Characteristics of two serious air pollution episodes(9–15 January, as the winter case; and30 June to 1 July, as the summer case), which occurred in Beijing in 2013 were investigated and compared using multi-method...Characteristics of two serious air pollution episodes(9–15 January, as the winter case; and30 June to 1 July, as the summer case), which occurred in Beijing in 2013 were investigated and compared using multi-method observations and numerical simulations. During these two air pollution episodes, PM2.5 concentrations varied significantly within Beijing, with PM2.5 concentrations in southern parts of Beijing being significantly higher than in northern areas. Typically, heavy air pollution episodes begin in the southern parts and disperse towards the northern parts of Beijing. Clearly, synoptic patterns and the stability of atmospheric circulation patterns were the main factors controlling air pollution in Beijing.During the winter case, a warm center above 900 h Pa occurred over Beijing. Meanwhile, in the summer case, although there was only a weak inversion, the convective inhibition energy was strong(over 200 J/k G). This clearly influenced the duration of the air pollution event. Except for the local accumulation and secondary atmospheric reactions in both cases, regional straw burnings contributed a lot to the PM2.5 concentrations in summer case.Using the CAMxmodel, we established that regional transport contributed almost 59% to the PM2.5 averaged concentration in Beijing in the winter case, but only 31% in the summer case. Thus, the winter case was a typical regional air pollution episode, while the summer case resulted from local accumulation straw burnings transportation and strong secondary atmospheric reactions. Given that air pollution is a regional problem in China, consistent and simultaneous implementation of regional prevention and control strategies is necessary to improve regional air quality.展开更多
In this paper,using concentration data of PM2. 5in 2013 in China and referring to a lot of literature,we preliminary studied the pollution of fine particulate matter and summarized PM2. 5source apportionment in the ke...In this paper,using concentration data of PM2. 5in 2013 in China and referring to a lot of literature,we preliminary studied the pollution of fine particulate matter and summarized PM2. 5source apportionment in the key cities in China. Our results showed that PM2. 5showed significant spatial and temporal distribution; high surface concentrations of PM2. 5concentrated mainly in the North China Plain,the Sichuan Basin,Yangtze River Delta and other regions; the average annual concentration of PM2. 5was about 80μg / m3 in North China Plain; Seasonal changes in the concentration of PM2. 5was winter > spring > autumn > summer; fired sources,industrial sources,vehicle exhaust were the major sources of PM2. 5; motor vehicle exhaust mostly contributed 10%- 30% to PM2. 5. This review provides a fundamental understanding of PM2. 5source apportionment and serves as an important reference for future source apportionment studies to be widely conducted in China.展开更多
基金supported by the Commonwealth Project of the Ministry of Environmental Protection (No. 201409005)the National Key Technology R&D Program (Nos. 2014BAC23B03, 2016YFC0208902 and D17110900150002)the excellent talents training project of the Organization Department of Beijing municipal Party Committee (2016000021733G166)
文摘Characteristics of two serious air pollution episodes(9–15 January, as the winter case; and30 June to 1 July, as the summer case), which occurred in Beijing in 2013 were investigated and compared using multi-method observations and numerical simulations. During these two air pollution episodes, PM2.5 concentrations varied significantly within Beijing, with PM2.5 concentrations in southern parts of Beijing being significantly higher than in northern areas. Typically, heavy air pollution episodes begin in the southern parts and disperse towards the northern parts of Beijing. Clearly, synoptic patterns and the stability of atmospheric circulation patterns were the main factors controlling air pollution in Beijing.During the winter case, a warm center above 900 h Pa occurred over Beijing. Meanwhile, in the summer case, although there was only a weak inversion, the convective inhibition energy was strong(over 200 J/k G). This clearly influenced the duration of the air pollution event. Except for the local accumulation and secondary atmospheric reactions in both cases, regional straw burnings contributed a lot to the PM2.5 concentrations in summer case.Using the CAMxmodel, we established that regional transport contributed almost 59% to the PM2.5 averaged concentration in Beijing in the winter case, but only 31% in the summer case. Thus, the winter case was a typical regional air pollution episode, while the summer case resulted from local accumulation straw burnings transportation and strong secondary atmospheric reactions. Given that air pollution is a regional problem in China, consistent and simultaneous implementation of regional prevention and control strategies is necessary to improve regional air quality.
文摘In this paper,using concentration data of PM2. 5in 2013 in China and referring to a lot of literature,we preliminary studied the pollution of fine particulate matter and summarized PM2. 5source apportionment in the key cities in China. Our results showed that PM2. 5showed significant spatial and temporal distribution; high surface concentrations of PM2. 5concentrated mainly in the North China Plain,the Sichuan Basin,Yangtze River Delta and other regions; the average annual concentration of PM2. 5was about 80μg / m3 in North China Plain; Seasonal changes in the concentration of PM2. 5was winter > spring > autumn > summer; fired sources,industrial sources,vehicle exhaust were the major sources of PM2. 5; motor vehicle exhaust mostly contributed 10%- 30% to PM2. 5. This review provides a fundamental understanding of PM2. 5source apportionment and serves as an important reference for future source apportionment studies to be widely conducted in China.