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Investigations of key issues on the reproducibility of high-Tc superconductivity emerging from compressed La3Ni2O7 被引量:1
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作者 Yazhou Zhou Jing Guo +12 位作者 Shu Cai Hualei Sun chengyu li Jinyu Zhao Pengyu Wang Jinyu Han Xintian Chen Yongjin Chen Qi Wu Yang Ding Tao Xiang Ho-kwang Mao liling Sun 《Matter and Radiation at Extremes》 2025年第2期80-89,共10页
Signatures of superconductivity near 80 K have recently been discovered in single crystals of La_(3)Ni_(2)O_(7)under pressure,which makes it a new candidate for high-temperature superconductors dominated by 3d transit... Signatures of superconductivity near 80 K have recently been discovered in single crystals of La_(3)Ni_(2)O_(7)under pressure,which makes it a new candidate for high-temperature superconductors dominated by 3d transition elements,following the cuprate and iron-pnictide superconductors.However,there are several critical questions that have been perplexing the scientificommunity:(1)What factors contribute to the inconsistent reproducibility of the experimental results?(2)What is the fundamental nature of pressure-induced superconductivity:bulk or nonbulk(filamentary-like)(3)Where is the superconducting phase located within the sample if it is filamentary-like(4)Is the oxygen content important for the development and stabilization of superconductivity?In this study,we employ comprehensive high-pressure techniques to address these questions.Through our modulated ac susceptibility measurements,we are the firs to fin that the superconductivity in this nickelate is filamentary-like Our scanning transmission electron microscopy investigations suggest that the filamentary-lik superconductivity most likely emerges at the interface between La_(3)Ni_(2)O_(7)and La_(4)Ni_(3)O_(10)phases.By tuning the oxygen content of polycrystalline La_(3)Ni_(2)O_(7),we also fin that it plays vital role in the development and stabilization of superconductivity in this material.The upper and lower bounds on the oxygen content are 7.35 and 6.89,respectively.Our results provide not only new insights into the puzzling issues regarding this material,but also significan information that will enable a better understanding of its superconductivity. 展开更多
关键词 scanning transmission electron microscopy oxygen content REPRODUCIBILITY filamentary superconductivity NICKELATE high temperature superconductivity d transition elementsfollowing pressure induced superconductivity
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Scalable topological-entanglement conductive coaxial fibers with superior durability for wearable strain sensing and triboelectric fabric
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作者 Yulong Wang Xia liu +7 位作者 chengyu li Wei Wang Di Guo Mengmeng Jia Shidai Tian lingyu Wan Aifang Yu Junyi Zhai 《Journal of Materials Science & Technology》 2025年第30期154-165,共12页
Although flexible,stretchable,and conductive core-sheath structured smart fibers have propelled to the forefront research in wearable strain sensors and self-powered electronics,challenges related to scalability,compl... Although flexible,stretchable,and conductive core-sheath structured smart fibers have propelled to the forefront research in wearable strain sensors and self-powered electronics,challenges related to scalability,complexity,and mechanical durability remain.In this study,we propose a strategy for the scalable production of conductive coaxial fiber(CCF)with superior durability through one-step direct wet spinning coherent solutions.By introducing the polystyrene-block-polyisoprene-block-polystyrene phase in both inner and outer layers,CCFs feature an interleaved topology and share a similar modulus,successfully resolving the issue of layer separation over time.They can endure up to 15,000 cycles with no damage at a strain of 100%.In addition,the topological entanglement CCF as a strain sensor exhibits a broad operational range of up to 398.3%strain,outstanding sensitivity(i.e.,gauge factor=6713 at 398.3%strain)and swift response time(248 ms).Enhanced by machine learning,the system achieves a high accuracy rate of 95%in gait recognition and 100%in American Sign Language identification.Furthermore,the CCF can function as a wearable triboelectric nanogenerator(TENG)for self-powered sensing and mechanical energy harvesting.This study represents a significant step toward the development of multifunctional micro-wearable electronic devices,which hold immense promise for medical sensing and energy harvesting in smart wearable electronics,human-computer interaction,and artificial intelligence. 展开更多
关键词 Conductive coaxial fiber Topological-entanglement Strain sensor Triboelectric nanogenerator Self-powered sensor
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Hybrid genetic algorithm for parametric optimization of surface pipeline networks in underground natural gas storage harmonized injection and production conditions
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作者 Jun Zhou Zichen li +4 位作者 Shitao liu chengyu li Yunxiang Zhao Zonghang Zhou Guangchuan liang 《Natural Gas Industry B》 2025年第2期234-250,共17页
The surface injection and production system(SIPS)is a critical component for effective injection and production processes in underground natural gas storage.As a vital channel,the rational design of the surface inject... The surface injection and production system(SIPS)is a critical component for effective injection and production processes in underground natural gas storage.As a vital channel,the rational design of the surface injection and production(SIP)pipeline significantly impacts efficiency.This paper focuses on the SIP pipeline and aims to minimize the investment costs of surface projects.An optimization model under harmonized injection and production conditions was constructed to transform the optimization problem of the SIP pipeline design parameters into a detailed analysis of the injection condition model and the production condition model.This paper proposes a hybrid genetic algorithm generalized reduced gradient(HGA-GRG)method,and compares it with the traditional genetic algorithm(GA)in a practical case study.The HGA-GRG demonstrated significant advantages in optimization outcomes,reducing the initial cost by 345.371×10^(4) CNY compared to the GA,validating the effectiveness of the model.By adjusting algorithm parameters,the optimal iterative results of the HGA-GRG were obtained,providing new research insights for the optimal design of a SIPS. 展开更多
关键词 Underground natural gas storage Surface injection and production pipeline Parameter optimization Hybrid genetic algorithm
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Eu^(3+)-doped BaLiZn_(3)(BO_(3))_(3):A novel red-emitting phosphor for blue chips excited white LEDs 被引量:4
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作者 Jiangyue Su Ran Pang +8 位作者 Haiyan Wu Shangwei Wang Tao Tan Weihong Yuan Su Zhang lihong Jiang Da li chengyu li Hongjie Zhang 《Journal of Rare Earths》 SCIE EI CAS CSCD 2022年第7期1014-1021,共8页
A series of novel red-emitting BaLiZn_(3)(BO_(3))_(3):Eu^(3+)phosphors were synthesized through the high temperature solid state reaction method.The phase composition,crystal structure,morphology and photo luminescenc... A series of novel red-emitting BaLiZn_(3)(BO_(3))_(3):Eu^(3+)phosphors were synthesized through the high temperature solid state reaction method.The phase composition,crystal structure,morphology and photo luminescence property of the BaLiZn_(3)(BO_(3))_(3):Eu^(3+)samples were systematically investigated.The phosphor can be efficiently excited by the near ultraviolet light(NUV)of 396 nm and blue light of 466 nm,and give out red light emission at 618 nm corresponding to the electric dipole transition(^(5)D_(0)→^(7)E_(2)).The optimal doping concentration of Eu^(3+)ions in BaLiZn_(3)(BO_(3))_(3)is determined to be about 3 mol%,and the concentration-quenching phenomenon arise from the electric dipole-dipole interaction.The temperature dependent luminescence behavior of BaLiZn_(3)(BO_(3))_(3):0.03 Eu^(3+)phosphor exhibits its good thermal stability,and the activation energy for thermal quenching characteristics is calculated to be 0.1844 eV.The decay lifetime of the BaLiZn_(3)(BO_(3))_(3):0.03 Eu^(3+)is measured to be 1.88 ms.These results suggest that the BaLiZn_(3)(BO_(3))_(3):Eu^(3+)phosphors have the potential application as a red component in white light emitting diodes(WLEDs)with NUV or blue chips. 展开更多
关键词 Light emitting diodes Red-emitting PHOSPHORS Blue chips Rare earths
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Defect in Brnym1,a magnesium-dechelatase protein,causes a stay-green phenotype in an EMSmutagenized Chinese cabbage(Brassica campestris L.ssp.pekinensis)line 被引量:7
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作者 Nan Wang Yun Zhang +3 位作者 Shengnan Huang Zhiyong liu chengyu li Hui Feng 《Horticulture Research》 SCIE 2020年第1期2667-2677,共11页
Leaf color is an important target trait in Chinese cabbage breeding programs.Leaf yellowing may reduce crop commercial and nutritional values.Some plants with the“stay-green”trait maintain leaf greenness during sene... Leaf color is an important target trait in Chinese cabbage breeding programs.Leaf yellowing may reduce crop commercial and nutritional values.Some plants with the“stay-green”trait maintain leaf greenness during senescence and even after death.Stay-green Chinese cabbage may be a focal point of future breeding projects because it could improve crop quality and yield and prolong shelf life.A new stay-green mutant,non-yellowing mutant 1(nym1),was identified in Chinese cabbage derived from an ethyl methane sulfonate(EMS)-mutagenized population.The mutant had stay-green characteristics and a higher chlorophyll content than the wild-type during leaf senescence.The staygreen trait in the mutant Chinese cabbage was controlled by the recessive gene Brnym1.MutMap and KASP analyses showed that Brnym1(BraA03g050600.3C)encodes an mg-dechelatase(SGR protein),which might be the causal gene of the mutation in Chinese cabbage.A nonsynonymous single nucleotide base substitution(G to A)in the third exon of Brnym1 caused an amino acid substitution from L to F in the highly conserved domain of the magnesiumdechelatase.Ectopic overexpression showed that the BrNYM1 gene of wild-type Chinese cabbage complemented the SGR-defective stay-green mutant nye1-1 of Arabidopsis.The magnesium-dechelatase activity in the nym1 mutant was significantly downregulated compared to that in the wild type.Brnym1 was relatively upregulated in the mutant during late senescence,and BrNYM1 was localized to the chloroplasts.These results indicate that Brnym1(BraA03g050600.3C)is the causal gene of the stay-green mutation and could be of particular significance in the genetic improvement of Chinese cabbage. 展开更多
关键词 breeding elata MAGNESIUM
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Hybrid coating SnO_(2)for enhanced Li ions storage 被引量:1
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作者 Yanan Gao Jie liu +10 位作者 Chenjie Lou Hailiang Geng Jipeng Fu chengyu li Yongjin Chen Cong Wang Wenda Zhang Xiaojun Kuang Yifan liu Xiang Gao Mingxue Tang 《Chinese Chemical Letters》 SCIE CAS CSCD 2023年第12期396-400,共5页
Anode SnO_(2)in lithium-ion batteries suffers from volume expansion and agglomeration.Here,the SnO_(2)nanoparticles are hybrided with ZrO_(2)particles by the support of carbon nanotube networks.The obtained SnO_(2)/C/... Anode SnO_(2)in lithium-ion batteries suffers from volume expansion and agglomeration.Here,the SnO_(2)nanoparticles are hybrided with ZrO_(2)particles by the support of carbon nanotube networks.The obtained SnO_(2)/C/ZrO_(2)composite shows improved electrochemical performances.Investigations reveal that the carbon nanotubes shorten the transmission path of electrons and Li^(+) ions.Ball milling with ZrO_(2)promotes the formation of nanosized SnO_(2)to weaken the internal strain change,being beneficial to buffering volume change during electrochemical cycling afterwards.High-resolution 6.7Li NMR investigations indicate that conversion and alloying reactions are stepwise involved for SnO_(2)/C/ZrO_(2)anode.The strategy of designing SnO_(2)/C/ZrO_(2)composite from the morphology-controlled metal-organic frameworks for energy storage widens the possibility to fabricate promising materials with enhanced performances. 展开更多
关键词 Hybrid regulation Lithium-ion batteries Fast migration Volume confinement Energy storage
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Yolk-shell nanoarchitecture for stabilizing a Ce_(2)S_(3)anode 被引量:1
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作者 Kanglong Hui Jipeng Fu +7 位作者 Jie liu Yongjin Chen Xiang Gao Tian Gao Qi Wei chengyu li Hongjie Zhang Mingxue Tang 《Carbon Energy》 CAS 2021年第5期709-720,共12页
Rare-earth sulfides are of research interest for lithium-ion batteries(LIBs)due to their abundant lithium intercalation sites and low redox voltage.However,their electrochemical performances are not satisfactory becau... Rare-earth sulfides are of research interest for lithium-ion batteries(LIBs)due to their abundant lithium intercalation sites and low redox voltage.However,their electrochemical performances are not satisfactory because of poor conductivity and volume change upon electrochemical cycling.Herein,nanoarchitectures ofγ-Ce_(2)S_(3)encapsulated in a hollow mesoporous carbon nanosphere(Ce_(2)S_(3)@HMCS)are fabricated using the self-template strategy combined with the in-sphere sulfuration method and tested as an LIB anode.The void space between the Ce_(2)S_(3)core and the outer layer of the carbon nanosphere has been properly designed and modulated to achieve excellent electrochemical performance in terms of electronic conductivity,reversibility,and rate capability.The reversible capacity of Ce_(2)S_(3)@HMCS is 2.6 times that of the pure Ce_(2)S_(3)anode,which can gradually increase and maintain a capacity of 282 mAh·g^(−1)at a current density of 1 A·g^(-1),and a high Coulombic efficiency(~100%)can be achieved even after 1000 cycles.This good performance is attributed to the unique yolk-shell nanostructure with a highly crystallized and stable Ce3S2 core and volume expansion buffer space upon lithiation/delithiation.Ex situ X-ray diffraction and nuclear magnetic resonance results indicate that the lithiation of Ce_(2)S_(3)@HMCS is an intercalation process.This study represents an important advancement in precise structural design with in-sphere sulfuration and sheds light on a potential direction for highperformance lithium storage. 展开更多
关键词 Ce_(2)S_(3)anode intercalation mechanism lithium ion batteries structure stabilizing yolk-shell nanoarchitecture
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Adjoint-based optimization of flapping plates hinged with a trailing-edge flap 被引量:1
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作者 Min Xu Mingjun Wei +1 位作者 chengyu li Haibo Dong 《Theoretical & Applied Mechanics Letters》 CAS CSCD 2015年第1期1-4,共4页
It is important to understand the impact of wing-morphing on aerodynamic performance in the study of flapping-wing flight of birds and insects. We use a flapping plate hinged with a trailing-edge flap as a simplified ... It is important to understand the impact of wing-morphing on aerodynamic performance in the study of flapping-wing flight of birds and insects. We use a flapping plate hinged with a trailing-edge flap as a simplified model for flexible/morphing wings in hovering. The trailing-edge flapping motion is opti- mized by an adjoint-based approach. The optimized configuration suggests that the trailing-edge flap can substantially enhance the overall lift. Further analysis indicates that the lift enhancement by the trailing- edge flapping is from the change of circulation in two ways: the local circulation change by the rotational motion of the flap, and the modification of vortex shedding process by the relative location between the trailing-edge flao and leading-edge main plate. 展开更多
关键词 Flapping wingTrailing-edge flapAdjoint-based optimization
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Dual-enhancement of chromaticity and thermal stability:In-situ synthesis of core-shell γ-Ce_(2)S_(3) @CePO_(4) configuration
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作者 Kanglong Hui Wei Dong +4 位作者 Jipeng Fu Mingxue Tang Qi Wei chengyu li Hongjie Zhang 《Journal of Rare Earths》 SCIE EI CAS CSCD 2022年第5期800-806,I0005,共8页
Non-toxic rare earth(RE) composite materials are promising and active in optoelectronic fields,such as pigment.In this work,Na ions doped γ-Ce_(2) S_(3) pigments were synthesized by solid-phase vulcanization and foll... Non-toxic rare earth(RE) composite materials are promising and active in optoelectronic fields,such as pigment.In this work,Na ions doped γ-Ce_(2) S_(3) pigments were synthesized by solid-phase vulcanization and followed by in-situ synthesis to prepare an outer layer of CePO_(4) film.The characterizations of X-ray diffraction(XRD),scanning electron microscopy(SEM),transmission electron microscopy(TEM),X-ray photoelectron spectroscopy(XPS),solid state nuclear magnetic resonance(NMR) indicate that Na-dopedγ-Ce_(2) S_(3) and CePO_(4) uniformly and tightly coated core-shell structure was successfully synthesized.The thermogravimetric analysis(TG) and reflection spectrum(RS) reveal that the CePO_(4) coating significantly improves the colorant and thermal stability performance of γ-Ce_(2) S_(3) .The excellent color quality of γ-Ce_(2) S_(3) @CePO_(4)(L*=45.16,a*=55.94.b*=44.53) is achieved and the red color(L*=43.82,a*=49.79,b*=38.04) is still retained even if the sample is heated in air at 400℃ for 30 min. 展开更多
关键词 γ-Ce_(2)S_(3) Red pigment Core-shell structure CePO_(4)coating Rare earths
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Efficacy and safety of Shen Zhi Ling oral liquid(a Chinese patent)for Alzheimer's disease:A meta-analysis of randomized controlled trials
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作者 Shiqi Chen Chunxiang liu +2 位作者 Hui Wang chengyu li Hongcai Shang 《TMR Modern Herbal Medicine》 2020年第4期224-232,共9页
Objective:To evaluate the efficacy and safety of Shen Zhi Ling oral liquid(SZL)alone or combined with basic treatment in treating Alzheimer's Disease(AD).Methods:Databases including PubMed,the Cochrane Library,Emb... Objective:To evaluate the efficacy and safety of Shen Zhi Ling oral liquid(SZL)alone or combined with basic treatment in treating Alzheimer's Disease(AD).Methods:Databases including PubMed,the Cochrane Library,Embase,Web of science,China National Knowledge Infrastructure(CNKI),Wanfang Database and the Chinese Science and Technology Journal Database(VIP)were searched from inception to September 20,2020 to collect relevant randomized controlled trials(RCTs)comparing SZL with other nootropic drugs for AD.The primary clinical outcomes were scores of the Mini Mental State Examination(MMSE)and the Activities of Daily Living(ADL)during treatment.The secondary outcomes of our study included other neuropsychological scale scores including Rapid Verbal Retrieve(RVR),Digit Span(DS),Fuld Object-Memory Evaluation(FOM)and adverse events or reactions.Two authors searched and screened the literature independently,then extracted the data and evaluated the methodological quality by using the handbook of Cochrane Collaboration,and analyzed the data via the Review Manager 5.3 software.Results:In total,we included four studies,covering 217 participants.All studies were in a low methodological quality.The result of MMSE score,ADL score,RVR score,DS score and FOM score in the meta-analysis showed that no statistically significant difference(P>0.05)between the treatment groups and control groups,and the statistical heterogeneity of all meta-analyses was small(I2<50%).SZL was indicated no better than other nootropic drugs.Among the included studies,no study described adverse events.Conclusions:Considering the low quality of the included trials and the different levels of AD patients,we are unable to come to any conclusion about the efficacy and safety of SZL compared with other nootropic drugs.Moreover,we still need rigorously designed,multi-center,large-scale trials to further confirm the efficacy and safety of SZL. 展开更多
关键词 Shen Zhi Ling oral liquid Traditional Chinese medicine Alzheimer's disease Systematic review META-ANALYSIS
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中国省际工业生态效率空间分布及影响因素研究 被引量:68
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作者 李成宇 张士强 张伟 《地理科学》 CSSCI CSCD 北大核心 2018年第12期1970-1978,共9页
将中国30省市(不含港、澳、台和西藏地区)作为研究对象,进行省际工业生态效率空间分布及影响因素研究。首先构建中国省际工业生态效率评价指标体系,其次利用DEA-BCC模型结合Malmquist指数对2006~2015年中国30省市在时空两个维度上的工... 将中国30省市(不含港、澳、台和西藏地区)作为研究对象,进行省际工业生态效率空间分布及影响因素研究。首先构建中国省际工业生态效率评价指标体系,其次利用DEA-BCC模型结合Malmquist指数对2006~2015年中国30省市在时空两个维度上的工业生态效率进行测算,再次运用Geoda软件分析中国工业生态效率的空间分布特征,最后通过空间误差模型对中国工业生态效率的影响因素进行检验。研究结果表明:①中国工业生态效率虽呈现小幅度下降趋势,但整体效率水平较高;30省市之间存在明显差异性,呈现出东部 >中部 >西部的分布格局。②中国工业生态效率Malmquist指数增长率水平较高;30省市Malmquist指数均为正向增长,呈现出稳定增长趋势;技术进步效率是Malmquist指数的主要推动力。③中国30省市工业生态效率呈现正向空间自相关性,且存在明显的集聚状态,近邻效应显著。④中国省际工业生态效率的主要影响因素有经济发展水平、产业结构、政府规制、技术进步、外商投资和产业集聚。 展开更多
关键词 工业生态效率 BCC模型 MALMQUIST指数
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Preparation and luminescence properties of orange-red Ba3Y4O9:Sm3+phosphors 被引量:8
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作者 Jiayu li Ran Pang +7 位作者 Zhan Yu liyan liu Haiyan Wu Huimin li lihong Jiang Su Zhang Jing Feng chengyu li 《Journal of Rare Earths》 SCIE EI CAS CSCD 2018年第7期680-684,共5页
A novel orange-red emitting Ba3 Y4 O9:Sm^(3+) phosphors were prepared by a high temperature solidstate reaction in air. X-ray diffraction(XRD), photoluminescence spectra, fluorescence decay and temperature-depen... A novel orange-red emitting Ba3 Y4 O9:Sm^(3+) phosphors were prepared by a high temperature solidstate reaction in air. X-ray diffraction(XRD), photoluminescence spectra, fluorescence decay and temperature-dependent emission spectra were utilized to characterize the structure and luminescence properties. The results show that the excitation spectrum includes a series of linear peaks at350, 367, 382, 410, 424, 445, 470 and 495 nm, respectively. Under 410 nm excitation, the emission peaks were located at 574 nm(~4 G(5/2)-~6 H(5/2)), 608 nm(~4 G(5/2)-~6 H(7/2)),659 nm(~4 G(5/2)-~6 H(9/2)) and722 nm(~4 G(5/2)-~6 H(11/2)), respectively. The concentration quenching occurs when x equals 0.08 for Ba3 Y(4-x)O9:xSm^(3+) phosphor and its mechanism is ascribed to the dipole-dipole interaction. The chromaticity coordinates of Ba3 Y(3.92)O9:0.08 Sm^(3+) phosphor are in the orange-red region. The temperature-dependent study shows that this phosphor has excellent luminescence thermal-stability.And the luminescence intensity of Ba3 Y(3.92)O9:0.08 Sm^(3+) phosphor at 473 K only declines by about25.75% of its initial intensity. The experimental data indicate that Ba3 Y4 O9:Sm^(3+) phosphor may be promising as an orange-red emitting phosphor for white light emitting diodes. 展开更多
关键词 Orange-red phosphors Rare earths Ba3Y4O9 PHOTOLUMINESCENCE
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Synthesis,structure and optical properties of novel thermally robust Dy^(3+)-doped Ca_(9)Sc(PO_(4))_(7) phosphors for NUV-excited white LEDs 被引量:5
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作者 Haiyan Wu Huimin li +7 位作者 lihong Jiang Ran Pang Su Zhang Da li Guanyu liu chengyu li Jing Feng Hongjie Zhang 《Journal of Rare Earths》 SCIE EI CAS CSCD 2021年第3期277-283,I0002,共8页
The powder samples of Ca_(9)Sc(PO_(4))_(7):xDy^(^(3+))white emitting phosphors were prepared via a solid state reaction technique.The Ca_(9)Sc(PO_(4))_(7):Dy^(3+)samples were researched by using the GSAS Rietveld refi... The powder samples of Ca_(9)Sc(PO_(4))_(7):xDy^(^(3+))white emitting phosphors were prepared via a solid state reaction technique.The Ca_(9)Sc(PO_(4))_(7):Dy^(3+)samples were researched by using the GSAS Rietveld refinement and X-ray diffraction(XRD) methods,and SEM images and elemental maps were recorded.Under 350 nm excitatio n,the emission spectra of Ca_(9)Sc(PO_(4))_(7):xDy^(3+)samples have two obvious peaks and one weak peak at 484,572 and660 nm,corresponding to the characteristic electron transitions of(^(4)F_(9/2)→ ^(6)H_(15/2),blue),(^(4)F_(9/2)→ ^(6)H_(13/2),yellow) and(^(4)F_(9/2)→ 6 H11/2,red),respectively.The concentration quenching effect,decay lifetime and thermal quenching of the as-synthesized Ca_(9)Sc(PO_(4))_(7):Dy^(3+)samples were researched systematically.The Ca_(9)Sc(PO_(4))_(7):0.02 Dy^(3+)phosphor possesses a good thermal stability,of which the emission intensity at 423 K can maintain 79% of the initial value(273 K).In addition,through the study of the chro maticity coordinates of the Ca_(9)Sc(PO_(4))_(7):0.02 Dy^(3+)phosphor,it is found that it is located in the white region,and the Commission Internationalede L’Eclairage(CIE) chromaticity coordinates are(0.339,0.389),The above results show that Ca_(9)Sc(PO_(4))_(7):xDy^(3+)phosphors can be excellent candidate material for applications in NUV-excited white LEDs. 展开更多
关键词 Ca_(9)Sc(PO_(4))7:Dy^(3+) White LEDs PHOSPHATE Photoluminescence Rare earths
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High-Efficiency Wastewater Purification System Based on Coupled Photoelectric–Catalytic Action Provided by Triboelectric Nanogenerator 被引量:4
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作者 Shen Shen Jiajia Fu +8 位作者 Jia Yi liyun Ma Feifan Sheng chengyu li Tingting Wang Chuan Ning Hongbo Wang Kai Dong Zhong lin Wang 《Nano-Micro Letters》 SCIE EI CAS CSCD 2021年第12期95-108,共14页
It is of great importance to explore a creative route to improve the degradation e ciency of organic pollutants in wastewater.Herein,we construct a unique hybrid system by combining self-powered triboelectric nanogene... It is of great importance to explore a creative route to improve the degradation e ciency of organic pollutants in wastewater.Herein,we construct a unique hybrid system by combining self-powered triboelectric nanogenerator(TENG)with carbon dots-TiO_(2)sheets doped three-dimensional graphene oxide photocatalyst(3 DGA@CDs-TNs),which can significantly enhance the degradation e ciency of brilliant green(BG)and direct blue 5 B(DB)owing to the powerful interaction of TENG and 3 DGA@CDs-TNs photocatalyst.The power output of TENG can be applied for wastewater purification directly,which exhibits a selfpowered electrocatalytic technology.Furthermore,the results also verify that TENG can replace conventional electric catalyst to remove pollutants e ectively from wastewater without any consumption.Subsequently,the unstable fragments and the plausible removal pathways of the two pollutants are proposed.Our work sheds light on the development of e cient and sustainable TENG/photocatalyst system,opening up new opportunities and possibilities for comprehensive utilization of random energy. 展开更多
关键词 Triboelectric nanogenerators SELF-POWERED 3DGA@CDs-TNs photocatalyst Hybrid system Wastewater purification
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The Uniform Distribution of SiC Particles in an A356-SiC_p Composite Produced by the Tilt-blade Mechanical Stirring 被引量:3
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作者 Yunhui DU Peng ZHANG +3 位作者 Yujie WANG Jun ZHANG Shasha YAO chengyu li 《Acta Metallurgica Sinica(English Letters)》 SCIE EI CAS CSCD 2013年第1期69-74,共6页
The tilt-blade mechanical stirring of A356-2.5vol.%SiCp liquid was conducted in a cylindrical crucible to solve the problem of nonhomogeneous radial distribution of SiC particles in conventional straight-blade mechani... The tilt-blade mechanical stirring of A356-2.5vol.%SiCp liquid was conducted in a cylindrical crucible to solve the problem of nonhomogeneous radial distribution of SiC particles in conventional straight-blade mechanical stirring. The radial distribution of SiC particles in A356 liquid was studied under the conditions of 25° for horizontal tilt angle α of the blade, 200 r/min for rotating speed of stirrer and 10 mm/s for speed of moving up and down of stirrer. The results show that there exists a nonlinear relationship between circumferential tilt angle β of the blade and radial relative deviation d of SiCp content in A356 liquid. When β is smaller than 20°, the d of SiCp content in A356 liquid between the center and the periphery of crucible decreases with increasing β. Conversely, when β is bigger than 26°, d increases with increasing β. Only when β is about 20°, d can be equal to nought i.e. uniform radial distribution of SiC particles can be realized. It can be seen that the nonhomogeneous radial distribution of SiC particles in conventional straight-blade mechanical stirring can be eliminated in this tilt-blade mechanical stirring of A356-SiCp liquid. 展开更多
关键词 Tilt-blade mechanical stirring Relationship Uniform distribution
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Single-phase white-emitting and tunable color phosphor Na_(3)Sc_(2)(PO_(4))_(3):Eu^(2+),Dy^(3+): Synthesis, luminescence and energy transfer 被引量:1
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作者 Sen Wang Haiyan Wu +10 位作者 Xin Wen Yanqing Luo Tao Tan Shengjian Jiao Ran Pang lihong jiang Su Zhang Da li Guanyu liu chengyu li Hongjie Zhang 《Journal of Rare Earths》 SCIE EI CAS CSCD 2022年第4期551-558,I0002,共9页
A series of Eu^(2+)/Dy^(3+) single doped and co-doped Na_(3)Sc_(2)(PO_(4))_(3) phosphors were synthesized by the high-temperature solid-state method,and their phase,morphology,and luminescence properties were characte... A series of Eu^(2+)/Dy^(3+) single doped and co-doped Na_(3)Sc_(2)(PO_(4))_(3) phosphors were synthesized by the high-temperature solid-state method,and their phase,morphology,and luminescence properties were characterized.Under the excitation of 370 nm,the Na_(3)Sc_(2)(PO_(4))_(3):Eu^(2+),Dy^(3+) phosphor can emit white light whose spectrum is composed of a broad emission band centered at 460 nm and the other three peaks at 483,577,and 672 nm,respectively.There is energy transfer from Eu^(2+)to Dy^(3+)ion in Na_(3)Sc_(2)(PO_(4))_(3):Eu^(2+),Dy^(3+) phosphor due to the good overlap between the emission spectrum of Na_(3)Sc_(2)(PO_(4))_(3):Eu^(2+) and the excitation spectrum of Na_(3)Sc_(2)(PO_(4))_(3):Dy^(3+),which is further confirmed by the fluorescence lifetime decrease of Eu^(2+)ion with the increase of Dy^(3+) concentration.The process of energy transfer is via dipole–quadruple interaction which is confirmed by applying Dexter's theory.By increasing the Dy^(3+)concentration,the color coordinates of the Na_(3)Sc_(2)(PO_(4))_(3):0.01Eu^(2+),xDy^(3+)phosphors can be adjusted from blue to white,and then to yellow.The optimized concentration of Dy^(3+)ions is 4.0 mol%,beyond which the concentration quenching will take place.The Na_(3)Sc_(2)(PO_(4))_(3):Eu^(2+),Dy^(3+)phosphor shows fairly good resistance to thermal quenching behavior,of which the emission intensity at 423 K can maintain 90.3%of the initial value(298 K).These results suggest that the Na_(3)Sc_(2)(PO_(4))_(3):0.01Eu^(2+),xDy^(3+)phosphors have potential applications as the color-tunable or a single-phase white emitting phosphor in white LEDs. 展开更多
关键词 Energy transfer PHOSPHATE LUMINESCENCE Rare earths
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Correlating O-deficiency and luminescence property of Tb^(3+)þdoped SrO 被引量:1
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作者 Kaina Wang Jipeng Fu +10 位作者 Shuqin Chang Xuan Sun Tianyi Sun Su Zhang Ran Pang lihong Jiang Xiaojun Kuang Evan Wenbo Zhao chengyu li Shiqing Xu Mingxue Tang 《Advanced Powder Materials》 2023年第3期28-35,共8页
Cubic rock salt can lower down or break the rare earth transition barrier through interstitial or vacancy defects owing to its great deformation and rotationflexibility.Here,we demonstrate that oxygen vacancies in SrO ... Cubic rock salt can lower down or break the rare earth transition barrier through interstitial or vacancy defects owing to its great deformation and rotationflexibility.Here,we demonstrate that oxygen vacancies in SrO are induced by proper oxidization and atmosphere adjustment,resulting in defects with various depths and crystalfield distortion.The thermally assisted tunneling from defects to 5 D_(4) state and electronic population decrease on 5 D_(3) state of Tb^(3+)þare observed by the deformation of adjacent oxygen octahedral structure.Finally,the asprepared SrO:0.01 Tb^(3+)þphosphors,commercial BaMgAl10O17:Eu^(2+)þblue phosphor,and CaAlSiN3:Eu^(2+)þred phosphor are mixed and coated onto 280 nm deep-ultraviolet LED chip to assemble white light-emitting LED device.The LEDs show CCT of 3850 K,4136 K,and 4741 K,with color rendering index of 90.3,90.8,and 92.1,respectively.These insights will advance the fundamental knowledge of crystal engineering in cubic rock salt,and enable new ways to manipulate energy transfer and electronic transition via defects. 展开更多
关键词 Oxygen vacancy Spectral modulation Long-lasting phosphorescence White LEDs Energy transfer
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Correction:A novel bright cyan emitting phosphor of Eu^(2+)activated Ba_(6)BO_(3)Cl_(9)with robust thermal stability for full-spectrum WLED applications
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作者 Shengjian Jiao Ran Pang +3 位作者 Jiutian Wang Tao Tan chengyu li Hongjie Zhang 《Inorganic Chemistry Frontiers》 2023年第10期3151-3151,共1页
The authors regret that Chengyu Li’s affiliation was incorrect in the original manuscript.The corrected list of affiliations for this paper is as shown here.The Royal Society of Chemistry apologises for these errors ... The authors regret that Chengyu Li’s affiliation was incorrect in the original manuscript.The corrected list of affiliations for this paper is as shown here.The Royal Society of Chemistry apologises for these errors and any consequent inconvenience to authors and readers. 展开更多
关键词 ba bo cl phosphor chengyu li s thermal stability eu full spectrum wled
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The research idea of Xuebijing injection in influencing severe pneumonia-pulmonary fibrosis with blood stasis syndrome evolution by inhibiting inflammation, endotoxin and dispersing blood stasis
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作者 Rui Zheng chengyu li +5 位作者 Ping Wang Min li Pengqian Wang Changming Zhong Jianxun Wang Hongcai Shang 《TMR Modern Herbal Medicine》 2020年第2期113-119,共7页
Severe pneumonia is one of the most serious infectious diseases.Delayed intervention may lead to pulmonary fibrosis,which greatly threatens people’s life and health.Blood stasis syndrome is an important underlying sy... Severe pneumonia is one of the most serious infectious diseases.Delayed intervention may lead to pulmonary fibrosis,which greatly threatens people’s life and health.Blood stasis syndrome is an important underlying syndrome throughout the evolution of severe pneumonia-pulmonary fibrosis.Xuebijing injection(XBJ)was developed under the theoretical system of“Three syndromes and three methods”,demonstrating a good efficacy in treating severe pneumonia and pulmonary fibrosis due to its effect of removing blood stasis and dispersing toxins.Previous studies have shown that XBJ can protect vascular endothelial function,improve coagulation function and regulate immunity by inhibiting inflammatory.Hence,the research hypothesis is put forward that XBJ treats blood stasis syndrome by removing blood stasis and dredging blood vessels,to inhibit the disease progress of severe pneumonia to pulmonary fibrosis.Further researches are need to confirm the function and explore the mechanism of XBJ. 展开更多
关键词 XUEBIJING injection Severe PNEUMONIA Pulmonary fibrosis Blood STASIS syndrome COAGULATION
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Deep Learning Model Coupling Wearable Bioelectric and Mechanical Sensors for Refined Muscle Strength Assessment
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作者 chengyu li Tingyu Wang +12 位作者 Siyu Zhou Yanshuo Sun Zijie Xu Shuxing Xu Sheng Shu Yi Zhao Bing Jiang Shiwang Xie Zhuoran Sun Xiaowei Xu Weishi li Baodong Chen Wei Tang 《Research》 2025年第1期215-229,共15页
Muscle strength(MS)is related to our neural and muscle systems,essential for clinical diagnosis and rehabilitation evaluation.Although emerging wearable technology seems promising for MS assessment,problems still exis... Muscle strength(MS)is related to our neural and muscle systems,essential for clinical diagnosis and rehabilitation evaluation.Although emerging wearable technology seems promising for MS assessment,problems still exist,including inaccuracy,spatiotemporal differences,and analyzing methods.In this study,we propose a wearable device consisting of myoelectric and strain sensors,synchronously acquiring surface electromyography and mechanical signals at the same spot during muscle activities,and then employ a deep learning model based on temporal convolutional network(TCN)+Transformer(Tcnformer),achieving accurate grading and prediction of MS.Moreover,by combining with deep clustering,named Tcnformer deep cluster(TDC),we further obtain a 25-level classification for MS assessment,refining the conventional 5 levels.Quantification and validation showcase a patient's postoperative recovery from level 3.2 to level 3.6 in the first few days after surgery.We anticipate that this system will importantly advance precise MS assessment,potentially improving relevant clinical diagnosis and rehabilitation outcomes. 展开更多
关键词 surface electromyography mechanical signals myoelectric sensors muscle strength ms clinical diagnosis wearable devices strain sensors
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