971,共10页
To reasonably implement the reliability analysis and describe the significance of influencing parameters for the multi-failure modes of turbine blisk, advanced multiple response surface method (AMRSM) was proposed for... To reasonably implement the reliability analysis and describe the significance of influencing parameters for the multi-failure modes of turbine blisk, advanced multiple response surface method (AMRSM) was proposed for multi-failure mode sensitivity analysis for reliability. The mathematical model of AMRSM was established and the basic principle of multi-failure mode sensitivity analysis for reliability with AMRSM was given. The important parameters of turbine blisk failures are obtained by the multi-failure mode sensitivity analysis of turbine blisk. Through the reliability sensitivity analyses of multiple failure modes (deformation, stress and strain) with the proposed method considering fluid-thermal-solid interaction, it is shown that the comprehensive reliability of turbine blisk is 0.9931 when the allowable deformation, stress and strain are 3.7 x 10(-3) m, 1.0023 x 10(9) Pa and 1.05 x 10(-2) m/m, respectively; the main impact factors of turbine blisk failure are gas velocity, gas temperature and rotational speed. As demonstrated in the comparison of methods (Monte Carlo (MC) method, traditional response surface method (RSM), multiple response surface method (MRSM) and AMRSM), the proposed AMRSM improves computational efficiency with acceptable computational accuracy. The efforts of this study provide the AMRSM with high precision and efficiency for multi-failure mode reliability analysis, and offer a useful insight for the reliability optimization design of multi-failure mode structure. (C) 2016 Chinese Society of Aeronautics and Astronautics. Production and hosting by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license. 展开更多
关键词 Advanced multiple response surface method Artificial neural network Intelligent algorithm Multi-failure mode Reliability analysis Turbine blisk
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