We present Parameter Quantification Network(PQ-Net),a regression deep convolutional neural network providing quantitative analysis of powder X-ray diffraction patterns from multi-phase systems.The network is tested ag...We present Parameter Quantification Network(PQ-Net),a regression deep convolutional neural network providing quantitative analysis of powder X-ray diffraction patterns from multi-phase systems.The network is tested against simulated and experimental datasets of increasing complexity with the last one being an X-ray diffraction computed tomography dataset of a multi-phase Ni-Pd/CeO_(2)-ZrO_(2)/Al_(2)O_(3) catalytic material system consisting of ca.20,000 diffraction patterns.It is shown that the network predicts accurate scale factor,lattice parameter and crystallite size maps for all phases,which are comparable to those obtained through full profile analysis using the Rietveld method,also providing a reliable uncertainty measure on the results.The main advantage of PQNet is its ability to yield these results orders of magnitude faster showing its potential as a tool for real-time diffraction data analysis during in situ/operando experiments.展开更多
Classification of sheep behaviour from a sequence of tri-axial accelerometer data has the potential to enhance sheep management.Sheep behaviour is inherently imbalanced(e.g.,more ruminating than walking)resulting in u...Classification of sheep behaviour from a sequence of tri-axial accelerometer data has the potential to enhance sheep management.Sheep behaviour is inherently imbalanced(e.g.,more ruminating than walking)resulting in underperforming classification for the minority activities which hold importance.Existing works have not addressed class imbalance and use traditional machine learning techniques,e.g.,Random Forest(RF).We investigated Deep Learning(DL)models,namely,Long Short Term Memory(LSTM)and Bidirectional LSTM(BLSTM),appropriate for sequential data,from imbalanced data.Two data sets were collected in normal grazing conditions using jaw-mounted and earmounted sensors.Novel to this study,alongside typical single classes,e.g.,walking,depending on the behaviours,data samples were labelled with compound classes,e.g.,walking_-grazing.The number of steps a sheep performed in the observed 10 s time window was also recorded and incorporated in the models.We designed several multi-class classification studies with imbalance being addressed using synthetic data.DL models achieved superior performance to traditional ML models,especially with augmented data(e.g.,4-Class+Steps:LSTM 88.0%,RF 82.5%).DL methods showed superior generalisability on unseen sheep(i.e.,F1-score:BLSTM 0.84,LSTM 0.83,RF 0.65).LSTM,BLSTM and RF achieved sub-millisecond average inference time,making them suitable for real-time applications.The results demonstrate the effectiveness of DL models for sheep behaviour classification in grazing conditions.The results also demonstrate the DL techniques can generalise across different sheep.The study presents a strong foundation of the development of such models for real-time animal monitoring.展开更多
基金We would like to thank Marco di Michiel(ID15A,ESRF)and Jakub Drnec(ID31,ESRF)for preparing beamline instrumentation and setup and for their help with the experimental XRD-CT data acquisition.We acknowledge ESRF for beamtime.Finden acknowledges funding through the Innovate UK Analysis for Innovators(A4i)program(Project No:106107)A.M.B.acknowledges EPSRC(grants EP/R026815/1 and EP/S016481/1).
文摘We present Parameter Quantification Network(PQ-Net),a regression deep convolutional neural network providing quantitative analysis of powder X-ray diffraction patterns from multi-phase systems.The network is tested against simulated and experimental datasets of increasing complexity with the last one being an X-ray diffraction computed tomography dataset of a multi-phase Ni-Pd/CeO_(2)-ZrO_(2)/Al_(2)O_(3) catalytic material system consisting of ca.20,000 diffraction patterns.It is shown that the network predicts accurate scale factor,lattice parameter and crystallite size maps for all phases,which are comparable to those obtained through full profile analysis using the Rietveld method,also providing a reliable uncertainty measure on the results.The main advantage of PQNet is its ability to yield these results orders of magnitude faster showing its potential as a tool for real-time diffraction data analysis during in situ/operando experiments.
文摘Classification of sheep behaviour from a sequence of tri-axial accelerometer data has the potential to enhance sheep management.Sheep behaviour is inherently imbalanced(e.g.,more ruminating than walking)resulting in underperforming classification for the minority activities which hold importance.Existing works have not addressed class imbalance and use traditional machine learning techniques,e.g.,Random Forest(RF).We investigated Deep Learning(DL)models,namely,Long Short Term Memory(LSTM)and Bidirectional LSTM(BLSTM),appropriate for sequential data,from imbalanced data.Two data sets were collected in normal grazing conditions using jaw-mounted and earmounted sensors.Novel to this study,alongside typical single classes,e.g.,walking,depending on the behaviours,data samples were labelled with compound classes,e.g.,walking_-grazing.The number of steps a sheep performed in the observed 10 s time window was also recorded and incorporated in the models.We designed several multi-class classification studies with imbalance being addressed using synthetic data.DL models achieved superior performance to traditional ML models,especially with augmented data(e.g.,4-Class+Steps:LSTM 88.0%,RF 82.5%).DL methods showed superior generalisability on unseen sheep(i.e.,F1-score:BLSTM 0.84,LSTM 0.83,RF 0.65).LSTM,BLSTM and RF achieved sub-millisecond average inference time,making them suitable for real-time applications.The results demonstrate the effectiveness of DL models for sheep behaviour classification in grazing conditions.The results also demonstrate the DL techniques can generalise across different sheep.The study presents a strong foundation of the development of such models for real-time animal monitoring.
