MoS_(2)targets were irradiated by infra-red(IR)pulsed laser in a high vacuum to determine hot plasma parameters,atomic,molecular and ion emission,and angular and charge state distributions.In this way,pulsed laser dep...MoS_(2)targets were irradiated by infra-red(IR)pulsed laser in a high vacuum to determine hot plasma parameters,atomic,molecular and ion emission,and angular and charge state distributions.In this way,pulsed laser deposition(PLD)of thin films on graphene oxide substrates was also realized.An Nd:YAG laser,operating at the 1064 nm wavelength with a 5 ns pulse duration and up to a 1 J pulse energy,in a single pulse or at a 10 Hz repetition rate,was employed.Ablation yield was measured as a function of the laser fluence.Plasma was characterized using different analysis techniques,such as time-of-flight measurements,quadrupole mass spectrometry and fast CCD visible imaging.The so-produced films were characterized by composition,thickness,roughness,wetting ability,and morphology.When compared to the MoS_(2)targets,they show a slight decrease of S with respect to Mo,due to higher ablation yield,low fusion temperature and high sublimation in vacuum.The pulsed IR laser deposited Mo Sx(with 1<x<2)films are uniform,with a thickness of about 130 nm,a roughness of about 50 nm and a higher wettability than the MoS_(2)targets.Some potential applications of the pulsed IR laser-deposited Mo Sx films are also presented and discussed.展开更多
A ns Nd:YAG pulsed laser has been employed to produce plasma from the interaction with a dense target,generating continuum and UV and soft x-ray emission depending on the laser parameters and target properties.The las...A ns Nd:YAG pulsed laser has been employed to produce plasma from the interaction with a dense target,generating continuum and UV and soft x-ray emission depending on the laser parameters and target properties.The laser hits solid and gaseous targets producing plasma in high vacuum,which was investigated by employing a silicon carbide detector.The two different interaction mechanisms were studied,as well as their dependence on the atomic number.The photon emission from laser-generated plasma produced by solid targets,such as boron nitride(BN)and other elements(Al,Cu,Sn and Ta)and compounds such as polyethylene,has been compared with that coming from plasma produced by irradiating different gas-puff targets based on N_(2)and other gases(Ar,Xe,Kr,SF_(6)).The experimental results demonstrated that the yields are comparable and,in both cases,increase proportionally to the target atomic number.The obtained results,focusing the attention on the advantages and drawbacks of the employed targets,are presented and discussed.展开更多
基金supported by OP RDE,MEYS,Czech Republic under the project CANAM OP(No.CZ.02.1.01/0.0/0.0/16_013/0001812)by the Czech Science Foundation GACR(No.23-06702S)。
文摘MoS_(2)targets were irradiated by infra-red(IR)pulsed laser in a high vacuum to determine hot plasma parameters,atomic,molecular and ion emission,and angular and charge state distributions.In this way,pulsed laser deposition(PLD)of thin films on graphene oxide substrates was also realized.An Nd:YAG laser,operating at the 1064 nm wavelength with a 5 ns pulse duration and up to a 1 J pulse energy,in a single pulse or at a 10 Hz repetition rate,was employed.Ablation yield was measured as a function of the laser fluence.Plasma was characterized using different analysis techniques,such as time-of-flight measurements,quadrupole mass spectrometry and fast CCD visible imaging.The so-produced films were characterized by composition,thickness,roughness,wetting ability,and morphology.When compared to the MoS_(2)targets,they show a slight decrease of S with respect to Mo,due to higher ablation yield,low fusion temperature and high sublimation in vacuum.The pulsed IR laser deposited Mo Sx(with 1<x<2)films are uniform,with a thickness of about 130 nm,a roughness of about 50 nm and a higher wettability than the MoS_(2)targets.Some potential applications of the pulsed IR laser-deposited Mo Sx films are also presented and discussed.
文摘A ns Nd:YAG pulsed laser has been employed to produce plasma from the interaction with a dense target,generating continuum and UV and soft x-ray emission depending on the laser parameters and target properties.The laser hits solid and gaseous targets producing plasma in high vacuum,which was investigated by employing a silicon carbide detector.The two different interaction mechanisms were studied,as well as their dependence on the atomic number.The photon emission from laser-generated plasma produced by solid targets,such as boron nitride(BN)and other elements(Al,Cu,Sn and Ta)and compounds such as polyethylene,has been compared with that coming from plasma produced by irradiating different gas-puff targets based on N_(2)and other gases(Ar,Xe,Kr,SF_(6)).The experimental results demonstrated that the yields are comparable and,in both cases,increase proportionally to the target atomic number.The obtained results,focusing the attention on the advantages and drawbacks of the employed targets,are presented and discussed.
