Although traditional soft magnetic materials have been investigated to improve triboelectric nanogenerator(TENG)performance,their electrical output performance remains insufficient.Magnetic high-entropy alloys(HEAs),a...Although traditional soft magnetic materials have been investigated to improve triboelectric nanogenerator(TENG)performance,their electrical output performance remains insufficient.Magnetic high-entropy alloys(HEAs),a new type of magnetic functional material,possess excellent mechanical and magnetic properties.However,the electrical characteristics of TENGs based on magnetic HEAs remain unexplored.Therefore,a TENG based on polyvinylidene fluoride/HEA-polyamide 66(PHP-TENG)is proposed in this study.The coupling of displacement current from the polarization field and magnetization current generated by time-varying electric-field magnetization of magnetic HEAs can improve the electrical characteristics of TENGs.The maximum voltage,current,and power density of the PHP-TENG are 156.34 V,1.56μA,and 188.40 mW·m^(−2),respectively.PHP-TENG maintains a stable current output even after 20,000 cycles.Furthermore,it can power a 47μF commercial capacitor to 2.5 V in 70 s and propel a hygrometer to function normally.In addition,PHP-TENG exhibits satisfactory sensitivity to humidity.These results indicate that TENGs based on magnetic HEAs exhibit potential for high-efficiency energy-collecting devices.展开更多
基金supported by the National Natural Science Foundation of China(No.52273077)the State Key Laboratory of Bio-Fibers&Eco-Textiles,Qingdao University(Nos.ZDKT202108 and G2RC202022).
文摘Although traditional soft magnetic materials have been investigated to improve triboelectric nanogenerator(TENG)performance,their electrical output performance remains insufficient.Magnetic high-entropy alloys(HEAs),a new type of magnetic functional material,possess excellent mechanical and magnetic properties.However,the electrical characteristics of TENGs based on magnetic HEAs remain unexplored.Therefore,a TENG based on polyvinylidene fluoride/HEA-polyamide 66(PHP-TENG)is proposed in this study.The coupling of displacement current from the polarization field and magnetization current generated by time-varying electric-field magnetization of magnetic HEAs can improve the electrical characteristics of TENGs.The maximum voltage,current,and power density of the PHP-TENG are 156.34 V,1.56μA,and 188.40 mW·m^(−2),respectively.PHP-TENG maintains a stable current output even after 20,000 cycles.Furthermore,it can power a 47μF commercial capacitor to 2.5 V in 70 s and propel a hygrometer to function normally.In addition,PHP-TENG exhibits satisfactory sensitivity to humidity.These results indicate that TENGs based on magnetic HEAs exhibit potential for high-efficiency energy-collecting devices.
