Aqueous zinc-halogen batteries are promising candidates for large-scale energy storage due to their abundant resources,intrinsic safety,and high theoretical capacity.Nevertheless,the uncontrollable zinc dendrite growt...Aqueous zinc-halogen batteries are promising candidates for large-scale energy storage due to their abundant resources,intrinsic safety,and high theoretical capacity.Nevertheless,the uncontrollable zinc dendrite growth and spontaneous shuttle effect of active species have prohibited their practical implementation.Herein,a double-layered protective film based on zinc-ethylenediamine tetramethylene phosphonic acid(ZEA)artificial film and ZnF2-rich solid electrolyte interphase(SEI)layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic optimization.The ZEA-based artificial film shows strong affinity for the ZnF2-rich SEI layer,therefore effectively suppressing the SEI breakage and facilitating the construction of double-layered protective film on the zinc metal anode.Such double-layered architecture not only modulates Zn2+flux and suppresses the zinc dendrite growth,but also blocks the direct contact between the metal anode and electrolyte,thus mitigating the corrosion from the active species.When employing optimized metal anodes and electrolytes,the as-developed zinc-(dual)halogen batteries present high areal capacity and satisfactory cycling stability.This work provides a new avenue for developing aqueous zinc-(dual)halogen batteries.展开更多
The Hehuang Valley,situated in the northeastern section of the Qinghai-Tibet Plateau,represents the upper reaches of the Yellow River(Fig.1A).It is a significant geographic region of origin for numerous Neolithic cult...The Hehuang Valley,situated in the northeastern section of the Qinghai-Tibet Plateau,represents the upper reaches of the Yellow River(Fig.1A).It is a significant geographic region of origin for numerous Neolithic cultures,including the Majiayao,Zongri,and Qijia cultures(Dong et al.,2013).展开更多
The accurate identification and diagnosis of chemical process faults are crucial for ensuring the safe and stable operation of production plants.The current hot topic in industrial process fault diagnosis research is ...The accurate identification and diagnosis of chemical process faults are crucial for ensuring the safe and stable operation of production plants.The current hot topic in industrial process fault diagnosis research is data-driven methods.Most of the existing fault diagnosis methods focus on a single shallow or deep learning model.This paper proposes a novel hybrid fault diagnosis method to fully utilize various features to improve the accuracy of fault diagnosis.Furthermore,the method addresses the issue of incomplete data,which has been largely overlooked in the majority of existing research.Firstly,the variable data is effectively fitted using orthogonal non-negative matrix tri-factorization,and the missing data in the matrix is solved to construct a complete production condition relationship.Next,the support vector machine model and the deep residual contraction network model are trained in parallel to prediagnose process faults by mining linear and non-linear interaction features.Finally,a novel mapping relationship is established between the result and model levels using the multi-layer perceptron algorithm to complete the final diagnosis and evaluation of the fault.To demonstrate the effectiveness of the proposed method,we conducted extensive comparative experiments on the Tennessee Eastman dataset and the ethylene plant cracking unit dataset.The experimental results show that the method has advantages in different evaluation metrics.展开更多
Through an example of a main transformer switch-in with load during the reverse transmission of a 750 kV power plan,the paper introduces the basic principle of transformer switch-in with load.EMTPE program that is use...Through an example of a main transformer switch-in with load during the reverse transmission of a 750 kV power plan,the paper introduces the basic principle of transformer switch-in with load.EMTPE program that is used to establish a calculation model,at the same time mainly considers the excitation characteristics of the transformer,the transient model of the circuit breaker,and the model of high voltage transformer,and calculated the inrush current with transformer switch-in with load in this plan.During system debugging in the plan,the two sets of main transformers passed the closing and opening test,and the data of inrush current in the test are recorded and analyzed.The simulation calculation and measured data show that the results are consistent.The simulation calculation also shows that it is not recommended to perform on-load closing of the transformer except for special circumstances,because of the influence of hysteresis characteristic when the transformer was switched in with load or the terminal voltage of the transformer resumed normal level from a low one after an external near-end fault was cleared,which various transformer differential protection using the characteristics of inrush to implement block scheme may mal-operate.展开更多
Designing cathode possessing crystalline@amorphous core-shell structure with both active core and shell is a meaningful work for resolving the low specific capacity,unstable cycling performance and sluggish reaction ki...Designing cathode possessing crystalline@amorphous core-shell structure with both active core and shell is a meaningful work for resolving the low specific capacity,unstable cycling performance and sluggish reaction kinetics issues of rechargeable magnesium batteries(RMBs)by providing more active sites as well as releasing inner stress during cycling.Herein,WO_(3)@WO_(3-x)S_(x) owning crystalline@amorphous core-shell structure containing both active core and active shell is constructed successfully by introducing S into metastable WO3 structure under temperaturefield applying.In such structure,amorphous shell would provide continuous Mg^(2+)diffusion channels due to its isotropy property for most Mg^(2+)migrating rapidly to interface and then adsorb at ions reservoir formed by interfacial electricfield for increasing specific capacity.It also makes security for stable structure of WO_(3)@WO_(3-x)S_(x) by alleviating volume expansion of crystalline core WO_(3) during cycling to prolong cycling life.Additionally,“softer”ions S^(2-)would weaken interaction between hard acid Mg^(2+) and ionic lattice to enhance Mg^(2+)storage kinetics.Therefore,WO_(3)@WO_(3-x)S_(x) delivers the superior cycling performance(1000 cycles with 83.3%),rate capability(88.5 mAh g^(-1) at 1000 mA g^(-1))and specific capacity(about 150 mAh g^(-1) at 50 mA g^(-1)),which is near 2 times higher than that of WO3.It is believed that the crystalline@amorphous core-shell structure with both active core and shell designing via doping strategy is enlightening for the development of high-performance RMBs,and such design can be extended to other energy storage devices for better electrochemical performance.展开更多
Bubble breakup at T-junction microchannels is the basis for the numbering-up of gas−liquid two-phase flow in parallelized microchannels. This article presents the bubble breakup in viscous liquids at a microfluidic T-...Bubble breakup at T-junction microchannels is the basis for the numbering-up of gas−liquid two-phase flow in parallelized microchannels. This article presents the bubble breakup in viscous liquids at a microfluidic T-junction. Nitrogen is used as the gas phase, and glycerol-water mixtures with different mass concentration of glycerol as the liquid phase. The evolution of the gas−liquid interface during bubble breakup at the microfluidic T-junction is explored. The thinning of the bubble neck includes the squeezing stage and the rapid pinch-off stage. In the squeezing stage, the power law relation is found between the minimum width of the bubble neck and the time, and the values of exponents α1 and α2 are influenced by the viscous force. The values of pre-factors m_(1) and m_(2) are negatively correlated with the capillary number. In the rapid pinch-off stage, the thinning of the bubble neck is predominated by the surface tension, and the minimum width of the bubble neck can be scaled with the remaining time as power-law. The propagation of the bubble tip can be characterized by the power law between the movement distance and the time, with decreasing exponent as increased liquid viscosity.展开更多
A temperature and acoustic impedance simultaneous sensor based on forward stimulated Brillouin scattering(FSBS)in highly nonlinear fiber(HNLF)with high sensitivity and high accuracy is proposed and demonstrated in thi...A temperature and acoustic impedance simultaneous sensor based on forward stimulated Brillouin scattering(FSBS)in highly nonlinear fiber(HNLF)with high sensitivity and high accuracy is proposed and demonstrated in this paper.High-order acoustic modes(HOAMs)are used to achieve individual or simultaneous measurement of the two parameters.Transverse acoustic waves(TAWs)involved in the FSBS process can efficiently sense the mechanical or environmental changes outside the fiber cladding,which will be reflected in a linear shift of the acoustic resonance frequency.By analyzing the frequencies of specific scattering peaks,the temperature and acoustic impedance outside the fiber cladding can be obtained simultaneously.The highest measured temperature and acoustic impedance sensitivities are 184.93 k Hz/℃and444.56 k Hz/MRayl,and the measurement accuracies are 0.09℃and 0.009 MRayl,respectively,which are both at desirable levels.We believe this work can provide potential application solutions for sensing fields involving temperature or acoustic impedance measurements.展开更多
Microwave discharge plasma in liquid(MDPL)is a new type of water purification technology with a high mass transfer efficiency.It is a kind of low-temperature plasma technology.The reactive species produced by the disc...Microwave discharge plasma in liquid(MDPL)is a new type of water purification technology with a high mass transfer efficiency.It is a kind of low-temperature plasma technology.The reactive species produced by the discharge can efficiently act on the pollutants.To clarify the application prospects of MDPL in water treatment,the discharge performance,practical application,and pollutant degradation mechanism of MDPL were studied in this work.The effects of power,conductivity,pH,and Fe^(2+)concentration on the amount of reactive species produced by the discharge were explored.The most common and refractory perfluorinated compounds(perfluorooctanoic acid(PFOA)and perfluorooctane sulfonate(PFOS)in water environments are degraded by MDPL technology.The highest defluorination of PFOA was 98.8% and the highest defluorination of PFOS was 92.7%.The energy consumption efficiency of 50% defluorination(G_(50-F))of PFOA degraded by MDPL is 78.43 mg/kWh,PFOS is 42.19 mg/kWh.The results show that the MDPL technology is more efficient and cleaner for the degradation of perfluorinated compounds.Finally,the reaction path and pollutant degradation mechanisms of MDPL production were analyzed.The results showed that MDPL technology can produce a variety of reactive species and has a good treatment effect for refractory perfluorinated pollutants.展开更多
GeTe-based alloys are promising thermoelectric materials for use at medium temperatures owing to their excellent thermoelectric performance.In this study,Ge_(0.8-x)Mn_(0.1)Pb_(0.1)Sb_(x)Te alloys were obtained via vac...GeTe-based alloys are promising thermoelectric materials for use at medium temperatures owing to their excellent thermoelectric performance.In this study,Ge_(0.8-x)Mn_(0.1)Pb_(0.1)Sb_(x)Te alloys were obtained via vacuum melting and hot-press sintering.Sb doping effectively decreased the carrier concentration,resulting in an enhancement of the Seebeck coefficient and consequently imparting excellent electrical transport performance to the sample.With doping concentration increasing,the structure of the sample changed from rhombohedral to cubic,creating a more favorable band structure for electronic transport properties.The incorporation of Sb into GeTe intensifies the lattice defects within the material.The significant decrease in the lattice thermal conductivity of the Ge_(0.71)Mn_(0.1)Pb_(0.1)Sb_(0.09)Te alloy to 0.84 W m^(-1)K^(-1)at 323 K is primarily attributed to the phonon scattering effect emanating from the presence of edge dislocation,point defects,and inherent grain boundaries.Finally,the maximum ZT value of the Ge_(0.74)Mn_(0.1)Pb_(0.1)Sb_(0.06)Te alloy was~1.53773 K,which is a significant enhancement of 0.35 compared to the undoped Ge_(0.8)Mn_(0.1)Pb_(0.1)Te alloy.This substantial improvement underscores the positive impact of the selected doping elements and their concentrations on the overall thermoelectric performance of the alloy.展开更多
Using the blood oxygen levels dependent technology of magnetic resonance imaging (BLOD-fMRI), we aimed to explore the brain activation after visual stimulation by Chinese words. In the current study, 24 healthy volunt...Using the blood oxygen levels dependent technology of magnetic resonance imaging (BLOD-fMRI), we aimed to explore the brain activation after visual stimulation by Chinese words. In the current study, 24 healthy volunteers (12 males, 12 females, right-handed, mean age 26 ± 2 years) were prospectively included. The event related design was used in the current fMRI study when participants silently read all words appearing in the middle of the screen. Images were processed with Statistical Parametric Mapping 8 (SPM8) software, by using a general linear model (GLM). Group activations were extracted from the 2nd level group analysis with a threshold of p < 0.001, and it was shown that the main activated areas by silent reading tasks were regions involved in brain semantic processing, including middle temporal gyrus, fusiform gyrus, supplementary motor area, inferior frontal gyrus, cingulate gyrus, superior parietal lobule and inferior parietal lobule. It was also learnt that superior parietal lobule and middle temporal gyrus are related with semantic understanding, lenticular nucleus are related with semantic processing. This means, in addition to the cerebral cortex, subcortical nuclei is also very important to the processing of words in Chinese language.展开更多
In this paper, the composition, two-dimensional and three-dimensional microstructure of heat-resistant wrought aluminum alloy with strong oxidation resistance, heat resistance and easy processing are analyzed by using...In this paper, the composition, two-dimensional and three-dimensional microstructure of heat-resistant wrought aluminum alloy with strong oxidation resistance, heat resistance and easy processing are analyzed by using direct reading spectrometer, metallographic microscope and scanning electron microscope. The main alloy elements of heat-resistant forging aluminum alloy include Cu, Mg, Si, Ni and Fe. The α solid solution of each element in aluminum consists of S phase (Al<sub>2</sub>CuMg), Mg<sub>2</sub>Si phase, bright gray Al<sub>2</sub>CuNi phase and dark brown Al<sub>9</sub>FeNi phase. The distribution of each phase in the aluminum alloy is determined by the three-dimensional energy spectrum analysis of the microstructure, and the distribution of each phase in the crystal position is analyzed. The mechanism of heat resistance, easy processing type and wear resistance is obtained, which provides the theoretical basis for the development and use of heat-resistant forged aluminum alloy.展开更多
With the progress of society, there is an increasing need to tackle disorders of the central nervous system. Human brain tissue, unlike animal tissues, is an irreplaceable resource for the study of neurological diseas...With the progress of society, there is an increasing need to tackle disorders of the central nervous system. Human brain tissue, unlike animal tissues, is an irreplaceable resource for the study of neurological diseases (1)Aimed at scientific research and education, the roles of human brain tissue repositories are to acquire brain tissue from donors, prepare, process, and preserve collected samples,provide tissue to specific eligible facilities, and determine the characteristics of each tissue sample.展开更多
Objective:To observe the effects antiarrhythmic peptide 10(AAPIO) aon acute ventricular arrhythmia and the phosphorylation state of ischemic myocardium conncxin.Methods:Acute total ischemia and partial ischemia models...Objective:To observe the effects antiarrhythmic peptide 10(AAPIO) aon acute ventricular arrhythmia and the phosphorylation state of ischemic myocardium conncxin.Methods:Acute total ischemia and partial ischemia models were established by ceasing perfusion and ligating the left anterior descending coronary artery in SD rats.The effects of AAP10(1 mg/L) on the incidence rate of ischemia-induced ventricular arrhythmia were observed.The ischemic myocardium was sampled to detect total-Cx43 and NP-Cx43 by immunofluorcsecnt staining and western blotting,the total-Cx43 expression was detected through image analysis system by semi-quantitative analysis.Results:AAP10 could significantly decrease the incidence of ischemia-induced ventricular tachycardia and ventricular fibrillation.During ischemic stage,total ischemia(TI) and AAP10 total ischemia(ATI) groups were compared with partial ischemia(Pi) and AAP10 partial ischemia(API) groups.The rates of incidence for arrhythmia in the ATI and API groups(10%and 0%) were lower than those in the TI and PI groups(60%and 45%).The difference between the two groups was statistically significant(P=0.019,P=0.020).The semi-quantitative analysis results of the ischemic myocardium showed that the total-Cx43 protein expression distribution areas for TI.ATI,PI and API groups were significantly decreased compared with the control group.On the other hand,the NP-Cx43 distribution areas of TI,ATI,PI and API groups were significantly increased compared with the control group(P>0.05).AAP10 could increase the total-Cx43 expression in the ischemic area and decrease the NP-Cx43 expression.Western blot results were consistent with the results of immunofluorescence staining.Conclusions:AAP10 can significantly decrease the rate of incidence of acute ischemia-induced ventricular tachycardia and ventricular fibrillation.Acute ischemic ventricular arrhythmias may have a relationship with the decreased phosphorylation of Cx43 induced by ischemia.AAP10 may stimulate the phosphorylation of Cx43 by increasing the totai-Cx43 expression and decreasing the NP-Cx43 expression in the ischemic area,so as to decrease ventricular arrhythmia.展开更多
In the process of in situ leaching of uranium,the microstructure controls and influences the flow distribution,percolation characteristics,and reaction mechanism of lixivium in the pores of reservoir rocks and directl...In the process of in situ leaching of uranium,the microstructure controls and influences the flow distribution,percolation characteristics,and reaction mechanism of lixivium in the pores of reservoir rocks and directly affects the leaching of useful components.In this study,the pore throat,pore size distribution,and mineral composition of low-permeability uranium-bearing sandstone were quantitatively analyzed by high pressure mercury injection,nuclear magnetic resonance,X-ray diffraction,and wavelength-dispersive X-ray fluorescence.The distribution characteristics of pores and minerals in the samples were qualitatively analyzed using energy-dispersive scanning electron microscopy and multi-resolution CT images.Image registration with the landmarks algorithm provided by FEI Avizo was used to accurately match the CT images with different resolutions.The multi-scale and multi-mineral digital core model of low-permeability uranium-bearing sandstone is reconstructed through pore segmentation and mineral segmentation of fusion core scanning images.The results show that the pore structure of low-permeability uranium-bearing sandstone is complex and has multi-scale and multi-crossing characteristics.The intergranular pores determine the main seepage channel in the pore space,and the secondary pores have poor connectivity with other pores.Pyrite and coffinite are isolated from the connected pores and surrounded by a large number of clay minerals and ankerite cements,which increases the difficulty of uranium leaching.Clays and a large amount of ankerite cement are filled in the primary and secondary pores and pore throats of the low-permeability uraniumbearing sandstone,which significantly reduces the porosity of the movable fluid and results in low overall permeability of the cores.The multi-scale and multi-mineral digital core proposed in this study provides a basis for characterizing macroscopic and microscopic pore-throat structures and mineral distributions of low-permeability uranium-bearing sandstone and can better understand the seepage characteristics.展开更多
To investigate the damage localization effects of the thrust chamber wall caused by combustions in LOX/methane rocket engines, a fluid-structural coupling computational methodology with a multi-channel model is develo...To investigate the damage localization effects of the thrust chamber wall caused by combustions in LOX/methane rocket engines, a fluid-structural coupling computational methodology with a multi-channel model is developed to obtain 3-demensioanl thermal and structural responses.Heat and mechanical loads are calculated by a validated finite volume fluid-thermal coupling numerical method considering non-premixed combustion processes of propellants. The methodology is subsequently performed on an LOX/methane thrust chamber under cyclic operation. Results show that the heat loads of the thrust chamber wall are apparently non-uniform in the circumferential direction. There are noticeable disparities between different cooling channels in terms of temperature and strain distributions at the end of the hot run phase, which in turn leads to different temperature ranges, strain ranges, and residual strains during one cycle. With the work cycle proceeding, the circumferential localization effect of the residual strain would be significantly enhanced. A post-processing damage analysis reveals that the low-cycle fatigue damage accumulated in each cycle is almost unchanged, while the quasi static damage accumulated in a considered cycle declines until stabilized after several cycles. The maximum discrepancy of the predicted lives between different cooling channels is about 30%.展开更多
DEAR EDITOR,Bellamya purificata(Gastropoda:Caenogastropoda;Architaenioglossa;Viviparidae:Bellamyinae;Sinotaia),a homotypic synonym of S.purificata,is widely distributed in freshwater habitats in Asia.It is an economic...DEAR EDITOR,Bellamya purificata(Gastropoda:Caenogastropoda;Architaenioglossa;Viviparidae:Bellamyinae;Sinotaia),a homotypic synonym of S.purificata,is widely distributed in freshwater habitats in Asia.It is an economically important edible snail and plays a vital function in freshwater wetland ecology.However,genomic resources for this snail are lacking and no reference genome has been released.In this study,we constructed the first chromosome-level genome of B.purificata using PacBio long-read sequencing and high-throughput chromosome conformation capture(Hi-C)technology.展开更多
Primary age-related tauopathy(PART) is characterized by tau neurofibrillary tangles(NFTs) in the absence of amyloid plaque pathology. In the present study,we analyzed the distribution patterns of phosphorylated43-kDa ...Primary age-related tauopathy(PART) is characterized by tau neurofibrillary tangles(NFTs) in the absence of amyloid plaque pathology. In the present study,we analyzed the distribution patterns of phosphorylated43-kDa TAR DNA-binding protein(pTDP-43) in the brains of patients with PART. Immunohistochemistry and immunofluorescence double-labeling in multiple brain regions was performed on brain tissues from PART,Alzheimer's disease(AD), and aging control cases. We examined the regional distribution patterns of pTDP-43 intraneuronal inclusions in PART with Braak NFT stages[ 0 and B IV, and a Thal phase of 0(no beta-amyloid present). We found four stages which indicated potentially sequential dissemination of pTDP-43 in PART. Stage I was characterized by the presence of pTDP-43 lesions in the amygdala, stage II by such lesions in the hippocampus,stage III by spread of pTDP-43 to the neocortex, and stage IV by pTDP-43 lesions in the putamen, pallidum, and insular cortex. In general, the distribution pattern of pTDP-43 pathology in PART cases was similar to the early TDP-43 stages reported in AD, but tended to be more restricted to the limbic system. However, there were some differences in the distribution patterns of pTDP-43 between PART and AD, especially in the dentate gyrus of the hippocampus. Positive correlations were found in PART between the Braak NFT stage and the pTDP-43 stage and density.展开更多
For a typical pressurized system with a novel dual-stage gas pressure reducing regulator,a system model is established with modular models of various typical components. The simulation study on the whole working perio...For a typical pressurized system with a novel dual-stage gas pressure reducing regulator,a system model is established with modular models of various typical components. The simulation study on the whole working period shows that the general trends and magnitudes of simulation curves are in agreement with experimental measured curves. As the key component in the pressurized system, the regulator is studied by a series of numerical simulations to reveal the influences of various structure parameters on its stability. Furthermore, the variable ranges which can guarantee the stability of regulator and system are obtained to provide guidance for design. The modeling and analysis approach can be applied to other systems and components.展开更多
基金support from the National Natural Science Foundation of China(22209089,22178187)Natural Science Foundation of Shandong Province(ZR2022QB048,ZR2021MB006)+2 种基金Excellent Youth Science Foundation of Shandong Province(Overseas)(2023HWYQ-089)the Taishan Scholars Program of Shandong Province(tsqn201909091)Open Research Fund of School of Chemistry and Chemical Engineering,Henan Normal University.
文摘Aqueous zinc-halogen batteries are promising candidates for large-scale energy storage due to their abundant resources,intrinsic safety,and high theoretical capacity.Nevertheless,the uncontrollable zinc dendrite growth and spontaneous shuttle effect of active species have prohibited their practical implementation.Herein,a double-layered protective film based on zinc-ethylenediamine tetramethylene phosphonic acid(ZEA)artificial film and ZnF2-rich solid electrolyte interphase(SEI)layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic optimization.The ZEA-based artificial film shows strong affinity for the ZnF2-rich SEI layer,therefore effectively suppressing the SEI breakage and facilitating the construction of double-layered protective film on the zinc metal anode.Such double-layered architecture not only modulates Zn2+flux and suppresses the zinc dendrite growth,but also blocks the direct contact between the metal anode and electrolyte,thus mitigating the corrosion from the active species.When employing optimized metal anodes and electrolytes,the as-developed zinc-(dual)halogen batteries present high areal capacity and satisfactory cycling stability.This work provides a new avenue for developing aqueous zinc-(dual)halogen batteries.
基金supported by the National Natural Science Foundation of China(42372017 and 42072018)the Fundamental Research Funds for the Central Universities(2022CXTD24)。
文摘The Hehuang Valley,situated in the northeastern section of the Qinghai-Tibet Plateau,represents the upper reaches of the Yellow River(Fig.1A).It is a significant geographic region of origin for numerous Neolithic cultures,including the Majiayao,Zongri,and Qijia cultures(Dong et al.,2013).
文摘The accurate identification and diagnosis of chemical process faults are crucial for ensuring the safe and stable operation of production plants.The current hot topic in industrial process fault diagnosis research is data-driven methods.Most of the existing fault diagnosis methods focus on a single shallow or deep learning model.This paper proposes a novel hybrid fault diagnosis method to fully utilize various features to improve the accuracy of fault diagnosis.Furthermore,the method addresses the issue of incomplete data,which has been largely overlooked in the majority of existing research.Firstly,the variable data is effectively fitted using orthogonal non-negative matrix tri-factorization,and the missing data in the matrix is solved to construct a complete production condition relationship.Next,the support vector machine model and the deep residual contraction network model are trained in parallel to prediagnose process faults by mining linear and non-linear interaction features.Finally,a novel mapping relationship is established between the result and model levels using the multi-layer perceptron algorithm to complete the final diagnosis and evaluation of the fault.To demonstrate the effectiveness of the proposed method,we conducted extensive comparative experiments on the Tennessee Eastman dataset and the ethylene plant cracking unit dataset.The experimental results show that the method has advantages in different evaluation metrics.
文摘Through an example of a main transformer switch-in with load during the reverse transmission of a 750 kV power plan,the paper introduces the basic principle of transformer switch-in with load.EMTPE program that is used to establish a calculation model,at the same time mainly considers the excitation characteristics of the transformer,the transient model of the circuit breaker,and the model of high voltage transformer,and calculated the inrush current with transformer switch-in with load in this plan.During system debugging in the plan,the two sets of main transformers passed the closing and opening test,and the data of inrush current in the test are recorded and analyzed.The simulation calculation and measured data show that the results are consistent.The simulation calculation also shows that it is not recommended to perform on-load closing of the transformer except for special circumstances,because of the influence of hysteresis characteristic when the transformer was switched in with load or the terminal voltage of the transformer resumed normal level from a low one after an external near-end fault was cleared,which various transformer differential protection using the characteristics of inrush to implement block scheme may mal-operate.
基金supported by the National Natural Science Foundation of China under Grant No.52072196,52002200,52102106,52202262,22379081,22379080,Major Basic Research Program of Natural Science Foundation of Shandong Province under Grant No.ZR2020ZD09the Natural Science Foundation of Shandong Province under Grant No.ZR2020QE063,ZR202108180009,ZR2023QE059the Postdoctoral Program in Qingdao under No.QDBSH20220202019.
文摘Designing cathode possessing crystalline@amorphous core-shell structure with both active core and shell is a meaningful work for resolving the low specific capacity,unstable cycling performance and sluggish reaction kinetics issues of rechargeable magnesium batteries(RMBs)by providing more active sites as well as releasing inner stress during cycling.Herein,WO_(3)@WO_(3-x)S_(x) owning crystalline@amorphous core-shell structure containing both active core and active shell is constructed successfully by introducing S into metastable WO3 structure under temperaturefield applying.In such structure,amorphous shell would provide continuous Mg^(2+)diffusion channels due to its isotropy property for most Mg^(2+)migrating rapidly to interface and then adsorb at ions reservoir formed by interfacial electricfield for increasing specific capacity.It also makes security for stable structure of WO_(3)@WO_(3-x)S_(x) by alleviating volume expansion of crystalline core WO_(3) during cycling to prolong cycling life.Additionally,“softer”ions S^(2-)would weaken interaction between hard acid Mg^(2+) and ionic lattice to enhance Mg^(2+)storage kinetics.Therefore,WO_(3)@WO_(3-x)S_(x) delivers the superior cycling performance(1000 cycles with 83.3%),rate capability(88.5 mAh g^(-1) at 1000 mA g^(-1))and specific capacity(about 150 mAh g^(-1) at 50 mA g^(-1)),which is near 2 times higher than that of WO3.It is believed that the crystalline@amorphous core-shell structure with both active core and shell designing via doping strategy is enlightening for the development of high-performance RMBs,and such design can be extended to other energy storage devices for better electrochemical performance.
基金supports for this project from State Key Laboratory of Chemical Safety(SKLCS–2024001)are gratefully acknowledged。
文摘Bubble breakup at T-junction microchannels is the basis for the numbering-up of gas−liquid two-phase flow in parallelized microchannels. This article presents the bubble breakup in viscous liquids at a microfluidic T-junction. Nitrogen is used as the gas phase, and glycerol-water mixtures with different mass concentration of glycerol as the liquid phase. The evolution of the gas−liquid interface during bubble breakup at the microfluidic T-junction is explored. The thinning of the bubble neck includes the squeezing stage and the rapid pinch-off stage. In the squeezing stage, the power law relation is found between the minimum width of the bubble neck and the time, and the values of exponents α1 and α2 are influenced by the viscous force. The values of pre-factors m_(1) and m_(2) are negatively correlated with the capillary number. In the rapid pinch-off stage, the thinning of the bubble neck is predominated by the surface tension, and the minimum width of the bubble neck can be scaled with the remaining time as power-law. The propagation of the bubble tip can be characterized by the power law between the movement distance and the time, with decreasing exponent as increased liquid viscosity.
文摘A temperature and acoustic impedance simultaneous sensor based on forward stimulated Brillouin scattering(FSBS)in highly nonlinear fiber(HNLF)with high sensitivity and high accuracy is proposed and demonstrated in this paper.High-order acoustic modes(HOAMs)are used to achieve individual or simultaneous measurement of the two parameters.Transverse acoustic waves(TAWs)involved in the FSBS process can efficiently sense the mechanical or environmental changes outside the fiber cladding,which will be reflected in a linear shift of the acoustic resonance frequency.By analyzing the frequencies of specific scattering peaks,the temperature and acoustic impedance outside the fiber cladding can be obtained simultaneously.The highest measured temperature and acoustic impedance sensitivities are 184.93 k Hz/℃and444.56 k Hz/MRayl,and the measurement accuracies are 0.09℃and 0.009 MRayl,respectively,which are both at desirable levels.We believe this work can provide potential application solutions for sensing fields involving temperature or acoustic impedance measurements.
基金supported by National Natural Science Foundation of China(Nos.12475258,12111530008 and 11675031)Major Scientific Research Project of Hebei Transportation Investment Group in 2024([202]155)the support of the Fundamental Research Funds for the Central Universities(No.3132023503)。
文摘Microwave discharge plasma in liquid(MDPL)is a new type of water purification technology with a high mass transfer efficiency.It is a kind of low-temperature plasma technology.The reactive species produced by the discharge can efficiently act on the pollutants.To clarify the application prospects of MDPL in water treatment,the discharge performance,practical application,and pollutant degradation mechanism of MDPL were studied in this work.The effects of power,conductivity,pH,and Fe^(2+)concentration on the amount of reactive species produced by the discharge were explored.The most common and refractory perfluorinated compounds(perfluorooctanoic acid(PFOA)and perfluorooctane sulfonate(PFOS)in water environments are degraded by MDPL technology.The highest defluorination of PFOA was 98.8% and the highest defluorination of PFOS was 92.7%.The energy consumption efficiency of 50% defluorination(G_(50-F))of PFOA degraded by MDPL is 78.43 mg/kWh,PFOS is 42.19 mg/kWh.The results show that the MDPL technology is more efficient and cleaner for the degradation of perfluorinated compounds.Finally,the reaction path and pollutant degradation mechanisms of MDPL production were analyzed.The results showed that MDPL technology can produce a variety of reactive species and has a good treatment effect for refractory perfluorinated pollutants.
基金financially supported by the National Natural Science Foundation of China(Nos.12204355,52272210,12364006 and 12164011)the Open Project of State Key Laboratory of Superhard Materials,Jilin University(No.202110)the Natural Science Foundation of Shandong Province(Nos.ZR2022QA018,ZR2023QE282,ZR2023ME001 and ZR2023MF081)
文摘GeTe-based alloys are promising thermoelectric materials for use at medium temperatures owing to their excellent thermoelectric performance.In this study,Ge_(0.8-x)Mn_(0.1)Pb_(0.1)Sb_(x)Te alloys were obtained via vacuum melting and hot-press sintering.Sb doping effectively decreased the carrier concentration,resulting in an enhancement of the Seebeck coefficient and consequently imparting excellent electrical transport performance to the sample.With doping concentration increasing,the structure of the sample changed from rhombohedral to cubic,creating a more favorable band structure for electronic transport properties.The incorporation of Sb into GeTe intensifies the lattice defects within the material.The significant decrease in the lattice thermal conductivity of the Ge_(0.71)Mn_(0.1)Pb_(0.1)Sb_(0.09)Te alloy to 0.84 W m^(-1)K^(-1)at 323 K is primarily attributed to the phonon scattering effect emanating from the presence of edge dislocation,point defects,and inherent grain boundaries.Finally,the maximum ZT value of the Ge_(0.74)Mn_(0.1)Pb_(0.1)Sb_(0.06)Te alloy was~1.53773 K,which is a significant enhancement of 0.35 compared to the undoped Ge_(0.8)Mn_(0.1)Pb_(0.1)Te alloy.This substantial improvement underscores the positive impact of the selected doping elements and their concentrations on the overall thermoelectric performance of the alloy.
文摘Using the blood oxygen levels dependent technology of magnetic resonance imaging (BLOD-fMRI), we aimed to explore the brain activation after visual stimulation by Chinese words. In the current study, 24 healthy volunteers (12 males, 12 females, right-handed, mean age 26 ± 2 years) were prospectively included. The event related design was used in the current fMRI study when participants silently read all words appearing in the middle of the screen. Images were processed with Statistical Parametric Mapping 8 (SPM8) software, by using a general linear model (GLM). Group activations were extracted from the 2nd level group analysis with a threshold of p < 0.001, and it was shown that the main activated areas by silent reading tasks were regions involved in brain semantic processing, including middle temporal gyrus, fusiform gyrus, supplementary motor area, inferior frontal gyrus, cingulate gyrus, superior parietal lobule and inferior parietal lobule. It was also learnt that superior parietal lobule and middle temporal gyrus are related with semantic understanding, lenticular nucleus are related with semantic processing. This means, in addition to the cerebral cortex, subcortical nuclei is also very important to the processing of words in Chinese language.
文摘In this paper, the composition, two-dimensional and three-dimensional microstructure of heat-resistant wrought aluminum alloy with strong oxidation resistance, heat resistance and easy processing are analyzed by using direct reading spectrometer, metallographic microscope and scanning electron microscope. The main alloy elements of heat-resistant forging aluminum alloy include Cu, Mg, Si, Ni and Fe. The α solid solution of each element in aluminum consists of S phase (Al<sub>2</sub>CuMg), Mg<sub>2</sub>Si phase, bright gray Al<sub>2</sub>CuNi phase and dark brown Al<sub>9</sub>FeNi phase. The distribution of each phase in the aluminum alloy is determined by the three-dimensional energy spectrum analysis of the microstructure, and the distribution of each phase in the crystal position is analyzed. The mechanism of heat resistance, easy processing type and wear resistance is obtained, which provides the theoretical basis for the development and use of heat-resistant forged aluminum alloy.
文摘With the progress of society, there is an increasing need to tackle disorders of the central nervous system. Human brain tissue, unlike animal tissues, is an irreplaceable resource for the study of neurological diseases (1)Aimed at scientific research and education, the roles of human brain tissue repositories are to acquire brain tissue from donors, prepare, process, and preserve collected samples,provide tissue to specific eligible facilities, and determine the characteristics of each tissue sample.
基金supported by the National Natural Science Foundation of China(No:81300150)
文摘Objective:To observe the effects antiarrhythmic peptide 10(AAPIO) aon acute ventricular arrhythmia and the phosphorylation state of ischemic myocardium conncxin.Methods:Acute total ischemia and partial ischemia models were established by ceasing perfusion and ligating the left anterior descending coronary artery in SD rats.The effects of AAP10(1 mg/L) on the incidence rate of ischemia-induced ventricular arrhythmia were observed.The ischemic myocardium was sampled to detect total-Cx43 and NP-Cx43 by immunofluorcsecnt staining and western blotting,the total-Cx43 expression was detected through image analysis system by semi-quantitative analysis.Results:AAP10 could significantly decrease the incidence of ischemia-induced ventricular tachycardia and ventricular fibrillation.During ischemic stage,total ischemia(TI) and AAP10 total ischemia(ATI) groups were compared with partial ischemia(Pi) and AAP10 partial ischemia(API) groups.The rates of incidence for arrhythmia in the ATI and API groups(10%and 0%) were lower than those in the TI and PI groups(60%and 45%).The difference between the two groups was statistically significant(P=0.019,P=0.020).The semi-quantitative analysis results of the ischemic myocardium showed that the total-Cx43 protein expression distribution areas for TI.ATI,PI and API groups were significantly decreased compared with the control group.On the other hand,the NP-Cx43 distribution areas of TI,ATI,PI and API groups were significantly increased compared with the control group(P>0.05).AAP10 could increase the total-Cx43 expression in the ischemic area and decrease the NP-Cx43 expression.Western blot results were consistent with the results of immunofluorescence staining.Conclusions:AAP10 can significantly decrease the rate of incidence of acute ischemia-induced ventricular tachycardia and ventricular fibrillation.Acute ischemic ventricular arrhythmias may have a relationship with the decreased phosphorylation of Cx43 induced by ischemia.AAP10 may stimulate the phosphorylation of Cx43 by increasing the totai-Cx43 expression and decreasing the NP-Cx43 expression in the ischemic area,so as to decrease ventricular arrhythmia.
基金This work was supported by the National Natural Science Foundation of China(No.11775107)the Key Projects of Education Department of Hunan Province of China(No.16A184).
文摘In the process of in situ leaching of uranium,the microstructure controls and influences the flow distribution,percolation characteristics,and reaction mechanism of lixivium in the pores of reservoir rocks and directly affects the leaching of useful components.In this study,the pore throat,pore size distribution,and mineral composition of low-permeability uranium-bearing sandstone were quantitatively analyzed by high pressure mercury injection,nuclear magnetic resonance,X-ray diffraction,and wavelength-dispersive X-ray fluorescence.The distribution characteristics of pores and minerals in the samples were qualitatively analyzed using energy-dispersive scanning electron microscopy and multi-resolution CT images.Image registration with the landmarks algorithm provided by FEI Avizo was used to accurately match the CT images with different resolutions.The multi-scale and multi-mineral digital core model of low-permeability uranium-bearing sandstone is reconstructed through pore segmentation and mineral segmentation of fusion core scanning images.The results show that the pore structure of low-permeability uranium-bearing sandstone is complex and has multi-scale and multi-crossing characteristics.The intergranular pores determine the main seepage channel in the pore space,and the secondary pores have poor connectivity with other pores.Pyrite and coffinite are isolated from the connected pores and surrounded by a large number of clay minerals and ankerite cements,which increases the difficulty of uranium leaching.Clays and a large amount of ankerite cement are filled in the primary and secondary pores and pore throats of the low-permeability uraniumbearing sandstone,which significantly reduces the porosity of the movable fluid and results in low overall permeability of the cores.The multi-scale and multi-mineral digital core proposed in this study provides a basis for characterizing macroscopic and microscopic pore-throat structures and mineral distributions of low-permeability uranium-bearing sandstone and can better understand the seepage characteristics.
文摘To investigate the damage localization effects of the thrust chamber wall caused by combustions in LOX/methane rocket engines, a fluid-structural coupling computational methodology with a multi-channel model is developed to obtain 3-demensioanl thermal and structural responses.Heat and mechanical loads are calculated by a validated finite volume fluid-thermal coupling numerical method considering non-premixed combustion processes of propellants. The methodology is subsequently performed on an LOX/methane thrust chamber under cyclic operation. Results show that the heat loads of the thrust chamber wall are apparently non-uniform in the circumferential direction. There are noticeable disparities between different cooling channels in terms of temperature and strain distributions at the end of the hot run phase, which in turn leads to different temperature ranges, strain ranges, and residual strains during one cycle. With the work cycle proceeding, the circumferential localization effect of the residual strain would be significantly enhanced. A post-processing damage analysis reveals that the low-cycle fatigue damage accumulated in each cycle is almost unchanged, while the quasi static damage accumulated in a considered cycle declines until stabilized after several cycles. The maximum discrepancy of the predicted lives between different cooling channels is about 30%.
基金supported by the Central Public-Interest Scientific Institution Basal Research Fund,CAFS(2021XT703)Central Public-interest Scientific Institution Basal Research Fund,Freshwater Fisheries Research Center,CAFS(2021JBFM07)。
文摘DEAR EDITOR,Bellamya purificata(Gastropoda:Caenogastropoda;Architaenioglossa;Viviparidae:Bellamyinae;Sinotaia),a homotypic synonym of S.purificata,is widely distributed in freshwater habitats in Asia.It is an economically important edible snail and plays a vital function in freshwater wetland ecology.However,genomic resources for this snail are lacking and no reference genome has been released.In this study,we constructed the first chromosome-level genome of B.purificata using PacBio long-read sequencing and high-throughput chromosome conformation capture(Hi-C)technology.
基金supported by the National Science Foundation China(91632109 to JHZ,KQZ and HJH)the Zhejiang Provincial Natural Science Foundation(LY16H090013 to KQZ)the Zhejiang Medical and Health Science and Technology Plan Project(WKJ20132-009 to KQZ)
文摘Primary age-related tauopathy(PART) is characterized by tau neurofibrillary tangles(NFTs) in the absence of amyloid plaque pathology. In the present study,we analyzed the distribution patterns of phosphorylated43-kDa TAR DNA-binding protein(pTDP-43) in the brains of patients with PART. Immunohistochemistry and immunofluorescence double-labeling in multiple brain regions was performed on brain tissues from PART,Alzheimer's disease(AD), and aging control cases. We examined the regional distribution patterns of pTDP-43 intraneuronal inclusions in PART with Braak NFT stages[ 0 and B IV, and a Thal phase of 0(no beta-amyloid present). We found four stages which indicated potentially sequential dissemination of pTDP-43 in PART. Stage I was characterized by the presence of pTDP-43 lesions in the amygdala, stage II by such lesions in the hippocampus,stage III by spread of pTDP-43 to the neocortex, and stage IV by pTDP-43 lesions in the putamen, pallidum, and insular cortex. In general, the distribution pattern of pTDP-43 pathology in PART cases was similar to the early TDP-43 stages reported in AD, but tended to be more restricted to the limbic system. However, there were some differences in the distribution patterns of pTDP-43 between PART and AD, especially in the dentate gyrus of the hippocampus. Positive correlations were found in PART between the Braak NFT stage and the pTDP-43 stage and density.
基金financially supported by the National Natural Science Foundation of China (No.11101023)the China Scholarship Council (No.201203070237)
文摘For a typical pressurized system with a novel dual-stage gas pressure reducing regulator,a system model is established with modular models of various typical components. The simulation study on the whole working period shows that the general trends and magnitudes of simulation curves are in agreement with experimental measured curves. As the key component in the pressurized system, the regulator is studied by a series of numerical simulations to reveal the influences of various structure parameters on its stability. Furthermore, the variable ranges which can guarantee the stability of regulator and system are obtained to provide guidance for design. The modeling and analysis approach can be applied to other systems and components.
