A range of partial top full bottom electrodes are used to explore the use of bi-polar Polarisation-Electricfield(PeE)measurements to quantify recoverable energy(Wrec),energy loss(W_(loss))and the efficiency(h)of ferro...A range of partial top full bottom electrodes are used to explore the use of bi-polar Polarisation-Electricfield(PeE)measurements to quantify recoverable energy(Wrec),energy loss(W_(loss))and the efficiency(h)of ferroelectric BaTiO_(3)ceramics.The values obtained are dependent on the ratio of sample thickness(S)and top contact radius(r).With increasing S/r from 0.17 to 1.96 the P-E responses become increasingly distorted and broader.Measurements show Wrec increases by a factor of~1.4 but Wloss increases by a factor of~7 with h decreasing from~29%to 8%.Finite element modelling was used to simulate the experimental set-up of the sample/electrode arrangements using the Jiles-Atherton model to replicate the ferroelectric behaviour of BaTiO_(3).These models demonstrate the experimentally applied electricfield using a simple geometric correction for sample thickness is an underestimation of the actualfield experienced by the material under the top contact at high S/r values.We stress the importance of reporting the contact sizes and thicknesses of samples when using PeE measurements to assess Wrec,W_(loss)andηin non-linear dielectric materials.This will allow a fairer comparison of performances between various types of materials being considered for high-energy-density ceramic capacitors.展开更多
The editorial office regrets that mistakes occurred during the presentation of Figs.1 and 4.Specifically,a typographic error in Figs.1 and 4 was mistakenly taken from a different article.The editorial office would lik...The editorial office regrets that mistakes occurred during the presentation of Figs.1 and 4.Specifically,a typographic error in Figs.1 and 4 was mistakenly taken from a different article.The editorial office would like to apologise for any inconvenience caused,and the corrected figures are pending as below.展开更多
基金the EPSRC funding to support this work through a CASE conversion DTP grant EP/T517835/1.
文摘A range of partial top full bottom electrodes are used to explore the use of bi-polar Polarisation-Electricfield(PeE)measurements to quantify recoverable energy(Wrec),energy loss(W_(loss))and the efficiency(h)of ferroelectric BaTiO_(3)ceramics.The values obtained are dependent on the ratio of sample thickness(S)and top contact radius(r).With increasing S/r from 0.17 to 1.96 the P-E responses become increasingly distorted and broader.Measurements show Wrec increases by a factor of~1.4 but Wloss increases by a factor of~7 with h decreasing from~29%to 8%.Finite element modelling was used to simulate the experimental set-up of the sample/electrode arrangements using the Jiles-Atherton model to replicate the ferroelectric behaviour of BaTiO_(3).These models demonstrate the experimentally applied electricfield using a simple geometric correction for sample thickness is an underestimation of the actualfield experienced by the material under the top contact at high S/r values.We stress the importance of reporting the contact sizes and thicknesses of samples when using PeE measurements to assess Wrec,W_(loss)andηin non-linear dielectric materials.This will allow a fairer comparison of performances between various types of materials being considered for high-energy-density ceramic capacitors.
文摘The editorial office regrets that mistakes occurred during the presentation of Figs.1 and 4.Specifically,a typographic error in Figs.1 and 4 was mistakenly taken from a different article.The editorial office would like to apologise for any inconvenience caused,and the corrected figures are pending as below.
