UV-pulsed laser cavity ringdown spectroscopy of the hydroxyl radical OH(A–X)(0–0)band in the wavelength range of 306–310 nm was employed to determine absolute number densities of OH in the atmospheric helium plasma...UV-pulsed laser cavity ringdown spectroscopy of the hydroxyl radical OH(A–X)(0–0)band in the wavelength range of 306–310 nm was employed to determine absolute number densities of OH in the atmospheric helium plasma jets generated by a 2.45 GHz microwave plasma source.The effect of the addition of molecular gases N2 and O2 to He plasma jets on OH generation was studied.Optical emission spectroscopy was simultaneously employed to monitor reactive plasma species.Stark broadening of the hydrogen Balmer emission line(Hβ)was used to estimate the electron density ne in the jets.For both He/N2 and He/O2 jets,ne was estimated to be on the order of 10^15 cm^?3.The effects of plasma power and gas flow rate were also studied.With increase in N2 and O2 flow rates,ne tended to decrease.Gas temperature in the He/O2 plasma jets was elevated compared to the temperatures in the pure He and He/N2 plasma jets.The highest OH densities in the He/N2 and He/O2 plasma jets were determined to be 1.0×10^16 molecules/cm^3 at x=4 mm(from the jet orifice)and 1.8×10^16 molecules/cm^3 at x=3 mm,respectively.Electron impact dissociation of water and water ion dissociative recombination were the dominant reaction pathways,respectively,for OH formation within the jet column and in the downstream and far downstream regions.The presence of strong emissions of the N2^+ bands in both He/N2 and He/O2 plasma jets,as against the absence of the N2^+ emissions in the Ar plasma jets,suggests that the Penning ionization process is a key reaction channel leading to the formation of N2^+ in these He plasma jets.展开更多
Fiber loop ringdown (FLRD) has demonstrated to be capable of sensing various quantities, such as chemical species, pressure, refractive index, strain, temperature, etc.;and it has high potential for the development of...Fiber loop ringdown (FLRD) has demonstrated to be capable of sensing various quantities, such as chemical species, pressure, refractive index, strain, temperature, etc.;and it has high potential for the development of a sensor network. In the present work, we describe design and development of three different types of FLRD sensors for water, cracks, and temperature sensing in concrete structures. All of the three aforementioned sensors were indigenously developed very recently in our laboratory and their capabilities of detecting the respective quantities were demonstrated. Later, all of the sensors were installed in a test grout cube for real-time monitoring. This work presents the results obtained in the laboratory-based experiments as well as the results from the real-time monitoring process in the test cube.展开更多
A light beam,such as a laser beam,carries photons that possess both momentum and energy.When a laser beam illuminates a microscopic object,the momentum and energy of these photons can be converted into a light force,w...A light beam,such as a laser beam,carries photons that possess both momentum and energy.When a laser beam illuminates a microscopic object,the momentum and energy of these photons can be converted into a light force,which can set the object in motion or even cause it to levitate within a medium by counteracting the gravitational force.The nature of the light force depends on the properties of the object’s material.展开更多
基金supported by the National Science Foundation through the grant CBET-1066486
文摘UV-pulsed laser cavity ringdown spectroscopy of the hydroxyl radical OH(A–X)(0–0)band in the wavelength range of 306–310 nm was employed to determine absolute number densities of OH in the atmospheric helium plasma jets generated by a 2.45 GHz microwave plasma source.The effect of the addition of molecular gases N2 and O2 to He plasma jets on OH generation was studied.Optical emission spectroscopy was simultaneously employed to monitor reactive plasma species.Stark broadening of the hydrogen Balmer emission line(Hβ)was used to estimate the electron density ne in the jets.For both He/N2 and He/O2 jets,ne was estimated to be on the order of 10^15 cm^?3.The effects of plasma power and gas flow rate were also studied.With increase in N2 and O2 flow rates,ne tended to decrease.Gas temperature in the He/O2 plasma jets was elevated compared to the temperatures in the pure He and He/N2 plasma jets.The highest OH densities in the He/N2 and He/O2 plasma jets were determined to be 1.0×10^16 molecules/cm^3 at x=4 mm(from the jet orifice)and 1.8×10^16 molecules/cm^3 at x=3 mm,respectively.Electron impact dissociation of water and water ion dissociative recombination were the dominant reaction pathways,respectively,for OH formation within the jet column and in the downstream and far downstream regions.The presence of strong emissions of the N2^+ bands in both He/N2 and He/O2 plasma jets,as against the absence of the N2^+ emissions in the Ar plasma jets,suggests that the Penning ionization process is a key reaction channel leading to the formation of N2^+ in these He plasma jets.
文摘Fiber loop ringdown (FLRD) has demonstrated to be capable of sensing various quantities, such as chemical species, pressure, refractive index, strain, temperature, etc.;and it has high potential for the development of a sensor network. In the present work, we describe design and development of three different types of FLRD sensors for water, cracks, and temperature sensing in concrete structures. All of the three aforementioned sensors were indigenously developed very recently in our laboratory and their capabilities of detecting the respective quantities were demonstrated. Later, all of the sensors were installed in a test grout cube for real-time monitoring. This work presents the results obtained in the laboratory-based experiments as well as the results from the real-time monitoring process in the test cube.
基金support of the National Science Foundation,Plasma Physics Program via grant No.2308947the support of the NASA Emerging Worlds NNH22ZDA001N-EW with grant No.22-EW22-0016supported by the U.S.Department of Energy,Office of Science,Office of Fusion Energy Sciences under award number DE-SC-0021030.
文摘A light beam,such as a laser beam,carries photons that possess both momentum and energy.When a laser beam illuminates a microscopic object,the momentum and energy of these photons can be converted into a light force,which can set the object in motion or even cause it to levitate within a medium by counteracting the gravitational force.The nature of the light force depends on the properties of the object’s material.